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Related papers: Barlowite as a canted antiferromagnet: theory and …

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We study polycrystalline samples of KCu3As2O7(OH)3, a new candidate spin-1/2 kagome antiferromagnet, by magnetic susceptibility and heat capacity measurements above 2 K. The unique arrangement of the 3z2 - r2 and x2 - y2 orbitals on the…

Materials Science · Physics 2015-06-04 Yoshihiko Okamoto , Hajime Ishikawa , Gøran J. Nilsen , Zenji Hiroi

Novel magnetic phases are expected to occur in highly frustrated spin systems. Here we study the structurally perfect kagom\'e antiferromagnet CdCu$_3$(OH)$_6$(NO$_3$)$_2\cdot$H$_2$O by magnetization, magnetic torque, and heat capacity…

Strongly Correlated Electrons · Physics 2017-03-29 Ryutaro Okuma , Takeshi Yajima , Daisuke Nishio-Hamane , Tsuyoshi Okubo , Zenji Hiroi

We prepared a powder sample of edwardsite Cd2Cu3(SO4)2(OH)6 4H2O, which is a new candidate compound for the spin-1/2 kagome antiferromagnet, and studied its magnetic properties by magnetic susceptibility and heat capacity measurements.…

Materials Science · Physics 2015-06-15 Hajime Ishikawa , Yoshihiko Okamoto , Zenji Hiroi

We report the synthesis, crystal structure, and magnetic properties of Co$^{2+}$ kagome magnets Co$_3$V$_2$O$_7$(OH)$_2$$\cdot$2H$_2$O and BaCo$_3$(VO$_4$)$_2$(OH)$_2$, which can be recognized as Co-analogues of the intensively researched…

Strongly Correlated Electrons · Physics 2024-06-06 Yuya Haraguchi , Takehiro Ohnoda , Akira Matsuo , Koichi Kindo , Hiroko Aruga Katori

The spin-1/2 kagome antiferromagnets are key prototype materials for studying frustrated magnetism. Three isostructural kagome antiferromagnets LnCu$_3$(OH)$_6$Cl$_3$ (Ln = Gd, Tb, Dy) have been successfully synthesized by the hydrothermal…

Strongly Correlated Electrons · Physics 2021-08-27 Ying Fu , Lianglong Huang , Xuefeng Zhou , Jian Chen , Xinyuan Zhang , Pengyun Chen , Shanmin Wang , Cai Liu , Dapeng Yu , Hai-Feng Li , Le Wang , Jia-Wei Mei

Spin-frustrated systems are one avenue for inducing macroscopic quantum states in materials. However, experimental realization of this goal has been difficult because of the lack of simple materials and, if available, the separation of the…

Strongly Correlated Electrons · Physics 2010-04-07 S. Chu , T. M. McQueen , R. Chisnell , D. E. Freedman , P. Müller , Y. S. Lee , D. G. Nocera

Realizing a quantum spin liquid (QSL) ground state in a real material is a leading issue in condensed matter physics research. In this pursuit, it is crucial to fully characterize the structure and influence of defects, as these can…

Magnetization and specific heat measurements have been carried out on Cs$_2$Cu$_3$ZrF$_{12}$ and Cs$_2$Cu$_3$HfF$_{12}$ single crystals, in which Cu$^{2+}$ ions with spin-1/2 form a regular Kagom\'{e} lattice. The antiferromagnetic exchange…

Strongly Correlated Electrons · Physics 2015-06-25 Y. Yamabe , T. Ono , T. Suto , H. Tanaka

A polycrystalline sample of vesignieite BaCu3V2O8(OH)2 comprising a nearly ideal kagome lattice composed of Cu2+ ions carrying spin 1/2 has been synthesized and studied by magnetization and heat capacity measurements. Magnetic…

Strongly Correlated Electrons · Physics 2009-11-13 Yoshihiko Okamoto , Hiroyuki Yoshida , Zenji Hiroi

Spin-$1/2$ kagome antiferromagnets are leading candidates for realizing quantum spin liquid (QSL) ground states. While QSL ground states are predicted for the pure Heisenberg model, understanding the robustness of the QSL to additional…

Strongly Correlated Electrons · Physics 2026-02-16 Shengtao Jiang , Arthur C. Campello , Wei He , Jiajia Wen , Daniel M. Pajerowski , Young S. Lee , Hong-Chen Jiang

The discovery of ideal spin-1/2 kagome antiferromagnets Herbertsmithite and Zn-doped Barlowite represents a breakthrough in the quest for quantum spin liquids (QSLs), and nuclear magnetic resonance (NMR) spectroscopy plays a prominent role…

Strongly Correlated Electrons · Physics 2019-12-06 Shunhong Zhang , Yi Zhou , Feng Liu , Zheng Liu

We report $^{51}$V NMR, $\mu$SR and zero applied field $^{63,65}$Cu NMR measurements on powder samples of Sr-vesignieite, SrCu$_3$V$_2$O$_8$(OH)$_2$, a $S = 1/2$ nearly-kagome Heisenberg antiferromagnet. Our results demonstrate that the…

Strongly Correlated Electrons · Physics 2020-02-26 A. Verrier , F. Bert , J. -M. Parent , M. El-Amine , J. C. Orain , D. Boldrin , A. S. Wills , P. Mendels , J. A. Quilliam

One of the key questions concerning frustrated lattices that has lately emerged is the role of disorder in inducing spin-liquid-like properties. In this context, the quantum kagome antiferromagnets YCu$_3$(OH)$_6$Cl$_3$, which has been…

Strongly Correlated Electrons · Physics 2019-07-02 A. Zorko , M. Pregelj , M. Klanjšek , M. Gomilšek , Z. Jagličić , J. S. Lord , J. A. T. Verezhak , T. Shang , W. Sun , J. -X. Mi

ScFe$_6$Ge$_4$ with the LiFe$_6$Ge$_4$-type structure (space group $R{\bar{3}}m$), which has a double-layered kagome lattice (18$h$ site) of Fe crystallographically equivalent to that of a well-known topological ferromagnet Fe$_3$Sn$_2$, is…

Strongly Correlated Electrons · Physics 2023-12-29 M. A. Kassem , T. Shiotani , H. Ohta , Y. Tabata , T. Waki , H. Nakamura

The kagome Heisenberg antiferromagnet formed by frustrated spins arranged in a lattice of corner-sharing triangles is a prime candidate for hosting a quantum spin liquid (QSL) ground state consisting of entangled spin singlets. But the…

Strongly Correlated Electrons · Physics 2022-03-09 Jiaming Wang , Weishi Yuan , Philip M. Singer , Rebecca W. Smaha , Wei He , Jiajia Wen , Young S. Lee , Takashi Imai

We have successfully synthesized S = 1/2 kagome antiferromagnets MCu3(OH)6Cl2 (M = Ni and Co) by hydrothermal method with rotating pressure vessel. Structural characterization shows that both compounds have the similar crystal structure as…

Strongly Correlated Electrons · Physics 2012-12-10 Yue-sheng Li , Qing-ming Zhang

We show that YCr6Ge6, comprising a kagome lattice made up of Cr atoms, is a plausible candidate compound for a kagome metal that is expected to exhibit anomalous phenomena such as flat-band ferromagnetism. Resistivity, magnetization, and…

Materials Science · Physics 2015-06-12 Yui Ishii , Hisatomo Harima , Yoshihiko Okamoto , Jun-ichi Yamaura , Zenji Hiroi

The study of quantum spin-liquid states (QSL) with lattice dimension $>1$ has proven an enduring problem in solid state physics. Key candidate materials are the $S=\frac{1}{2}$ kagome magnets due to their ability to host quantum…

Materials Science · Physics 2016-10-04 E Connolly , P Reeves , D Boldrin , A S Wills

Experimental studies of high-purity kagome-lattice antiferromagnets (KAFM) are of great importance in attempting to better understand the predicted enigmatic quantum spin-liquid ground state of the KAFM model. However, realizations of this…

Strongly Correlated Electrons · Physics 2021-06-02 W. Sun , T. Arh , M. Gomilšek , P. Koželj , S. Vrtnik , M. Herak , J. -X. Mi , A. Zorko

Flat-band (FB) systems originating from special lattice geometry like in kagome metals as well as localized orbitals in the materials such as heavy-fermion (HF) compounds have induced intensive interest due to their band topology and strong…

Strongly Correlated Electrons · Physics 2026-01-12 Wenxin Lv , Pengcheng Ma , Tianqi Wang , Shangjie Tian , Ying Ma , Shouguo Wang , Xiao Zhang , Zhonghao Liu , Hechang Lei