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Using an effective genetic algorithm, we uncover the structure of a metastable Al41Sm5 phase that supplements its family sharing similar short-range orders. The phase evolves upon heating an amorphous Al-9.7at.%Sm ribbon, produced by…

Materials Science · Physics 2017-12-29 Z. Ye , F. Meng , F. Zhang , Y. Sun , L. Yang , S. H. Zhou , R. E. Napolitano , M. I. Mendelev , R. T. Ott , M. J. Kramer , C. Z. Wang , K. M. Ho

The discovery of ultrastable glasses has raised novel challenges about glassy systems. Recent experiments studied the macroscopic devitrification of ultrastable glasses into liquids upon heating but lacked microscopic resolution. We use…

Statistical Mechanics · Physics 2023-04-13 Cecilia Herrero , Camille Scalliet , M. D. Ediger , Ludovic Berthier

Conventional crystalline alloys usually possess a low atomic size difference in order to stabilize its crystalline structure. However, in this article, we report a single phase chemically complex alloy which possesses a large atomic size…

A metastable {\epsilon}-Al60Sm11 phase appears during the initial devitrification of as-quenched Al-10.2 at.% Sm glasses. The {\epsilon} phase is nonstoichiometric in nature since Al occupation is observed on the 16f Sm lattice sites.…

Crucial to gaining control over crystallisation in multicomponent materials or accurately modelling rheological behaviour of magma flows is to understand the mechanisms by which crystal nuclei form. The microscopic nature of such nuclei,…

Soft Condensed Matter · Physics 2019-08-07 Trond S. Ingebrigtsen , Jeppe C. Dyre , Thomas B. Schrøder , C. Patrick Royall

During devitrification, pre-existing crystallites grow by adding particles to their surface via a process that is either thermally activated (diffusive mode) or happens without kinetic barriers (fast crystal growth mode). It is yet unclear…

Soft Condensed Matter · Physics 2023-08-30 Taiki Yanagishima , John Russo , Roel P A Dullens , Hajime Tanaka

Supercooled liquids are kinetically trapped materials in which the transition to a thermodynamically more stable state with long-range order is strongly suppressed. To assess the glass-forming abilities of a liquid empirical rules exist,…

Statistical Mechanics · Physics 2019-09-04 Francesco Turci , C. Patrick Royall , Thomas Speck

The search for effective methods to fabricate bulk single-phase quasicrystalline Al-Cu-Fe alloys is currently an important task. Crucial to solving this problem is to understand mechanisms of phase formation in this system. Here we study…

Chemical Physics · Physics 2020-01-08 L. V. Kamaeva , I. V. Sterkhova , V. I. Ladyanov , R. E. Ryltsev , N. M. Chtchelkatchev

Special role in computer simulations of supercooled liquid and glasses is played by few general models representing certain classes of real glass-forming systems. Recently, it was shown that one of the most widely used model glassformers --…

Materials Science · Physics 2018-11-14 R. E. Ryltsev , B. A. Klumov , N. M. Chtchelkatchev , K. Yu. Shunyaev

We consider both equilibrium and kinetic aspects of the phase separation (``thermal faceting") of thermodynamically unstable crystal surfaces into a hill--valley structure. The model we study is an Ising lattice gas for a simple cubic…

Condensed Matter · Physics 2009-10-22 Joel D. Shore , Dirk Jan Bukman

Below the melting temperature $T_m$ crystals are the stable phase of typical elemental or molecular systems. However, cooling down a liquid below $T_m$, crystallization is anything but inevitable. The liquid can be supercooled, eventually…

Disordered Systems and Neural Networks · Physics 2017-03-07 M. Zanatta , L. Cormier , L. Hennet , C. Petrillo , F. Sacchetti

The liquid crystalline 4-pentylphenyl-4'-decyloxythiobenzoate is investigated in various temperature programs for determination of crystallization kinetics and glassforming properties. The Avrami model, Augis-Bennett method and…

Extensive molecular dynamics simulations show that a short-range central potential, suited to model C60, undergoes a high temperature transition to a glassy phase characterized by the positional disorder of the constituent particles.…

Soft Condensed Matter · Physics 2007-05-23 Maria C. Abramo , Carlo Caccamo , Dino Costa , Romina Ruberto

By molecular-dynamics simulations, we have studied the devitrification (or crystallization) of aged hard-sphere glasses. First, we find that the dynamics of the particles are intermittent: Quiescent periods, when the particles simply…

Soft Condensed Matter · Physics 2014-04-03 Eduardo Sanz , Chantal Valeriani , Emanuela Zaccarelli , Wilson C K Poon , Michael E Cates , Peter N Pusey

Precipitation-strengthened alloys, such as Ni-base, Co-base and Fe-base superalloys, show the development of dendrite-like precipitates in the solid state during aging at near-$\gamma^{\prime}$ solvus temperatures. These features arise out…

Materials Science · Physics 2024-01-25 Tushar Jogi , Saurav Shenoy , R. Sankarasubramanian , Abhik Choudhury , Saswata Bhattacharyya

Unlike crystals, glasses age or devitrify over time, reflecting their non-equilibrium nature. This lack of stability is a serious issue in many industrial applications. Here, we show by numerical simulations that the devitrification of…

Soft Condensed Matter · Physics 2021-11-25 Taiki Yanagishima , John Russo , Roel P A Dullens , Hajime Tanaka

Metallic glasses have attracted considerable interest in recent years due to their unique combination of superb properties and processability. Predicting bulk metallic glass formers from known parameters remains a challenge and the search…

Using simulations and theory, we show that the cubatic phase is metastable for three model hard platelets. The locally favored structures of perpendicular particle stacks in the fluid prevent the formation of the columnar phase through…

Soft Condensed Matter · Physics 2015-03-13 Matthieu Marechal , Alessandro Patti , Matthew Dennison , Marjolein Dijkstra

We systematically study the relationship between equilibrium and non-equilibrium phase diagrams of a system of short-ranged attractive colloids. Using Monte Carlo and Brownian dynamics simulations we find a window of enhanced…

Soft Condensed Matter · Physics 2009-11-13 Andrea Fortini , Eduardo Sanz , Marjolein Dijkstra

We numerically investigate the competition between phase separation and dynamical arrest in a colloidal system interacting via a short ranged attractive potential. Equilibrium fluid configurations are quenched at two different temperatures…

Soft Condensed Matter · Physics 2007-05-23 G. Foffi , C. De Michele , F. Sciortino , P. Tartaglia
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