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We report the magnetic diffraction pattern and spin wave excitations in (CD$_3$)$_2$ND$_2$[Mn(DCO$_2$)$_3$] measured using elastic and inelastic neutron scattering. The magnetic structure is shown to be a G-type antiferromagnet with moments…

Strongly Correlated Electrons · Physics 2017-10-02 H. C. Walker , H. D. Duncan , M. D. Le , D. A. Keen , D. J. Voneshen , A. E. Phillips

The structural and magnetic interactions in stoichiometric (Mn$_3$SnC), carbon deficient (Mn$_3$SnC$_{0.8}$) and tin deficient (Mn$_3$Sn$_{0.85}$C) antiperovskite compounds are studied using x-ray absorption fine structure spectroscopy and…

Materials Science · Physics 2020-04-02 V. N. Gaonkar , E. T. Dias , A. Das , A. K. Nigam , K. R. Priolkar

We have studied the structural phase transition of multiferroic YMnO$_3$ from first principles. Using group-theoretical analysis and first-principles density functional calculations of the total energy and phonons, we perform a systematic…

Materials Science · Physics 2009-11-11 Craig J. Fennie , Karin M. Rabe

We have analyzed the experimental evidence of charge and orbital ordering in La0.5Sr1.5MnO4 using first principles band structure calculations. Our results suggest the presence of two types of Mn sites in the system. One of the Mn sites…

Strongly Correlated Electrons · Physics 2009-11-07 Priya Mahadevan , K. Terakura , D. D. Sarma

We studied the crystal and magnetic structure of the La$_{1-x}$Ca$_{x}$MnO$_{3}$ compound for $(0.11\leq x\leq 0.175)$ using stoichiometric samples. For $x<0.13$ the system's ground state is insulating canted antiferromagnetic. For $0.13\le…

Strongly Correlated Electrons · Physics 2009-11-11 M. Pissas , I. Margiolaki , G. Papavassiliou , D. Stamopoulos , D. Argyriou

A phenomenological theory of magnetic states in noncentrosymmetric tetragonal antiferromagnets is developed, which has to include homogeneous and inhomogeneous terms (Lifshitz-invariants) derived from Dzyaloshinskii-Moriya couplings.…

Strongly Correlated Electrons · Physics 2009-11-07 A. N. Bogdanov , U. K. Roessler , M. Wolf , K. -H. Muller

Cooperative Jahn-Teller ordering is well-known to drive the cubic $Fd\overline{3}m$ to tetragonal $I$4$_1$/$amd$ structural distortion in Mn$_3$O$_4$ at 1170 $^{\circ}$C. Further structural distortion occurs in Mn$_3$O$_4$ upon magnetic…

Materials Science · Physics 2014-08-26 Moureen C. Kemei , Jaye K. Harada , Ram Seshadri , Matthew R. Suchomel

Magnetic, dielectric and calorimetric studies on 0.9BiFeO3-0.1BaTiO3 indicate strong magnetoelectric coupling. XRD studies reveal a very remarkable change in the rhombohedral distortion angle and a significant shift in the atomic positions…

Materials Science · Physics 2009-11-13 Anar Singh , Vibhav Pandey , R. K. Kotnala , Dhananjai Pandey

We study in this paper bond distortion effect on electric polarization in spiral multiferroic magnets based on cluster and chain models. The bond distortion break inversion symmetry and modify the $d$-$p$ hybridization. Consequently, it…

Strongly Correlated Electrons · Physics 2015-06-04 Hong-Bo Chen , Yi Zhou , You-Quan Li

The complex interplay between the 3d and 4f moments in hexagonal ErMnO3 is investigated by magnetization, optical second harmonic generation, and neutron-diffraction measurements. We revise the phase diagram and provide a microscopic model…

Strongly Correlated Electrons · Physics 2012-11-14 D. Meier , H. Ryll , K. Kiefer , B. Klemke , J. -U. Hoffmann , R. Ramesh , M. Fiebig

Two-dimensional (2D) multiferroics exhibit cross-control capacity between magnetic and electric responses in reduced spatial domain, making them well suited for next-generation nanoscale devices; however, progress has been slow in…

Materials Science · Physics 2020-05-15 Jing Shang , Chun Li , Aijun Du , Ting Liao , Yuantong Gu , Yandong Ma , Liangzhi Kou , Changfeng Chen

The structure and magnetic properties of Mn1+xV2-xO4 (0<x<=1), a complex frustrated system, were investigated by heat capacity, magnetization, x-ray diffraction, and neutron diffraction measurements. For x<=0.3, a cubic-to-tetragonal (c >…

Strongly Correlated Electrons · Physics 2020-10-07 J. L. Jiao , H. P. Zhang , Q. Huang , W. Wang , G. Wang , Q. Ren , R. Sinclair , G. T. Lin , A. Huq , H. Cao , H. D. Zhou , M. Z. Li , J. Ma

The functional properties of transition metal perovskite oxides are known to result from a complex interplay of magnetism, polarization, strain, and stoichiometry. Here, we show that for materials with a cooperative Jahn-Teller distortion,…

Materials Science · Physics 2021-01-04 Chiara Ricca , Nicolas Niederhauser , Ulrich Aschauer

With a combined ab initio density functional and model Hamiltonian approach we establish that in the recently discovered multiferroic phase of the manganite Sr$_{1/2}$Ba$_{1/2}$MnO$_{3}$ the polar distortion of Mn and O ions is stabilized…

Materials Science · Physics 2015-03-09 Gianluca Giovannetti , Sanjeev Kumar , Carmine Ortix , Massimo Capone , Jeroen van den Brink

The magnetic and multiferroic phase diagram of Mn$_{0.85}$Co$_{0.15}$WO$_4$ single crystals is investigated by means of magnetic, heat capacity, dielectric, polarization, and neutron scattering experiments. Three magnetic phase transitions…

Strongly Correlated Electrons · Physics 2010-12-01 R. P. Chaudhury , F. Ye , J. A. Fernandez-Baca , Y. -Q. Wang , Y. Y. Sun , B. Lorenz , H. A. Mook , C. W. Chu

The effect of uniaxial strain on electronic structure and magnetism in LaMnO$_3$ is studied from a model Hamiltonian that illustrates the competition between the Jahn-Teller, super exchange, and double exchange interactions. We retain in…

Materials Science · Physics 2010-12-07 B. R. K. Nanda , S. Satpathy

The ferroelectric order and magnetic field induced effects observed in the spiral phase of MnWO4 are described theoretically. It is demonstrated explicitly that the Dzyaloshinskii-Moriya antisymmetric interactions contribute to the…

Strongly Correlated Electrons · Physics 2010-01-25 P. Toledano , B. Mettout , W. Schranz , G. Krexner

We investigated the static and dynamic magnetic properties of the polar ferrimagnet Mn$_2$Mo$_3$O$_8$ in three magnetically ordered phases via magnetization, magnetic torque, and THz absorption spectroscopy measurements. The observed…

First-principles density functional theory calculations have been performed to understand the electronic structure and orbital polarization of LaNiO$_3$ with a reduced coordination and under strain. From the slab calculation to simulate…

Materials Science · Physics 2011-10-03 Myung Joon Han , Michel van Veenendaal

The crystal and magnetic structure of multiferroic LiFe(WO$_4$)$_2$ were investigated by temperature and magnetic-field dependent specific heat, susceptibility and neutron diffraction experiments on single crystals. Considering only the two…

Strongly Correlated Electrons · Physics 2021-04-21 S. Biesenkamp , D. Gorkov , D. Brüning , A. Bertin , T. Fröhlich , X. Fabrèges , A. Gukasov , M. Meven , P. Becker , L. Bohatý , T. Lorenz , M. Braden