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We present an analytical and numerical study of the coherent exciton polarization including exciton-exciton correlation. The time evolution after excitation with ultrashort optical pulses can be divided into a slowly varying polarization…

Condensed Matter · Physics 2009-10-31 Th. Oestreich , L. J. Sham

Spatiotemporal dynamics of excitons in isolated semiconducting single-walled carbon nanotubes are studied using transient absorption microscopy. Differential reflection and transmission of an 810-nm probe pulse after excitation by a 750-nm…

Mesoscale and Nanoscale Physics · Physics 2013-01-08 Brian A. Ruzicka , Rui Wang , Jessica Lohrman , Shenqiang Ren , Hui Zhao

Understanding how dielectric anisotropy governs excitonic behavior in two-dimensional (2D) halide perovskites is critical for predicting and engineering their optoelectronic properties. In this work, we investigate Cs(n+1)PbnBr3n+1…

Charge-transfer excitons (CTX) at organic donor/acceptor interfaces are considered important intermediates for charge separation in photovoltaic devices. Crystalline model systems provide microscopic insights into the nature of such states…

Materials Science · Physics 2021-11-19 Darius Günder , Ana M. Valencia , Michele Guerrini , Tobias Breuer , Caterina Cocchi , Gregor Witte

Understanding the transport mechanism of electronic excitations in conjugated polymers is key to advancing organic optoelectronic applications, such as solar cells, OLEDs and flexible electronics. While crystalline polymers can be studied…

Materials Science · Physics 2021-12-13 Francesco Campaioli , Jared H. Cole

The PINTEX facility at the IUCF Cooler ring, dedicated to the study of spin dependence in nucleon-nucleon interactions, has been used to measure polarization observables of the reaction pp -> pp pi0 at beam energies between 325 and 400 MeV.…

Collective (elementary) excitations of quantum bosonic condensates, including condensates of exciton polaritons in semiconductor microcavities, are a sensitive probe of interparticle interactions. In anisotropic microcavities with…

The growing interest in harnessing singlet fission for photovoltaic applications stems from the possibility of generating two excitons from a single photon. Quantum efficiencies above unity have been reported, yet the correlation between…

We report on a strong dependence of the phonon-induced damping of Rabi dynamics in an optically driven exciton-biexciton quantum dot system on the polarization of the exciting pulse. While for a fixed pulse intensity the damping is maximal…

Mesoscale and Nanoscale Physics · Physics 2013-03-15 M. Glässl , V. M. Axt

Singlet fission (SF) is a very significant photophysical phenomenon and possesses potential applications. In this work, we try to give the rather detailed theoretical investigation of the SF process in the stacked polyacene dimer by…

Chemical Physics · Physics 2023-09-01 Jiawei Peng , Deping Hu , Hong Liu , Qiang Shi , Peng Bao , Zhenggang Lan

Transfer and decay dynamics of an exciton coupled to a polarization vibration in a dimer is investigated in a mixed quantum-classical picture with the exciton decay incorporated by a sink site. Using a separation of time scales, it is…

Condensed Matter · Physics 2009-10-28 Holger Schanz , Ivan Barvik , Bernd Esser

Using femtosecond pump-probe spectroscopy, we identify excitation induced dephasing as a major mechanism responsible for the breaking of the strong-coupling between excitons and photons in a semiconductor microcavity. The effects of…

Recent advances in singlet-fission research make it imperative that structure-property correlations that determine optical signatures of the triplet-triplet spin biexciton as well as its binding energy be understood precisely. We report…

Strongly Correlated Electrons · Physics 2020-03-06 Souratosh Khan , Sumit Mazumdar

Lead halide perovskite nanocrystals are promising materials for classical and quantum light emission. To understand these outstanding properties, a thorough analysis of the band-edge exciton emission is needed which is not reachable in…

Mesoscale and Nanoscale Physics · Physics 2023-04-07 Mohamed-Raouf Amara , Zakaria Said , Caixia Huo , Aurélie Pierret , Christophe Voisin , Weibo Gao , Qihua Xiong , Carole Diederichs

Exciton-exciton annihilation is a ubiquitous nonlinear dynamical phenomenon in materials hosting Frenkel excitons, that has been employed to probe exciton diffusion processes in conjugated polymeric materials. In this work, we investigate…

The ultrafast formation of strongly bound excitons in two-dimensional semiconductors provide a rich platform for studying fundamental physics as well as developing novel optoelectronic technologies. While extensive research has explored the…

Optical processes in insulators and semiconductors, including excitonic effects, can be described in principle exactly using time-dependent density-functional theory (TDDFT). Starting from a linearization of the TDDFT semiconductor Bloch…

Materials Science · Physics 2015-05-13 V. Turkowski , C. A. Ullrich

We present a theoretical analysis of a spin-dependent multicomponent condensate in two dimensions. The case of a condensate of resonantly photoexcited excitons having two different spin orientations is studied in detail. The energy and the…

Mesoscale and Nanoscale Physics · Physics 2009-10-30 J. Fernandez-Rossier , C. Tejedor

We consider a condensate of exciton-polaritons in a diluted magnetic semiconductor microcavity. Such system may exhibit magnetic self-trapping in the case of sufficiently strong coupling between polaritons and magnetic ions embedded in the…

Quantum Gases · Physics 2017-10-04 Paweł Miętki , Michał Matuszewski

Vector solitons present unique optical pulses characterised by coupled orthogonal polarisation components, offering rich, multidimensional dynamics. Their enhanced degrees of freedom make them highly versatile for exploring nonlinear wave…