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Two-dimensional (2D) hexagonal boron nitride (BN) nanosheets are excellent dielectric substrate for graphene, molybdenum disulfide and many other 2D nanomaterials based electronic and photonic devices. To optimize the performance of these…

A comprehensive uncertainty quantification framework has been developed for integrating computational and experimental kinetic data and to identify active sites and reaction mechanisms in catalysis. Three hypotheses regarding the active…

Chemical Physics · Physics 2017-10-11 Eric A. Walker , Donald Mitchell , Gabriel A. Terejanu , Andreas Heyden

Ferroelectric nematic liquid crystals represent not only interesting fundamental science, but they also hold promise for storage capacitors with high power density or new information display technology having sub-millisecond switching. In…

We investigate the DFT+U approach as a viable solution to describe the low-lying states of ligated and unligated iron heme complexes. Besides their central role in organometallic chemistry, these compounds represent a paradigmatic case…

Soft Condensed Matter · Physics 2007-05-23 Damian A. Scherlis , Matteo Cococcioni , Patrick Sit , Nicola Marzari

Nitrogen-doped graphene was recently synthesized and was reported to be a catalyst for hydrogen dissociative adsorption under a perpendicular applied electric field (F). In this work, the diffusion of H atoms on N-doped graphene, in the…

Materials Science · Physics 2012-02-15 Z. M. Ao , A. D. Hernández-Nieves , F. M. Peeters , S. Li

The double electron attachment (DEA) and double ionization potential (DIP) equation-of-motion coupled-cluster (EOMCC) methods including up to 4-particle-2-hole (4$p$-2$h$) and 4-hole-2-particle (4$h$-2$p$) excitations on top of…

Chemical Physics · Physics 2026-05-21 Jun Shen , Karthik Gururangan , Piotr Piecuch

A new reactive force field to describe proton diffusion within the solid-oxide fuel cell material BaZrO3 has been derived. Using a quantum mechanical potential energy surface, the parameters of an interatomic potential model to describe…

Materials Science · Physics 2015-03-19 Paolo Raiteri , Julian D. Gale , Giovanni Bussi

We employ density functional theory (DFT) to investigate the adsorption and dehydrogenation of methane on the BNG-Ir13 cluster at both low and high oxygen coverage. The DFT calculations show that the low-oxygen-coverage BNG-Ir13 cluster…

Applied Physics · Physics 2024-05-21 Jemal Yimer Damte , Jiri Houska

Nitrate reduction to ammonia has attracted much attention for nitrate (NO3-) removal and ammonia (NH3) production. Identifying promising catalyst for active nitrate electroreduction reaction (NO3RR) is critical to realize efficient…

Materials Science · Physics 2023-08-29 Zheng Shu , Hongfei Chen , Xing Liu , Huaxian Jia , Hejin Yan , Yongqing Cai

Recent implosion experiments performed at the OMEGA laser facility reported by Casey et al.[1], displayed an anomalously low dd proton yield and a high tt neutron yield as compared to dt fusion reactions, explained as a stratification of…

Plasma Physics · Physics 2013-03-20 Hua Zheng , Aldo Bonasera

A serious concern in the safety and economy of a pressurized water nuclear reactor is related to the accumulation of boron inside the metal oxide (mostly NiFe${}_{2}$O${}_{4}$ spinel) deposits on the upper regions of the fuel rods. Boron,…

Materials Science · Physics 2014-09-08 Zs. Rak , E. W. Bucholz , D. W. Brenner

Ammonia, a versatile compound that can be used as a fertilizer, chemical or fuel, has since long been produced through the energy-intensive Haber-Bosch process. Recently, the electrochemical nitrate reduction reaction (NO3RR) using…

Density Functional Theory (DFT) is a powerful and accurate tool exploited in Nuclear Physics to investigate the ground-state and some collective properties of nuclei along the whole nuclear chart. Models based on DFT are, however, not…

Nuclear Theory · Physics 2017-10-26 X. Roca-Maza , Y. F. Niu , G. Colò , P. F. Bortignon

Phosphorylation is one of the most important protein modifications, and electron-transfer dissociation tandem mass spectrometry (ETD-MS/MS) is a potentially useful method for the sequencing of phosphopeptides, including determination of the…

Chemical Physics · Physics 2018-11-27 Daiki Asakawa , Akio Miyazato , Frederic Rosu , Valérie Gabelica

Two-dimensional (2D) materials, such as transition metal dichalcogenides (TMDCs) in the 2H or 1T crystal phases, are promising (electro)catalyst candidates due to their high surface to volume ratio and composition of low-cost, abundant…

Materials Science · Physics 2025-02-11 Mohammad Amin Akhound , Karsten Wedel Jacobsen , Kristian Sommer Thygesen

Although many programs have been published for fully numerical Hartree--Fock (HF) or density functional (DF) calculations on atoms, we are not aware of any that support hybrid DFs, which are popular within the quantum chemistry community…

Chemical Physics · Physics 2019-08-19 Susi Lehtola

The class of two-dimensional metal carbides and nitrides known as MXenes offer a distinct manner of property tailoring for a wide range of applications. The ability to tune the surface chemistry for expanding the property space of MXenes is…

Graphite is one of the most chemically inert materials. Its elementary constituent, monolayer graphene, is generally expected to inherit most of the parent material's properties including chemical inertness. Here we show that, unlike…

In this work, electrically and thermally conductive poly (butylene terephthalate) nanocomposites were prepared by in-situ ring-opening polymerization of cyclic butylene terephthalate (CBT) in presence of a tin-based catalyst. One type of…

Materials Science · Physics 2016-10-28 S. Colonna , O. Monticelli , J. Gomez , C. Novara , G. Saracco , A. Fina

We report on the investigation of dielectron production in tagged quasi-free neutron-proton collisions by using a deuteron beam of kinetic energy 1.25 GeV/u inpinging on a liquid hydrogen target. Our measurements with HADES confirm a…

Nuclear Experiment · Physics 2017-09-15 J. Adamczewski-Musch , O. Arnold , E. T. Atomssa , C. Behnke , A. Belounnas , A. Belyaev , J. C. Berger-Chen , J. Biernat , A. Blanco , C. Blume , M. Böhmer , P. Bordalo , S. Chernenko , L. Chlad , C. Deveaux , J. Dreyer , A. Dybczak , E. Epple , L. Fabbietti , O. Fateev , P. Filip , P. Finocchiaro , P. Fonte , C. Franco , J. Friese , I. Fröhlich , T. Galatyuk , J. A. Garzón , R. Gernhäuser , M. Golubeva , F. Guber , M. Gumberidze , S. Harabasz , T. Heinz , T. Hennino , S. Hlavac , C. Höhne , R. Holzmann , A. Ierusalimov , A. Ivashkin , B. Kämpfer , T. Karavicheva , B. Kardan , I. Koenig , W. Koenig , B. W. Kolb , G. Korcyl , G. Kornakov , R. Kotte , W. Kühn , A. Kugler , T. Kunz , A. Kurepin , A. Kurilkin , P. Kurilkin , V. Ladygin , R. Lalik , K. Lapidus , A. Lebedev , T. Liu , L. Lopes , M. Lorenz , T. Mahmoud , L. Maier , A. Mangiarotti , J. Markert , S. Maurus , V. Metag , J. Michel , E. Morinière , D. M. Mihaylov , S. Morozov , C. Müntz , R. Münzer , L. Naumann , K. N. Nowakowski , M. Palka , Y. Parpottas , V. Pechenov , O. Pechenova , O. Petukhov , J. Pietraszko , W. Przygoda , S. Ramos , B. Ramstein , A. Reshetin , P. Rodriguez-Ramos , P. Rosier , A. Rost , A. Sadovsky , P. Salabura , T. Scheib , H. Schuldes , E. Schwab , F. Scozzi , F. Seck , P. Sellheim , J. Siebenson , L. Silva , Yu. G. Sobolev , S. Spataro , H. Ströbele , J. Stroth , P. Strzempek , C. Sturm , O. Svoboda , P. Tlusty , M. Traxler , H. Tsertos , E. Usenko , V. Wagner , C. Wendisch , M. G. Wiebusch , J. Wirth , Y. Zanevsky , P. Zumbruch , A. V. Sarantsev