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The spin-$\frac{1}{2}$ kagome antiferromagnet is an archetypal frustrated system predicted to host a variety of exotic magnetic states. We show using neutron scattering measurements that deuterated vesignieite…

Strongly Correlated Electrons · Physics 2018-09-12 D. Boldrin , B. Fåk , E. Canévet , J. Ollivier , H. C. Walker , P. Manuel , D. Khalyavin , A. S. Wills

Recently, the superconductivity in a metal-organic framework (MOF) has been discovered for the first time in copper(II) benzenehexathiolate ([Cu$_3$(C$_6$S$_6$)]$_n$, Cu-BHT). The Cu atoms form a two-dimensional perfect Kagome lattice,…

Superconductivity · Physics 2020-09-21 T. Takenaka , K. Ishihara , Y. Miao , X. Huang , W. Xu , D. Zhu , N. Su , J. -G. Cheng , T. Shibauchi

We report results of magnetic susceptibility and 51V- and 63,65Cu-NMR measurements on a high-quality powder sample of vesignieite BaCu3V2O8(OH)2, a candidate for the spin-1/2 kagome antiferromagnet. We observed a twostep magnetic…

Strongly Correlated Electrons · Physics 2017-12-01 Makoto Yoshida , Yoshihiko Okamoto , Masashi Takigawa , Zenji Hiroi

The CsCr$_3$Sb$_5$ exhibits superconductivity in close proximity to a density-wave (DW) like ground state at ambient pressure\cite{Liu:2024aa}, however details of the DW is still elusive. Using first-principles density-functional…

Superconductivity · Physics 2025-04-08 Chenchao Xu , Siqi Wu , Guo-Xiang Zhi , Guanghan Cao , Jianhui Dai , Chao Cao , Xiaoqun Wang , Hai-Qing Lin

Double perovskite-based magnets wherein frustration and competition between emergent degrees of freedom are at play can lead to novel electronic and magnetic phenomena. Herein, we report the electronic structure and magnetic properties of…

Kagome metals with van Hove singularities near the Fermi level can host intriguing quantum phenomena such as chiral loop currents, electronic nematicity, and unconventional superconductivity. However, to our best knowledge, unconventional…

The magnetic susceptibility and magnetization of two new layered S=1/2 Heisenberg antiferromagnets with moderate exchange are reported. The two isostructural compounds, (2-amino-5-chloropyridinium)2CuBr4 ((5CAP)2CuBr4) and…

Materials Science · Physics 2009-11-07 F. M. Woodward , A. S. Albrecht , C. M. Wynn , C. P. Landee , M. M. Turnbull

In this work, we theoretically study the charge order and orbital magnetic properties of a new type of antiferromagnetic kagome metal FeGe. Based on first principles density functional theory (DFT) calculations, we have studied the…

Mesoscale and Nanoscale Physics · Physics 2023-03-07 Hai-Yang Ma , Jia-Xin Yin , M. Zahid Hasan , Jianpeng Liu

We have found weak long range antiferromagnetic order in the quasi-two-dimensional insulating oxide $ KCr_3(OD)_6(SO_4)_2$ which contains Cr$^{3+}$ S=3/2 ions on a kagom\'{e} lattice. In a sample with $\approx$ 76% occupancy of the chromium…

Strongly Correlated Electrons · Physics 2009-10-30 S. -H. Lee , C. Broholm , M. F. Collins , L. Heller , A. P. Ramirez , C. Kloc , E. Bucher , R. W. Erwin , N. Lacevic

The kagome lattice can host exotic magnetic phases arising from frustrated and competing magnetic interactions. However, relatively few insulating kagome materials exhibit incommensurate magnetic ordering. Here, we present a study of the…

Strongly Correlated Electrons · Physics 2023-04-19 Joseph A. M. Paddison , Li Yin , Keith M. Taddei , Malcolm J. Cochran , Stuart A. Calder , David S. Parker , Andrew F. May

An oxygen hyperstoichiometric ferrite CaBaFe4O7+\delta (\delta \approx 0.14) has been synthesized using "soft" reduction of CaBaFe4O8. Like the oxygen stoichiometric ferrimagnet CaBaFe4O7, this oxide also keeps the hexagonal symmetry (space…

Strongly Correlated Electrons · Physics 2011-03-16 Tapati Sarkar , V. Duffort , V. Pralong , V. Caignaert , B. Raveau

Here we present the discovery and characterization of the kagome metal TbTi$_3$Bi$_4$ in tandem with a new series of compounds, the Ln$_{2-x}$Ti$_{6+x}$Bi$_9$ (Ln: Tb-Lu) shurikagome metals. We previously reported on the growth of the…

The double-perovskite A$_2$BB'O$_6$ with heavy transition metal ions on the ordered B' sites is an important family of compounds to study the interplay between electron correlation and spin-orbit coupling (SOC). Here we prepared…

Strongly Correlated Electrons · Physics 2020-07-01 Shang Gao , Daigorou Hirai , Hajime Sagayama , Hiroyuki Ohsumi , Zenji Hiroi , Taka-hisa Arima

Ru based perovskites demonstrate an amazing richness in their magnetic properties, including 3D and quasi-2D ferromagnetism, antiferromagnetism, and unconventional superconductivity. Tendency to ferromagnetism, stemming from the unusually…

Superconductivity · Physics 2009-10-31 I. I. Mazin , D. J. Singh

We used single-crystal x-ray and neutron diffraction to investigate the crystal and magnetic structures of trigonal lattice iridate Ca2Sr2IrO6. The crystal structure is determined to be $R\bar3$ with two distinct Ir sites. The system…

Strongly Correlated Electrons · Physics 2018-06-14 Jieming Sheng , Feng Ye , Christina Hoffmann , Valentino R. Cooper , Satoshi Okamoto , Jasminka Terzic , Hao Zheng , Hengdi Zhao , G. Cao

We analyze the experimental data for the magnetic susceptibility of the material ZnCu3(OH)6Cl2 in terms of the Kagome Lattice Heisenberg model (KLHM), discussing possible role of impurity spins, dilution, exchange anisotropy, and both…

Strongly Correlated Electrons · Physics 2007-05-23 Marcos Rigol , Rajiv R. P. Singh

A new spin-1/2 quasi-one-dimensional antiferromagnet KCuMoO_4(OH) is prepared by the hydrothermal method. The crystal structures of KCuMoO_4(OH) and the already-known Na-analogue, NaCuMoO_4(OH), are isotypic, comprising chains of Cu^{2+}…

Strongly Correlated Electrons · Physics 2015-05-21 Kazuhiro Nawa , Takeshi Yajima , Yoshihiko Okamoto , Zenji Hiroi

The newly identified field-induced up-up-down order in Ba$_3$CoSb$_2$O$_9$ etc. renewed attention on exotic phases in spin-1/2 triangular-lattice antiferromagnets. Here, we report a unique zero-field noncoplanar up,up,down, down,down,up…

Strongly Correlated Electrons · Physics 2024-11-05 X. G. Zheng , M. Hagihala , I. Yamauchi , E. Nishibori , T. Honda , T. Yuasa , C. -N. Xu

Several doped 6H hexagonal ruthenates, having the general formula Ba3MRu2O9, have been studied over a significant period of time in order to understand the unusual magnetism of ruthenium metal. However, among them, the M=Fe compound appears…

Herbertsmithite, ZnCu$_3$(OH)$_6$Cl$_2$, is a two dimensional kagom\'{e} lattice realization of a spin liquid, with evidence for fractionalized excitations and a gapped ground state. Such a quantum spin liquid has been proposed to underlie…

Strongly Correlated Electrons · Physics 2016-10-18 Z. A. Kelly , M. J. Gallagher , T. M. McQueen