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Scale-up of flow-electrode capacitive deionization is hindered due to the reliance on thick brittle graphite current collectors. Inspired by developments of electrochemical technologies we present the use of flexible membrane electrode…

Electrochemical kinetics at electrode-electrolyte interfaces limit performance of devices including fuel cells and batteries. While the importance of moving beyond Butler-Volmer kinetics and incorporating the effect of electronic density of…

Chemical Physics · Physics 2021-01-06 Rachel Kurchin , Venkatasubramanian Viswanathan

Conventional phase-field models often drive solid-solid interfaces to coalesce when in close proximity. This feature limits their use for processes like diffusion bonding, where the interfaces might need to remain distinct under certain…

Materials Science · Physics 2026-02-20 Maryam Khodadad , Noel Walkington , Suresh Kalyanam , Matteo Pozzi , Kaushik Dayal

Inertial microfluidics has been limited to dilute particle concentrations due to defocusing (spreading out) at high particle concentrations. We observe a counterintuitive shift of focusing to the outer curved wall under high concentration…

Interfaces between demixed fluid phases of binary mixtures of hard platelets are investigated using density-functional theory. The corresponding excess free energy functional is calculated within a fundamental measure theory adapted to the…

Soft Condensed Matter · Physics 2011-09-14 M. Bier , L. Harnau , S. Dietrich

We present a new phase-field model of solidification which allows efficient computations in the regime when interface kinetic effects dominate over capillary effects. The asymptotic analysis required to relate the parameters in the…

Condensed Matter · Physics 2007-05-23 Kalin Vetsigian , Nigel Goldenfeld

In this paper, density functional theory calculations are used to explore the electronic and atomic reconstruction at interfaces between III-III/I-V oxides. In particular, at these interfaces, two dimensional electron gases (2DEGs) with…

Materials Science · Physics 2012-06-06 Valentino R. Cooper

We consider a system of two coupled parabolic PDEs introduced in [1] to model motility of eukaryotic cells. We study the asymptotic behavior of solutions in the limit of a small parameter related to the width of the interface in phase field…

Analysis of PDEs · Mathematics 2016-02-05 Leonid Berlyand , Mykhailo Potomkin , Volodymyr Rybalko

We deduce the mixing-demixing phase diagram for binary liquid mixtures in an electric field for various electrode geometries and arbitrary constitutive relation for the dielectric constant. By focusing on the behavior of the liquid-liquid…

Soft Condensed Matter · Physics 2013-07-18 Jennifer Galanis , Yoav Tsori

Motivated by ideas of fractionalization and intrinsic topological order in bosonic models with short-range interactions, we consider similar phenomena in formal lattice gauge theory models. Specifically, we show that a compact quantum…

Statistical Mechanics · Physics 2014-12-10 Scott D. Geraedts , Olexei I. Motrunich

Understanding over-limiting current (faster than diffusion) is a long-standing challenge in electrochemistry with applications in desalination and energy storage. Known mechanisms involve either chemical or hydrodynamic instabilities in…

Chemical Physics · Physics 2017-06-27 Ji-Hyung Han , Edwin Khoo , Peng Bai , Martin Z. Bazant

The rapid charging and/or discharging of electrochemical cells can lead to localized depletion of electrolyte concentration. This depletion can significantly impact the system's time dependent resistance. For systems with porous electrodes,…

Chemical Physics · Physics 2017-12-27 James W. Palko , Ali Hemmatifar , Juan G. Santiago

We present a sharp-interface model of two-dimensional ramified growth during quasi-steady electrodeposition. Our model differs from previous modeling methods in that it includes the important effects of extended space-charge regions and…

Fluid Dynamics · Physics 2015-10-14 Christoffer P. Nielsen , Henrik Bruus

A phase-field description of brittle fracture is employed in the reported four-point bending analyses of monolithic and laminated glass plates. Our aims are: (i) to compare different phase-field fracture formulations applied to thin glass…

Computational Engineering, Finance, and Science · Computer Science 2020-12-30 Jaroslav Schmidt , Alena Zemanová , Jan Zeman , Michal Šejnoha

Zinc-air batteries offer large specific energy densities, while relying on abundant and non-toxic materials. In this paper, we present the first multi-dimensional simulations of zinc-air batteries. We refine our existing theory-based model…

Chemical Physics · Physics 2019-06-25 Tobias Schmitt , Tobias Arlt , Ingo Manke , Arnulf Latz , Birger Horstmann

Solute trapping is an important phenomenon in rapid solidification of alloys, for which the continuous growth model (CGM) is a popular sharp interface theory. Using matched asymptotic analysis, we show how to quantitatively map the sharp…

Materials Science · Physics 2018-09-17 Tatu Pinomaa , Nikolas Provatas

Electropolymerization is a bottom-up materials engineering process of micro and nano-scale that utilizes electrical signals to deposit conducting dendrites' morphologies by a redox reaction in the liquid phase. It resembles synaptogenesis…

Disordered Systems and Neural Networks · Physics 2021-07-08 Ankush Kumar , Kamila Janzakova , Yannick Coffinier , Sébastien Pecqueur , Fabien Alibart

In this paper, phase field models are developed for multi-component vesicle membranes with different lipid compositions and membranes with free boundary. These models are used to simulate the deformation of membranes under the elastic…

Biological Physics · Physics 2007-05-23 Xiaoqiang Wang , Qiang Du

A model of multicellular systems with several types of cells is developed from the phase field model. The model is presented as a set of partial differential equations of the field variables, each of which expresses the shape of one cell.…

Biological Physics · Physics 2015-05-30 Makiko Nonomura

A new phase field model of microstructural evolution is presented that includes the effects of elastic strain energy. The model's thin interface behavior is investigated by mapping it onto a recent model developed by Echebarria et al (Phys…

Materials Science · Physics 2008-10-29 Michael Greenwood , Jeffrey J. Hoyt , Nikolas Provatas
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