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The kinetic Monte Carlo method is used to model the dynamic properties of proton diffusion in anhydrous proton conductors. The results have been discussed with reference to a two-step process called the Grotthuss mechanism. There is a…

The kinetic Monte Carlo simulations are employed to study the proton conductivity for anhydrous heterocyclic based polymers. The proton transport is based on a two-step process called the Grotthuss mechanism. In the referring system the…

Materials Science · Physics 2015-06-23 T. Masłowski , A. Drzewiński , P. Ławniczak , J. Ulner

Imidazole and 1,2,3-triazole are promising hydrogen-bonded heterocycles that conduct protons via a structural mechanism and whose derivatives are present in systems ranging from biological proton channels to proton exchange membrane fuel…

Chemical Physics · Physics 2021-10-28 Austin O. Atsango , Mark E. Tuckerman , Thomas E. Markland

Imidazole is a promising anhydrous proton conductor with a high conductivity comparable to that of water at a similar temperature relative to its melting point. Previous theoretical studies of the mechanism of proton transport in imidazole…

The BaCe0.8Y0.2O3-{\delta} proton conductor under hydration and under compressive strain has been analyzed with high pressure Raman spectroscopy and high pressure x-ray diffraction. The pressure dependent variation of the Ag and B2g bending…

Benzoic acid (BA) is a model system for studying proton transfer (PT) reactions. The properties of solid BA subject to high pressure (exceeding 1 kbar = 0.1 GPa) are of particular interest due to the possibility of compression-tuning of the…

Chemical Physics · Physics 2022-01-26 Dominik Kurzydłowski

The influence of an intramolecular proton transfer reaction on the conductance of a molecular junction is investigated employing a generic model, which includes the effects of the electric field of the gate and leads electrodes and the…

Mesoscale and Nanoscale Physics · Physics 2017-03-08 Chriszandro Hofmeister , Pedro B. Coto , Michael Thoss

The hydrostatic pressure induced changes in the transport properties of monolayer (ML) MoS$_2$ have been investigated using first-principles density functional theory based calculations. The application of pressure induces shift in the…

Materials Science · Physics 2023-08-02 Saumen Chaudhuri , Amrita Bhattacharya , A. K. Das , G. P. Das , B. N. Dev

We report new results on the liquid to solid phase transition of benzene. We determine experimentally and investigate the properties of a number of parameters of the benzene metastable state under different pressures (from 0.1 up to 2200…

Chemical Physics · Physics 2019-08-06 Mustapha Azreg-Aïnou , Beycan İbrahimoǧlu

The study of the high pressure phase diagram of hydrogen has continued with renewed effort for about one century as it remains a fundamental challenge for experimental and theoretical techniques. Here we employ an efficient molecular…

Chemical Physics · Physics 2014-04-23 Guglielmo Mazzola , Seiji Yunoki , Sandro Sorella

Pressure-induced phase transitions of spin-crossover materials were simulated by a Monte Carlo simulation in the constant pressure ensemble for the first time. Here, as the origin of the cooperative interaction, we adopt elastic interaction…

Materials Science · Physics 2008-04-09 Yusuke Konishi , Hiroko Tokoro , Masamichi Nishino , Seiji Miyashita

In-situ electrochemical impedance spectroscopy was used to study the effect of lattice volume and strain on the proton conductivity of the yttrium-doped barium cerate proton conductor by applying the hydrostatic pressure up to 1.25 GPa. An…

Materials Science · Physics 2012-06-28 Qianli Chen , Artur Braun , Songhak Yoon , Nikolai Bagdassarov , Thomas Graule

A three-dimensional atomistic Kinetic Monte Carlo model was developed and used to study the interaction between mobile solutes and a migrating interface. While the model was developed with a simplified energetic and topological description,…

Materials Science · Physics 2015-06-16 Aulia Tegar Wicaksono , Chad W. Sinclair , Matthias Militzer

It is widely perceived that the correlation effect may play an important role in several unconventional superconducting families, such as cuprate, iron-based and heavy-fermion superconductors. The application of high pressure can tune the…

Superconductivity · Physics 2019-02-15 Enyu Wang , Jing Si , Xiyu Zhu , Guan-Yu Chen , Hai Lin , Hai-Hu Wen

Among various perovskite proton conducting oxides, Y-doped BaZrO3 perovskite is a promising material for electrochemical hydrogen devices due to the good chemical stability and higher proton conductivity at higher operating temperatures…

Materials Science · Physics 2022-01-27 M. Khalid Hossain , T. Yamamoto , K. Hashizume

We have reported the effect of pressure on the magnetization, and transport properties in the nominal composition Pr$_{2}$Ba$_{4}$Cu$_{7}$O$_{15-\delta}$ synthesized by a sol-gel technique. A reduction treatment of the as-sintered sample in…

Light-element compounds hold great promise of high critical temperature superconductivity judging from the theoretical perspective. Hydrogen-rich material, benzene, is such a kind of candidate but also an organic compound. A series of…

Superconductivity · Physics 2018-05-24 Guo-Hua Zhong , Chun-Lei Yang , Xiao-Jia Chen , Hai-Qing Lin

Solid CO2 phase I was studied using the pressure-constant NPT Monte Carlo simulation and the Kihara core potential in the temperature range below 194 K and the pressure range below 10 GPa. At a pressure of 1 bar, the temperature dependence…

Materials Science · Physics 2023-05-30 Koji Kobashi

We introduce an efficient scheme for the molecular dynamics of electronic systems by means of quantum Monte Carlo. The evaluation of the (Born-Oppenheimer) forces acting on the ionic positions is achieved by two main ingredients: i) the…

Strongly Correlated Electrons · Physics 2007-05-23 Sandro Sorella , Claudio Attaccalite

Yttrium substituted BaZrO3, with nominal composition BaZr0.9Y0.1O3, a ceramic proton conductor, was subject to impedance spectroscopy for temperatures 300 K < T < 715 K at mechanical pressures 1 GPa < p < 2 GPa. The activation energies Ea…

Strongly Correlated Electrons · Physics 2011-06-07 Qianli Chen , Artur Braun , Alejandro Ovalle , Cristian-Daniel Savaniu , Thomas Graule , Nikolai Bagdassarov
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