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We report on time-resolved ultrafast terahertz third-harmonic generation spectroscopy of nonequilibrium dynamics of Weyl fermions in a nanometer thin film of the Weyl semimetal TaP. Terahertz third-harmonic generation is observed at room…

Strongly Correlated Electrons · Physics 2025-11-26 Patrick Pilch , Changqing Zhu , Sergey Kovalev , Renato M. A. Dantas , Amilcar Bedoya-Pinto , Stuart S. P. Parkin , Zhe Wang

A new scheme for enantiomer differentiation of chiral molecules using a pair of linearly polarized intense ultrashort laser pulses with skewed mutual polarization is presented. The technique relies on the fact that the off-diagonal…

Chemical Physics · Physics 2017-05-04 Andrey Yachmenev , Sergei N. Yurchenko

Ultrafast laser pulses provide unique tools to manipulate magnetization dynamics at femtosecond timescales, where the interaction of the electric field -- such as excitation of spin carriers to non-equilibrium states, generation of…

Sculpting sub-cycle temporal structures of optical waveforms allows one to image and even control electronic clouds in atoms, molecules and solids. Here we show how the transverse spin component arising upon spatial confinement of such…

Optics · Physics 2020-11-17 David Ayuso , Andres Ordonez , Misha Ivanov , Olga Smirnova

A promising route for the development of opto-elelctronic technology is to use terahertz radiation to modulate the optical properties of semiconductors. Here we demonstrate the dynamical control of photoluminescence (PL) emission in…

We consider the formation of RbCs by an elliptically polarized laser pulse. By varying the ellipticity of the laser for sufficiently large laser intensity, we see that the formation probability presents a strong dependence, especially…

Atomic Physics · Physics 2019-02-06 J. Pablo Salas , Cristel Chandre , J Salas

Elliptically polarized laser pulses (EPLPs) are widely applied in many fields of ultrafast sciences, but the ellipticity~($\varepsilon$) has never been in situ measured in the interaction zone of the laser focus. In this work, we propose…

We study interaction of generic asymmetric molecules with a pair of strong time-delayed short laser pulses with crossed linear polarizations. We show that such an excitation not only provides unidirectional rotation of the most polarizable…

Chemical Physics · Physics 2018-02-28 E. Gershnabel , I. Sh. Averbukh

We present the generation of THz radiation by focusing ultrafast laser pulses with three incommensurate wavelengths to form a plasma. The three colors include 800 nm and the variable IR signal and idler outputs from an optical parametric…

Plasma Physics · Physics 2018-08-01 Jacob D. Bagley , Clayton D. Moss , Jeremy A. Johnson

We explore a pure optical method for enantioselective orientation of chiral molecules by means of laser fields with twisted polarization. Several field implementations are considered, including a pair of delayed cross-polarized laser…

Chemical Physics · Physics 2018-03-23 I. Tutunnikov , E. Gershnabel , S. Gold , I. Sh. Averbukh

The nonlinear interaction between Near-Infrared (NIR) and Terahertz pulses is principally investigated as a means for the detection of radiation in the hardly accessible THz spectral region. Most studies have targeted second-order nonlinear…

In this study the generation of energetic coherent extreme ultraviolet (XUV) radiation with controlled polarization, is reported. The XUV radiation results from the process of high harmonic generation (HHG), in a gas phase atomic medium,…

Atomic Physics · Physics 2021-06-17 E. Vassakis , I. Orfanos , I. Liontos , D. Charalambidis , P. Tzallas , E. Skantzakis

Laser radiation incident on a ferromagnetic sample produces excited electrons and currents whose spin polarization must not be aligned with the magnetization -- an effect due to spin-orbit coupling that is ubiquitous in spin- and…

Materials Science · Physics 2023-11-03 Oliver Busch , Franziska Ziolkowski , Ingrid Mertig , Jürgen Henk

Generation of ultrarelativistic polarized positrons during interaction of an ultrarelativistic electron beam with a counterpropagating two-color petawatt laser pulse is investigated theoretically. Our Monte Carlo simulation based on a…

Polarisation analysis of synchrotron THz radiation was carried out with a standard stretched polyethylene polariser and revealed that the linearly polarised (horizontal) component contributes up to 22 +/- 5% to the circular polarised…

The brightness of a light source defines its applicability to nonlinear phenomena in science. Bright low frequency terahertz (< 5THz) radiation confined to a diffraction-limited spot size is a present hurdle due to the broad bandwidth and…

Optics · Physics 2014-07-08 Mostafa Shalaby , Christoph P. Hauri

Terahertz radiation by optical rectification has been observed at room temperature in a hydrogen-bonded organic molecular ferroelectric crystal, 2-phenyl malondialdehyde (PhMDA). The radiated electromagnetic wave consisted of a single-cycle…

Materials Science · Physics 2015-06-22 W. Guan , N. Kida , M. Sotome , Y. Kinoshita , R. Takeda , A. Inoue , S. Horiuchi , H. Okamoto

We show that isotropic component of circular polarization of stochastic gravitational wave background can be explored by breaking two dimensional configuration of multiple laser interferometers for correlation analysis. By appropriately…

Astrophysics · Physics 2008-11-26 Naoki Seto

We explore a plasma based analogue of a helical undulator capable of providing circularly and elliptically polarised betatron radiation. We focus on ionisation injection configurations and in the conditions where the laser pulse driver can…

Plasma Physics · Physics 2016-01-19 J. Vieira , J. Martins , U. Sinha

We demonstrate a new method to detect ferroelectric domains in inside and surface regions of organic ferroelectrics by mapping out two orthogonally polarized terahertz waves radiated from the crystal upon the irradiation of near-infrared…

Materials Science · Physics 2014-12-10 M. Sotome , N. Kida , S. Horiuchi , H. Okamoto