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The phase behavior of a cross-linked polymer blend made of two incompatible species, $A$ and $B$, of different chemical nature is analyzed. Besides a homogeneous phase, this system also exhibits two microphases and a phase of total…

Condensed Matter · Physics 2007-05-23 Edilson Vargas , Marcia C. Barbosa

Polymer mixtures fractionate between phases depending on their molecular weight. Consequently, by varying solvent conditions, a polydisperse polymer sample can be separated between phases so as to achieve a particular molecular weight…

Soft Condensed Matter · Physics 2026-04-10 J. Pedro de Souza , William M. Jacobs , Howard A. Stone

Large-scale Monte Carlo simulations of a phase-separating colloid-polymer mixture are performed and compared to recent experiments. The approach is based on effective interaction potentials in which the central monomers of self-avoiding…

Soft Condensed Matter · Physics 2007-05-23 R. L. C. Vink , A. Jusufi , J. Dzubiella , C. N. Likos

The effect of quenched disorder in the one-dimensional asymmetric exclusion process is reviewed. Both particlewise and sitewise disorder generically induces phase separation in a range of densities. In the particlewise case the existence of…

Statistical Mechanics · Physics 2011-05-20 Joachim Krug

We investigate interfacial properties between two highly incompatible polymers of different stiffness. The extensive Monte Carlo simulations of the binary polymer melt yield detailed interfacial profiles and the interfacial tension via an…

Statistical Mechanics · Physics 2009-10-30 Marcus Mueller , Andreas Werner

The properties of the interface in a phase-separated solution of polymers with different degrees of polymerization and Kuhn segment lengths are calculated. The starting point is the planar interface, the profile of which is calculated in…

Soft Condensed Matter · Physics 2015-06-15 R. H. Tromp , E. M. Blokhuis

Mixtures of ideal polymers with hard spheres whose diameters are smaller than the radius of gyration of the polymer, exhibit extensive immiscibility. The interfacial tension between demixed phases of these mixtures is estimated, as is the…

Soft Condensed Matter · Physics 2009-11-07 Richard P. Sear

Dispersions of immiscible liquids, such as emulsions and polymer blends, are at the core of many industrial applications which makes the understanding of their properties (morphology, stability, etc.) of great interest. A wide range of…

Chemical Physics · Physics 2017-08-10 Anaïs Giustiniani , Wiebke Drenckhan , Christophe Poulard

Spatially uniform electric fields have been used to induce instabilities in liquids and polymers, and to orient and deform ordered phases of block-copolymers. Here we discuss the demixing phase transition occurring in liquid mixtures when…

Statistical Mechanics · Physics 2015-05-13 G. Marcus , Y. Tsori

We study morphologies of thin-film diblock copolymers between two flat and parallel walls. The study is restricted to the weak segregation regime below the order-disorder transition temperature. The deviation from perfect lamellar shape is…

Soft Condensed Matter · Physics 2009-11-07 Yoav Tsori , David Andelman

The possibility to induce demixing in a colloidal mixture by adding small polymers, or other equivalent depletant agents, is theoretically investigated. By use of Mean Field Theory, suitably generalized to deal with short range effective…

Soft Condensed Matter · Physics 2015-10-28 Alberto Parola , Luciano Reatto

Within self-consistent field theory we study the phase behavior of a symmetrical binary AB polymer blend confined into a thin film. The film surfaces interact with the monomers via short range potentials. One surface attracts the A…

Statistical Mechanics · Physics 2007-05-23 M. Mueller , K. Binder , E. V. Albano

Most of our current understanding of phase separation is based on ideas that disregard correlaions. Here we illuminate unexpected effects of correlations on the structure and thermodynamics of interfaces and in turn phase separation, which…

Statistical Mechanics · Physics 2024-03-15 Kristian Blom , Noah Ziethen , David Zwicker , Aljaž Godec

In this work we investigated the phase behavior of melts of block-copolymers with one charged block by means of dissipative particle dynamics with explicit electrostatic interactions. We assumed that all the Flory-Huggins \c{hi} parameters…

Soft Condensed Matter · Physics 2019-06-12 Alexey A. Gavrilov , Alexander V. Chertovich , Igor I. Potemkin

We study interfacial behavior of a lamellar (stripe) phase coexisting with a disordered phase. Systematic analytical expansions are obtained for the interfacial profile in the vicinity of a tricritical point. They are characterized by a…

Soft Condensed Matter · Physics 2009-10-31 Simon Villain-Guillot , David Andelman

The effect of adding nonadsorbing polymer to a lamellar phase of surfactant bilayers is studied theoretically. We find that the polymer produces coexistence between two lamellar phases of different layer spacings. The coexistence region is…

Soft Condensed Matter · Physics 2008-02-03 Richard P. Sear

The density profile and surface tension for the interface of phase-separated colloid-polymer mixtures have been studied in the framework of the square gradient approximation for both ideal and interacting polymers in good solvent. The…

Soft Condensed Matter · Physics 2009-11-10 A. Moncho-Jorda , B. Rotenberg , A. A. Louis

We present a theoretical model for predicting the phase behavior of polymer solutions in which phase separation competes with oligomerization. Specifically, we consider scenarios in which the assembly of polymer chains into stoichiometric…

Soft Condensed Matter · Physics 2024-07-31 Tianhao Li , W. Benjamin Rogers , William M. Jacobs

We study the phase diagram of the one-dimensional boson gas trapped inside an optical lattice with contact and dipolar interaction taking into account next-nearest terms for both tunneling and interaction. Using the density matrix…

Quantum Gases · Physics 2018-06-06 Krzysztof Biedroń , Mateusz Łącki , Jakub Zakrzewski

Letting free polymers diffuse from solution into a crosslinked polymer gel is often a crucial processing step in the synthesis of multiphase polymer-based gels, e.g., core-shell microgels. Here we use coarse-grained molecular dynamics…

Soft Condensed Matter · Physics 2024-12-17 Jude Ann Vishnu , Torsten Gereon Linder , Sebastian Seiffert , Friederike Schmid