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Thermodynamics and dynamics of a classical two-dimensional system with dipole-like isotropic repulsive interactions are studied systematically using extensive molecular dynamics (MD) simulations supplemented by appropriate theoretical…

Soft Condensed Matter · Physics 2018-03-02 Sergey Khrapak , Nikita Kryuchkov , Stanislav Yurchenko

Thermodynamics and kinetics are thought to be linked in glass transitions. The quantitative predictions of -relaxation activation barriers provided by the theory of glasses based on random first order transitions are compared with…

Soft Condensed Matter · Physics 2007-05-23 Jacob D. Stevenson , Peter G. Wolynes

We present a calculation of a fourth-order, time-dependent density correlation function that measures higher-order spatiotemporall correlations of the density of a liquid. From molecular dynamics simulations of a glass-forming Lennard-Jones…

Statistical Mechanics · Physics 2009-11-07 N. Lacevic , F. W. Starr , T. B. Schroder , V. N. Novikov , S. C. Glotzer

We use the replica method to study the ideal glass transition of a liquid of identical Hard Spheres. We obtain estimates of the configurational entropy in the liquid phase, of the Kauzmann packing fraction, in the range 0.58--0.62, and of…

Soft Condensed Matter · Physics 2009-11-11 G. Parisi , F. Zamponi

We study whether fine discretization (i.e., terracing) of continuous pair interactions, when used in combination with first-order mean-spherical approximation theory, can lead to a simple and general analytical strategy for predicting the…

Soft Condensed Matter · Physics 2013-10-29 Kyle B. Hollingshead , Avni Jain , Thomas M. Truskett

We examine the phenomenon of dynamical heterogeneity in computer simulations of an equilibrium, glass-forming liquid. We describe several approaches to quantify the spatial correlation of single-particle motion, and show that spatial…

Soft Condensed Matter · Physics 2009-09-25 Sharon C. Glotzer , Claudio Donati

A thermodynamically self-consistent Ornstein-Zernike approximation (SCOZA) is applied to a fluid of spherical particles with a pair potential given by a hard-core repulsion and a Yukawa attractive tail $w(r)=-\exp [-z(r-1)]/r$. This…

Statistical Mechanics · Physics 2009-10-31 D. Pini , G. Stell , N. B. Wilding

We provide a consistent statistical-mechanical treatment for describing the thermodynamics and the structure of fluids embedded in the hyperbolic plane. In particular, we derive a generalization of the virial equation relating the bulk…

Statistical Mechanics · Physics 2009-05-18 François Sausset , Gilles Tarjus , Pascal Viot

We use molecular dynamics simulations in 2d to study multi-component fluid in the limiting case where {\it all the particles are different} (APD). The particles are assumed to interact via Lennard-Jones (LJ) potentials, with identical size…

Soft Condensed Matter · Physics 2015-06-23 Lenin S. Shagolsem , Dino Osmanović , Orit Peleg , Yitzhak Rabin

Correlation of interacting particles is studied in their dynamics and localization in ideal and disordered lattice systems with the help of numerical tools. Both 1D and 2D systems are considered. In 1D lattices with long-range hopping,…

Quantum Gases · Physics 2018-09-27 Tirthaprasad Chattaraj

In this article I study pairing of two interacting particles in ideal 1D, 2D and Bethe lattices. I employ the method of recursion that has been formulated recently by Berciu et. al. to compute the pair functions in real space without…

Computational Physics · Physics 2019-09-26 Tirthaprasad Chattaraj

We assess the validity of "microscopic" approaches of glass-forming liquids based on the sole k nowledge of the static pair density correlations. To do so we apply them to a benchmark provided by two liquid models that share very similar…

Statistical Mechanics · Physics 2011-10-10 Ludovic Berthier , Gilles Tarjus

A characteristic property of many soft matter systems is an ultrasoft effective interaction between their structural units. This softness often leads to complex behavior. In particular, ultrasoft systems under pressure demonstrate…

Soft Condensed Matter · Physics 2019-09-19 V. A. Levashov , R. E. Ryltsev , N. M. Chtchelkatchev

A first-principle multiscale modeling approach is presented, which is derived from the solution of the Ornstein-Zernike equation for the coarse-grained representation of polymer liquids. The approach is analytical, and for this reason is…

Soft Condensed Matter · Physics 2009-09-09 J. McCarty , I. Y. Lyubimov , M. G. Guenza

The liquid and crystal phase of a single-component Fermi gas with dipolar interactions are investigated using quantum Monte Carlo methods in two spatial dimensions and at zero temperature. The dipoles are oriented by an external field…

Quantum Gases · Physics 2013-05-30 N. Matveeva , S. Giorgini

The ion-induced long-range orientational order between water molecules recently observed in second harmonic scattering experiments and illustrated with large scale molecular dynamics simulations is quantitatively explained using the…

Chemical Physics · Physics 2018-03-29 Luc Belloni , Daniel Borgis , Maximilien Levesque

We develop a microscopic theory to analyze the phase behaviour and compute correlation functions of dense assemblies of soft repulsive particles both at finite temperature, as in colloidal materials, and at vanishing temperature, a…

Disordered Systems and Neural Networks · Physics 2011-11-09 Ludovic Berthier , Hugo Jacquin , Francesco Zamponi

A free energy functional for a crystal that contains both the symmetry conserved and symmetry broken parts of the direct pair correlation function has been used to investigate the crystallization of fluids in three-dimensions. The symmetry…

Soft Condensed Matter · Physics 2015-06-15 Atul S. Bharadwaj , Swarn L. Singh , Yashwant Singh

We consider fluids where the attractive interaction at distances slightly larger than the particle size is dominated at larger distances by a repulsive contribution. A previous investigation of the effects of the competition between…

Soft Condensed Matter · Physics 2009-11-11 D. Pini , A. Parola , L. Reatto

In this paper we propose and explore a method of analysis of the scattering experimental data for uniform liquid-like systems. In our pragmatic approach we are not trying to introduce by hands an artificial small parameter to work out a…

Soft Condensed Matter · Physics 2018-01-24 E. I. Kats , A. R. Muratov