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High harmonic generation (HHG) is a highly nonlinear emission process in which systems driven by intense laser pulses emit integer multiples (harmonics) of the driving field. This feature is considered universal to all occurrences of HHG.…

Characterizing chirality is highly important for applications in the pharmaceutical industry, as well as in the study of dynamical chemical and biological systems. However, this task has remained challenging, especially due to the ongoing…

Chemical Physics · Physics 2022-01-28 Ofer Neufeld , Omri Wengrowicz , Or Peleg , Angel Rubio , Oren Cohen

High-harmonic generation from solids can be utilized as probe of ultrafast dynamics, but thus far only over extended sample areas, since its spatial resolution is diffraction-limited. Here we propose spatial polarization gating, that is…

Generation of odd harmonics by a super strong focused laser beam in vacuum is considered. The process occurs due to the plural light-by-light scattering effect. In the leading order of perturbation theory, generation of $(2k+1)$th harmonic…

High Energy Physics - Phenomenology · Physics 2008-11-26 A. M. Fedotov , N. B. Narozhny

The harmonic generation has always been of fundamental interest in studying the nonlinear nature of any physical system. In the present study, Particle - In - Cell (PIC) simulations have been carried out to explore the harmonic generation…

Plasma Physics · Physics 2023-07-12 Trishul Dhalia , Rohit Juneja , Laxman Prasad Goswami , Srimanta Maity , Amita Das

The production of a highly-polarized positron beam via nonlinear Breit-Wheeler processes during the interaction of an ultraintense circularly polarized laser pulse with a longitudinally spin-polarized ultrarelativistic electron beam is…

Plasma Physics · Physics 2020-07-29 Yan-Fei Li , Yue-Yue Chen , Wei-Min Wang , Hua-Si Hu

We generate high-order harmonics of a mid-infrared laser from a silicon single crystal and find their origin in the recollision of coherently accelerated electrons with their holes, analogously to the atomic and molecular case, and to ZnO…

High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…

We present analytically and numerically the spectrum of high harmonic emission generated by twisted electrons in the presence of linearly polarized light. Ensuing transitions from electronic continuum states with orbital angular momentum to…

Atomic Physics · Physics 2019-10-23 Sebastian Gemsheim , Jan-Michael Rost

We studied the high-harmonic generation by the interaction of sub-cycle laser pulses with the He atom. The sub-cycle pulses are modeled using the complex source vector beam model, which is an exact solution to Maxwell's equations and…

The first scheme for quasi-phase-matching high harmonic generation of circularly polarized radiation is proposed: optical rotation quasi-phase-matching (ORQPM). In ORQPM propagation of the driving radiation in a system exhibiting circular…

Optics · Physics 2013-03-19 Lewis Z. Liu , Kevin O'Keeffe , Simon M. Hooker

High-order harmonic generation via single-slit diffraction of relativistic laser pulses is investigated. Using fully kinetic 2D and 3D particle-in-cell simulations, we show that interesting optical phenomena emerge, including the generation…

Plasma Physics · Physics 2025-05-07 Longqing Yi

Alignment and orientation of molecules by intense, ultrashort laser fields are crucial for a variety of applications in physics and chemistry. These include control of high harmonics generation, molecular orbitals tomography, control of…

Thermotropic liquid crystals are versatile optical materials that exhibit a state of matter intermediate between liquids and solids. Their properties can change significantly with temperature, pressure, or other external factors, leading to…

Ultrafast extreme ultraviolet (XUV) sources with a controllable polarization state are powerful tools for investigating the structural and electronic as well as the magnetic properties of materials. However, such light sources are still…

Plasma Physics · Physics 2016-08-18 Zi-Yu Chen , Alexander Pukhov

High-order harmonic generation (HHG) is a powerful tool for probing electronic structure and ultrafast dynamics in matter. Traditionally studied in atomic and molecular gases, HHG has recently been extended to condensed matter, enabling…

Nonlinear metasurfaces have become prominent tools for controlling and engineering light at the nanoscale. Usually, the polarization of the total generated third harmonic is studied. However, diffraction orders may present different…

High-order harmonic generation (HHG) from atoms is a coherent light source that opens up attosecond physics, but it is the application of HHG to solids that brings much of excitement for the last decade. Here we report a completely new kind…

Materials Science · Physics 2019-08-28 G. P. Zhang , Y. H. Bai

High harmonic generation (HHG) is an established means of producing coherent, short wavelength, ultrafast pulses from a compact set-up. Table-top high-harmonic sources are increasingly being used to image physical and biological systems…

We generate high-order harmonics at high pulse repetition rates using a turnkey laser. High-order harmonics at 400 kHz are observed when argon is used as target gas. In neon we achieve generation of photons with energies exceeding 90 eV…

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