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Molecular magnets are attractive as spin qubits due to their chemical tunability, addressability through electron-spin resonance techniques, and long coherence times. Clock transitions (CTs), for which the system is immune to the effect of…
Nuclear spins with hyperfine coupling to single electron spins are highly valuable quantum bits. In this work we probe and characterise the particularly rich nuclear spin environment around single silicon vacancy color-centers (V2) in…
Quantum probes can measure time-varying fields with high sensitivity and spatial resolution, enabling the study of biological, material, and physical phenomena at the nanometer scale. In particular, nitrogen-vacancy centers in diamond have…
Spectroscopic labels for a few particles with spin that are harmonically trapped in one-dimension with effectively zero-range interactions are provided by quantum numbers that characterize the symmetries of the Hamiltonian: permutations of…
Nuclear quadrupolar resonance (NQR) spectroscopy reveals chemical bonding patterns in materials and molecules through the unique coupling between nuclear spins and local fields. However, traditional NQR techniques require macroscopic…
A multi-high-frequency electron paramagnetic resonance method is used to probe the magnetic excitations of a dimer of single-molecule magnets. The measured spectra display well resolved quantum transitions involving coherent superposition…
One approach to maintaining phase coherence of qubits through dynamical decoupling consists of applying a sequence of Hahn spin-echo pulses. Recent studies have shown that, in certain noise environments, judicious choice of the delay times…
Methods that preserve coherence broadly impact all quantum information processing and metrology applications. Dynamical decoupling methods accomplish this by protecting qubits in noisy environments but are typically constrained to the limit…
The interband polarizations induced by two phase-locked pulses in a semiconductor show strong interference effects depending on the time tau_1 separating the pulses. The four-wave mixing signal diffracted from a third pulse delayed by tau…
A quantum memory at microwave frequencies, able to store the state of multiple superconducting qubits for long times, is a key element for quantum information processing. Electronic and nuclear spins are natural candidates for the storage…
We show how nitrogen vacancy (NV) centers can be used to determine the amplitude, phase and frequency of unknown weak monochromatic and multichromatic oscillating magnetic fields using only the periodic dynamical decoupling (PDD) and…
Characterizing and understanding noise affecting quantum states has immense benefits in spectroscopy as well as in realizing quantum devices. Transverse relaxation times under a set of dynamical decoupling (DD) sequences with varying…
Quantum sensing takes advantage of well controlled quantum systems for performing measurements with high sensitivity and precision. We have implemented a concept for quantum sensing with arbitrary frequency resolution, independent of the…
We introduce a new method for analysing the aperiodic variability of coherent pulsations in accreting millisecond X-ray pulsars. Our method involves applying a complex frequency correction to the time-domain light curve, allowing for the…
We study the performance of composite pulses in the presence of time-varying control noise on a single qubit. These protocols, originally devised only to correct for static, systematic errors, are shown to be robust to time-dependent…
Spin fluctuations are an important issue for the design and operation of future spintronic devices. Femtosecond noise correlation spectroscopy (FemNoC) was recently applied to detect ultrafast magnetization fluctuations. FemNoC gives direct…
For a system of globally pulse-coupled phase-oscillators, we derive conditions for stability of the completely synchronous state and all possible two-cluster states and explain how the different states are naturally connected via…
We continuously observe dynamical decoupling in a spin-1 quantum gas using a weak optical measurement of spin precession. Continuous dynamical decoupling aims to dramatically modify the character and energy spectrum of spin states to render…
We report the observation of macroscopic harmonic states in an optically induced confinement in a highly photoexcited semiconductor microcavity at room temperature. The spatially photomodulated refractive index changes result in the…
We describe a method for improving coherent control through the use of detailed knowledge of the system's Hamiltonian. Precise unitary transformations were obtained by strongly modulating the system's dynamics to average out unwanted…