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Raman spectroscopy is a powerful experimental technique for characterizing molecules and materials that is used in many laboratories. First-principles theoretical calculations of Raman spectra are important because they elucidate the…

Materials Science · Physics 2025-06-25 David A. Egger , Manuel Grumet , Tomáš Bučko

Imaging Raman spectroscopy can be used to identify cancerous tissue. Traditionally, a step-by-step scanning of the sample is applied to generate a Raman image, which, however, is too slow for routine examination of patients. By transferring…

Instrumentation and Methods for Astrophysics · Physics 2018-10-09 Elmar Schmälzlin , Benito Moralejo , Ingo Gersonde , Johannes Schleusener , Maxim E. Darvin , Gisela Thiede , Martin M. Roth

Raman scattering spectroscopy is widely used as an analytical technique in various fields, but its measurement process tends to be slow due to the low scattering cross-section. In the last decade, various broadband coherent Raman scattering…

Optics · Physics 2025-05-06 Takuma Nakamura , Kazuki Hashimoto , Takuro Ideguchi

Time-resolved spectral techniques play an important analysis tool in many contexts, from physical chemistry to biomedicine. Customarily, the label-free detection of analytes is manually performed by experts through the aid of classic…

Machine Learning · Computer Science 2020-11-17 Stefano Rini , Hirotsugu Hiramatsu

In this work, we propose a two-stage algorithm based on Bayesian modeling and computation aiming at quantifying analyte concentrations or quantities in complex mixtures with Raman spectroscopy. A hierarchical Bayesian model is built for…

Applications · Statistics 2018-05-22 Ningren Han , Rajeev J. Ram

Stimulated Raman scattering, employing a pump and a Stokes beam, exhibits itself through both the Raman loss observed in the pump beam and the Raman gain in the Stokes beam. This phenomenon finds application in spectroscopy for chemical…

Optics · Physics 2024-08-13 Minhaeng Cho

The success of non-linear optics relies largely on pulse-to-pulse consistency. In contrast, covariance based techniques used in photoionization electron spectroscopy and mass spectrometry have shown that wealth of information can be…

Micro-ring resonators (MRRs) "trap" incoming light, and therefore, have been shown to achieve extremely high local intensities of light. Thus, they can be used to facilitate highly non-linear optical signals. By embedding materials that…

Mesoscale and Nanoscale Physics · Physics 2024-09-04 A. Sharma , Y. Li , M. K. Prasad , W. L. Ho , S. T. Chu , I. V. Borzenets

Lattice structure and symmetry of two-dimensional (2D) layered materials are of key importance to their fundamental mechanical, thermal, electronic and optical properties. Raman spectroscopy, as a convenient and nondestructive tool, however…

Mesoscale and Nanoscale Physics · Physics 2015-08-28 Yanqing Feng , Wei Zhou , Yaojia Wang , Jian Zhou , Erfu Liu , Yajun Fu , Zhenhua Ni , Xinglong Wu , Hongtao Yuan , Feng Miao , Baigeng Wang , Xiangang Wan , Dingyu Xing

Stimulated Raman scattering (SRS) represents a powerful tool for accessing the vibrational properties of molecular compounds or solid state systems. From a spectroscopic perspective, SRS is able to capture Raman spectra free from incoherent…

Noise manifests ubiquitously in nonlinear spectroscopy, where multiple sources contribute to experimental signals generating interrelated unwanted components, from random point-wise fluctuations to structured baseline signals. Mitigating…

While the interaction of ultra-intense ultra-short laser pulses with near- and overcritical plasmas cannot be directly observed, experimentally accessible quantities (observables) often only indirectly give information about the underlying…

Plasma Physics · Physics 2022-12-13 Thomas Miethlinger , Nico Hoffmann , Thomas Kluge

This paper develops a spectral fitting technology based on the particle swarm optimization (PSO) algorithm, which is applied to a calibration-free wavelength modulation spectroscopy system to achieve concentration retrieval. As compared…

Instrumentation and Detectors · Physics 2022-12-13 Tingting Zhang , Yongjie Sun , Pengpeng Wang , Cunguang Zhu

We present multi-color imaging by stimulated Raman scattering (SRS) enabled by an ultrafast fiber-based light source with integrated amplitude modulation and frame-to-frame wavelength tuning. With a relative intensity noise level of -153.7…

We present an upconversion imaging experiment from the near-infrared to the visible spectrum. Using a dedicated broadband pump laser to increase the number of resolved elements converted in the image we obtain up to 56x64 spatial elements…

Surface Enhanced Raman Spectroscopy (SERS) is a well-established technique for enhancing Raman signals. Recently photonic integrated circuits have been used, as an alternative to microscopy based excitation and collection, to probe SERS…

Confocal Raman microscopy offers a particular pathway for monitoring chemical "fingerprints" of intracellular components like the cell membrane, organelles, and nucleus. Nevertheless, conventional Raman acquisitions of fixed or randomly…

Raman spectroscopy is an advantageous method for studying the local structure of materials, but the interpretation of measured spectra is complicated by the presence of oblique phonons in polycrystals of polar materials. Whilst group theory…

Waveguide-enhanced Raman spectroscopy (WERS) is a promising technique for sensitive and selective detection of chemicals in a compact chip-scale platform. Coupling light on and off the sensor chip with fibers however presents challenges…

Applied Physics · Physics 2020-05-05 Derek M. Kita , Jérôme Michon , Juejun Hu

As a highly sensitive vibrational imaging method, stimulated Raman scattering (SRS) microscopy is finding various applications, while its theoretical treatment seems still under development. Here we present a theoretical estimation of…

Optics · Physics 2024-03-11 Yasuyuki Ozeki