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We have calculated the pair correlation functions of a fluid interacting via the Gay-Berne(n-6) pair potentials using the \PY integral equation theory and have shown how these correlations depend on the value of n which measures the…

Soft Condensed Matter · Physics 2009-11-07 Ram C. Singh , Jokhan Ram , Yashwant Singh

We test the validity of some widely used phenomenological criteria for the localization of the fluid-solid transition thresholds against the phase diagrams of particles interacting through the exp-6, inverse-power-law, and Gaussian…

Soft Condensed Matter · Physics 2011-10-25 Franz Saija , Santi Prestipino , Paolo V. Giaquinta

We present thermodynamic relationships between the free energy of the phase-field crystal (PFC) model and thermodynamic state variables for bulk phases under hydrostatic pressure. This relationship is derived based on the thermodynamic…

Materials Science · Physics 2015-02-09 Victor W. L. Chan , Nirand Pisutha-Arnond , Katsuyo Thornton

We consider fluids where the attractive interaction at distances slightly larger than the particle size is dominated at larger distances by a repulsive contribution. A previous investigation of the effects of the competition between…

Soft Condensed Matter · Physics 2009-11-11 D. Pini , A. Parola , L. Reatto

The equilibrium density distribution and thermodynamic properties of a Lennard-Jones fluid confined to nano-sized spherical cavities at constant chemical potential was determined using Monte Carlo simulations. The results describe both a…

Mesoscale and Nanoscale Physics · Physics 2010-04-27 James F. Lutsko , Julien Laidet , Patrick Grosfils

We perform the analysis of predictions of a classical density functional theory for associating fluids with different association strength concerned with wetting of solid surfaces. The four associating sites water-like models with…

Soft Condensed Matter · Physics 2024-04-01 A. Kozina , M. Aguilar , O. Pizio , S. Sokołowski

The interplay between the structure and dynamics of partially confined Lennard Jones (LJ) fluids, deep into the supercritical phase, is studied over a wide range of densities in the context of the Frenkel line (FL), which separates rigid…

Statistical Mechanics · Physics 2019-03-20 Kanka Ghosh , C. V. Krishnamurthy

Kinetics of crystal-growth is investigated along the solid-liquid coexistence line for the (100), (110) and (111) orientations of the Lennard-Jones and Weeks-Chandler-Andersen fcc crystal-liquid interface, using non-equilibrium molecular…

Statistical Mechanics · Physics 2015-04-29 Ronald Benjamin , Jürgen Horbach

Direct correlation functions (DCFs), linked to the second functional derivative of the free energy with respect to the one-particle density, play a fundamental role in a statistical mechanics description of matter. This holds in particular…

Soft Condensed Matter · Physics 2021-08-25 S. -C. Lin , M. Oettel , J. M. Hring , R. Haussmann , M. Fuchs , G. Kahl

In this work we start from the assumption that normal solid to supersolid (NS-SS) phase transition is continuous, and develop a phenomenological Landau theory of the transition in which superfluidity is coupled to the elasticity of the…

Soft Condensed Matter · Physics 2013-05-29 Alan T. Dorsey , Paul M. Goldbart , John Toner

We consider a simple fluid confined between two parallel walls (substrates), separated by a distance L. The walls exert competing surface fields so that one wall is attractive and may be completely wet by liquid (it is solvophilic) while…

Soft Condensed Matter · Physics 2014-09-01 Maria C. Stewart , Robert Evans

We study the liquid-solid transition in a collection of interacting particles moving through a dissipative medium under the action of a constant, spatially uniform external force, e.g. a charge-stabilized suspension in a fluidized bed or a…

Soft Condensed Matter · Physics 2007-05-23 Rangan Lahiri , Sriram Ramaswamy

We computed a Lennard Jones frozen liquid with a free surface using classical molecular dynamics. The structure factor curves on the free surface of this sample was calculated for different depths knowing that we have periodic boundary…

Soft Condensed Matter · Physics 2015-05-13 N. Olivi-Tran , A. Faivre

Symmetry-breaking bifurcations, where a flow state with a certain symmetry undergoes a transition to state with a different symmetry, are ubiquitous in fluid mechanics. Much can be understood about the nature of these transitions from…

Fluid Dynamics · Physics 2024-11-20 John F. Rudge , Dan McKenzie

A thermodynamic framework that predicts the thermal conductivity $\lambda$ of simple fluids beyond the dilute-gas limit is introduced. By generalizing the transition-rate approach of particles on a lattice to conserved quantities in…

Statistical Mechanics · Physics 2025-12-03 Miguel Hoyuelos

A novel thermodynamic integration (TI) scheme is presented to compute the crystal-liquid interfacial free energy ($\gamma_{\rm cl}$) from molecular dynamics simulation. The scheme is applied to a Lennard-Jones system. By using extremely…

Soft Condensed Matter · Physics 2015-06-19 Ronald Benjamin , Jürgen Horbach

Using molecular dynamics simulations, we study a liquid model which consists of particles interacting via a spherically-symmetric two-scale Jagla ramp potential with both repulsive and attractive ramps. The Jagla potential displays…

Soft Condensed Matter · Physics 2009-11-11 Limei Xu , Sergey V. Buldyrev , C. Austen Angell , H. Eugene Stanley

A "supersolid" -- a crystal that exhibits an off-diagonal long-range order and a superflow -- has been a subject of much research since its first proposal [Andreev and Lifshitz 1969], but has not been realized as a ground state of…

Quantum Gases · Physics 2023-11-09 Leo Radzihovsky

We study the glass and jamming transition of finite-dimensional models of simple liquids: hard- spheres, harmonic spheres and more generally bounded pair potentials that modelize frictionless spheres in interaction. At finite temperature,…

Disordered Systems and Neural Networks · Physics 2013-07-16 Hugo Jacquin

In a recent class of phase field crystal (PFC) models, the density order parameter is coupled to powers of its mean field. This effectively introduces a phenomenology of higher-order direct correlation functions acting on long wavelengths,…

Materials Science · Physics 2024-08-21 Daniel L. Coelho , Duncan Burns , Emily Wilson , Nikolas Provatas