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Electro-optic frequency combs were employed to rapidly interrogate an optomechanical sensor, demonstrating spectral resolution substantially exceeding that possible with a mode-locked frequency comb. Frequency combs were generated using an…

Optics · Physics 2022-04-01 D. A. Long , B. J. Reschovsky , F. Zhou , Y. Bao , T. W. LeBrun , J. J. Gorman

Frequency comb spectroscopy has significantly advanced molecular spectroscopy across scientific research and diverse applications. Among its key performance metrics especially for time-resolved studies, sensitivity and measurement speed are…

Dual-comb spectroscopy allows for the rapid, multiplexed acquisition of high-resolution spectra without the need for moving parts or low-resolution dispersive optics. This method of broadband spectroscopy is most often accomplished via…

Cavity-enhanced frequency comb spectroscopy for molecule detection in the mid-infrared powerfully combines high resolution, high sensitivity, and broad spectral coverage. However, this technique, and essentially all spectroscopic methods,…

We present a versatile mid-infrared frequency comb spectroscopy system based on a doubly resonant optical parametric oscillator tunable in the 3-5.4 {\mu}m range and two detection methods, a Fourier transform spectrometer (FTS) and a…

We present a new technique using a frequency comb laser and optical cavities for performing ultrafast transient absorption spectroscopy with improved sensitivity. Resonantly enhancing the probe pulses, we demonstrate a sensitivity of…

Optics · Physics 2016-04-05 Melanie A. R. Reber , Yuning Chen , Thomas K. Allison

Direct optical frequency Comb Spectroscopy (DCS) is proving to be a fundamental tool in many areas of science and technology thanks to its unique performance in terms of ultra-broadband, high-speed detection and frequency accuracy, allowing…

We have demonstrated a new technique that provides massively parallel comb spectroscopy sensitive specifically to ions through the combination of cavity-enhanced direct frequency comb spectroscopy with velocity modulation spectroscopy.…

Atomic Physics · Physics 2015-05-28 Laura C. Sinclair , Kevin C. Cossel , Tyler Coffey , Jun Ye , Eric A. Cornell

We report on an ultrastable molecular clock based on the interrogation of the 3{\nu} rotational-vibrational combination band at 1563nm of carbon monoxide 12C16O. The laser stabilization scheme is based on frequency modulation (FM)…

Atomic Physics · Physics 2016-05-25 Shailendar Saraf , Paul Berceau , Alberto Stochino , Robert Byer , John Lipa

Optical frequency-comb-based-high-resolution spectrometers offer enormous potential for spectroscopic applications. Although various implementations have been demonstrated, the lack of suitable mid-infrared comb sources has impeded…

We present broadband cavity-enhanced complex refractive index spectroscopy (CE-CRIS), a technique for calibration-free determination of the complex refractive index of entire molecular bands via direct measurement of transmission modes of a…

We report on the Doppler-free saturation spectroscopy of the nitrous oxide (N$_2$O) overtone transition at 1.28~$\mu$m. This measurement is performed by the noise-immune cavity-enhanced optical heterodyne molecular spectroscopy (NICE-OHMS)…

Atomic and Molecular Clusters · Physics 2017-08-02 Tzu-Ling Chen , Yi-Wei Liu

Optical cavities provide high sensitivity to dispersion since their resonance frequencies depend on the index of refraction. We present a direct, broadband, and accurate measurement of the modes of a high finesse cavity using an optical…

We perform femtosecond frequency comb vernier spectroscopy in the near infrared with a femtosecond Er doped fiber laser, a scanning high-finesse cavity and an InGaAs camera. By utilizing the properties of a frequency comb and a scanning…

The noise dynamics of an Optical Frequency Comb (OFC) based on a mode-locked Ti-Sapphire laser is analyzed in terms of noise modes. A spectrally resolved multipixel homodyne detection enables the simultaneous measurement of the amplitude…

Instrumentation and Detectors · Physics 2021-08-04 Matthieu Ansquer , Valérian Thiel , Syamsundar De , Bérengère Argence , Gregory Gredat , Fabien Bretenaker , Nicolas Treps

Two techniques that employ equally spaced trains of optical pulses to map an optical high frequency into a low frequency modulation of the signal that can be detected in real time are compared. The development of phase-stable optical…

Quantum Physics · Physics 2017-08-22 Kochise Bennett , Jeremy Rouxel , Shaul Mukamel

Absorption spectroscopy is a widely used technique that permits the detection and characterization of gas species at low concentrations. We propose a sensing strategy combining the advantages of frequency modulation spectroscopy with the…

Quantum Physics · Physics 2023-03-30 Alexandre Belsley

Massive multiple input and multiple output (MIMO) systems with orthogonal frequency division multiplexing (OFDM) are foundational for downlink multi-user (MU) communication in future wireless networks, for their ability to enhance spectral…

Signal Processing · Electrical Eng. & Systems 2025-07-30 Erdeng Zhang , Shuntian Zheng , Sheng Wu , Haoge Jia , Zhe Ji , Ailing Xiao

We have developed an extreme ultraviolet (XUV) frequency comb for performing ultra-high precision spectroscopy on the many XUV transitions found in highly charged ions (HCI). Femtosecond pulses from a 100 MHz phase-stabilized near-infrared…

Optical frequency combs have attracted attention as optical frequency rulers due to their tooth-like discrete spectra together with their inherent mode-locking nature and phase-locking control to a frequency standard. Based on this concept,…