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Surface plasmons in a centrosymmetric metal nanocrystal have been perceived as achiral, based on the quantum-mechanical theory of molecular optical activity. The one-electron theory is insufficient to describe optical activity in crystals,…

Mesoscale and Nanoscale Physics · Physics 2018-03-02 Jong-Won Park

Chirality refers to a geometric phenomenon in which objects are not superimposable on their mirror image. Structures made of nano-scale chiral elements can display chiroptical effects, such as dichroism for left- and right- handed…

Optics · Physics 2020-02-25 Behrooz Semnani , Jeremy Flannery , Rubayet Al Maruf , Michal Bajcsy

Large optical chirality in the vicinity of achiral high index dielectric nanostructures has been recently demonstrated as useful means of enhancing molecular circular dichroism. We theoretically study the spatial dependence of optical…

Optics · Physics 2022-05-25 Krzysztof M. Czajkowski , Tomasz J. Antosiewicz

Chirality is a concept that one object is not superimposable on its mirror image by translation and rotation. In particular, chiral plasmonics have been widely investigated due to their excellent optical chiral properties, and have led to…

Optics · Physics 2023-07-18 Yuqing Cheng , Mengtao Sun

While plasmonic particles can provide optical resonances in a wide spectral range from the lower visible up to the near-infrared, often symmetry effects are utilized to obtain particular optical responses. By breaking certain spatial…

Helicity preserving nanostructures and metasurfaces have been recently proposed as suitable candidates to enhance spectroscopic features of chiral matter. With this in mind, we highlight that losses in the constituent nonmagnetic materials…

Simple analytic expressions for the polarizability of metallic nanoparticles are in wide use in the field of plasmonics, but their origins are not obvious. In this article, expressions for the polarizability of a particle are derived in the…

Optics · Physics 2016-09-15 William L. Barnes

We present a new design of plasmonic nanoantenna with a slant gap for optical chirality engineering. At resonance, the slant gap provides highly enhanced electric field parallel to external magnetic field with a phase delay of 90 degree,…

Mesoscale and Nanoscale Physics · Physics 2014-03-26 Daniel Lin , Jer-Shing Huang

Chirality is an intriguing property of certain molecules, materials or artificial nanostructures, which allows them to interact with the spin angular momentum of the impinging light field. Due to their chiral geometry, they can distinguish…

Optics · Physics 2016-11-03 Peter Banzer , Pawel Wozniak , Uwe Mick , Israel De Leon , Robert W. Boyd

We systematically investigate the generation of optical chirality patterns by applying the superposition of two waves in three scenarios, namely plane waves in free space, evanescent waves of totally reflected light at dielectric interface…

Optics · Physics 2020-02-19 Jiwei Zhang , Shiang-Yu Huang , Zhan-Hong Lin , Jer-Shing Huang

Structured light enables the characterization of chirality of optically small nanoparticles by taking advantage of the helicity maximization concept recently introduced in[1]. By referring to fields with nonzero helicity density as chiral…

Applied Physics · Physics 2020-11-04 Mina Hanifeh , Mohammad Albooyeh , Filippo Capolino

The optical response of metallic nanoparticle arrays is dominated by localized surface plasmon excitations and is the sum of individual particle contributions modified by inter-particle coupling depending on specific array geometry. Here we…

Dark-field illumination is shown to make planar chiral nanoparticle arrangements exhibit circular dichroism in extinction analogous to true chiral scatterers. Circular dichrosim is experimentally observed at the maximum scattering of single…

A promising trend in plasmonics involves shrinking the size of plasmon-supporting structures down to a few nanometers, thus enabling control over light-matter interaction at extreme-subwavelength scales. In this limit, quantum mechanical…

Chirality in inorganic nanoparticles and nanostructures has gained increasing scientific interest, because of the possibility to tune their ability to interact differently with left- and right-handed circularly polarized light. In some…

When the sizes of photonic nanoparticles are much smaller than the excitation wavelength, their optical response can be efficiently described with a series of polarizability tensors. Here, we propose a universal method to extract the…

Mesoscale and Nanoscale Physics · Physics 2020-06-22 Adelin Patoux , Clément Majorel , Peter R. Wiecha , Aurélien Cuche , Otto L. Muskens , Christian Girard , Arnaud Arbouet

Chiral near fields possessing enhanced asymmetry (superchirality), created by the interaction of light with (chiral) nanostructures, potentially provide a route to novel sensing and metrology technologies for biophysical applications.…

Light interacts differently with left and right handed three dimensional chiral objects, like helices, and this leads to the phenomenon known as optical activity. Here, by applying a polarization tomography, we show experimentally, for the…

Optics · Physics 2015-05-18 A. Drezet , C. Genet , J. -Y. Laluet , T. W. Ebbesen

Chirality is a highly important topic in modern chemistry, given the dramatically different pharmacological effects that enantiomers can have on the body. Chirality of natural molecules can be controlled by reconfiguration of molecular…

Optics · Physics 2018-03-21 Xiaoyang Duan , Simon Kamin , Florian Sterl , Harald Giessen , Na Liu

Chirality is a fundamental asymmetry phenomenon, with chiral optical elements exhibiting asymmetric response in reflection or absorption of circularly polarized light. Recent realizations of such elements include nanoplasmonic systems with…