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We present results of the coefficient of thermal expansion for the frustrated quasi-two-dimensional molecular conductor $\theta$-(BEDT-TTF)$_2$RbZn(SCN)$_4$ for temperatures 1.5 K $\leq T \leq$ 290 K. A pronounced first-order phase…

Strongly Correlated Electrons · Physics 2024-05-08 Yohei Saito , Owen Ganter , Chao Shang , Kenichiro Hashimoto , Takahiko Sasaki , Stephen M. Winter , Jens Müller , Michael Lang

We present a study of the influence of disorder on the Mott metal-insulator transition for the organic charge-transfer salt $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Cl. To this end, disorder was introduced into the system in a controlled way by…

Strongly Correlated Electrons · Physics 2018-01-17 Elena Gati , Ulrich Tutsch , Ammar Naji , Markus Garst , Sebastian Köhler , Harald Schubert , Takahiko Sasaki , Michael Lang

We present high-resolution measurements of the relative length change as a function of temperature of the organic charge-transfer salt $\kappa$-(BEDT-TTF)$_2$Hg(SCN)$_2$Cl. We identify anomalous features at $T_g \approx\,63$ K which can be…

Strongly Correlated Electrons · Physics 2018-02-14 Elena Gati , Stephen M. Winter , John A. Schlueter , Harald Schubert , Jens Müller , Michael Lang

The organic charge-transfer salt $\kappa$-(BEDT-TTF)$_{2}$Hg(SCN)$_{2}$Br is a quasi two-dimensional metal with a half-filled conduction band at ambient conditions. When cooled below $T=80$ K it undergoes a pronounced transition to an…

The two-dimensional organic conductor $\alpha$-(BEDT-TTF)$_2$I$_3$ undergoes a metal-insulator transition at $T_{\rm CO}=135$ K due to electronic charge ordering. We have conducted time-resolved investigations of its electronic properties…

Strongly Correlated Electrons · Physics 2016-06-15 Tobias Peterseim , Tomislav Ivek , Dieter Schweitzer , Martin Dressel

We have performed in-plane transport measurements on the two-dimensional organic salt $\kappa$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Cl. A variable (gas) pressure technique allows for a detailed study of the changes in conductivity through the…

Strongly Correlated Electrons · Physics 2009-11-10 P. Limelette , P. Wzietek , S. Florens , A. Georges , T. A. Costi , C. Pasquier , D. Jerome , C. Meziere , P. Batail

We investigate the dynamics of correlated charge carriers in the vicinity of the Mott metal-to-insulator transition in various of the title quasi-two-dimensional organic charge-transfer salts by means of fluctuation (noise) spectroscopy.…

Strongly Correlated Electrons · Physics 2015-03-19 Jens Brandenburg , Jens Müller , Dieter Schweitzer , John A. Schlueter

Interaction-driven metal-insulator transitions or Mott transitions are widely observed in condensed-matter systems. In multi-orbital systems, many-body physics is richer in which an orbital-selective metal-insulator transition is an…

Strongly Correlated Electrons · Physics 2018-11-09 Hanghui Chen

The organic conductor $\alpha$-(BEDT-TTF)$_2$I$_3$ provides the prime example of a charge-order-driven metal-insulator transition. Restricted chemical substitution of S atoms by Se in the constituent molecules allows us to modify the…

The electronic properties of molecular conductors can be readily varied via physical or chemical pressure as it increases the bandwidth W; this enables crossing the Mott insulator-to-metal phase transition by reducing electronic…

Strongly Correlated Electrons · Physics 2019-11-18 Y. Saito , R. Rösslhuber , A. Löhle , M. Sanz Alonso , M. Wenzel , A. Kawamoto , A. Pustogow , M. Dressel

We present the carrier transport properties in the vicinity of a doping-driven Mott transition observed at a field-effect transistor (FET) channel using a single crystal of the typical two-dimensional organic Mott insulator…

Strongly Correlated Electrons · Physics 2017-01-13 Yoshiaki Sato , Yoshitaka Kawasugi , Masayuki Suda , Hiroshi M. Yamamoto , Reizo Kato

This review first describes the evidence that strongly suggests the existence of the metal-insulator transition (MIT) in a two-dimensional electron system in Si regardless of the amount of disorder. Extensive studies of the charge dynamics…

Strongly Correlated Electrons · Physics 2011-09-22 Dragana Popović

We present measurements of the infrared response of the quasi-one-dimensional organic conductor (TMTSF)2$SO3 along (E||a) and perpendicular (E||b') to the stacking axis as a function of temperature. Above the metal-insulator transition…

Strongly Correlated Electrons · Physics 2007-06-13 A. Pashkin , K. Thirunavukkuarasu , Y. -L. Mathis , W. Kang , C. A. Kuntscher

We report on the dramatic slowing down of the charge carrier dynamics in a quasi-two-dimensional organic conductor, which can be reversibly tuned through the Mott metal-insulator transition (MIT). At the finite-temperature critical endpoint…

Strongly Correlated Electrons · Physics 2015-06-02 B. Hartmann , D. Zielke , J. Polzin , T. Sasaki , J. Müller

We explore the nature of the metal-insulator transition in $\beta^{\prime\prime}$-(BEDT-TTF)$_{2}$Hg(SCN)$_{2}$Cl by x-ray, electrical transport, ESR, Raman and infrared investigations. Magnetic and vibrational spectroscopy concurrently…

In this overview we provide a general introduction to metal-insulator transitions, with focus on specific mechanisms that can localize the electrons in absence of magnetic or charge ordering, and produce well defined quantum critical…

Strongly Correlated Electrons · Physics 2011-12-30 V. Dobrosavljevic

Mott metal-insulator transitions possess electronic, magnetic, and structural degrees of freedom promising next generation energy-efficient electronics. We report a previously unknown, hierarchically ordered state during a Mott transition…

In the field of interacting electron systems the Mott metal-to-insulator (MI) transition represents one of the pivotal issues. The role played by lattice degrees of freedom for the Mott MI transition and the Mott criticality in a variety of…

Strongly Correlated Electrons · Physics 2015-01-28 Mariano de Souza , Lorenz Bartosch

In the two-dimensional organic charge-transfer salts kappa-(BEDT-TTF)2Cu[N(CN)2]Br{x}Cl{1-x} a systematic variation of the Br content from x = 0 to 0.9 allows us to tune the Mott transition by increasing the bandwidth. At temperatures below…

Strongly Correlated Electrons · Physics 2009-06-18 Michael Dumm , Daniel Faltermeier , Natalia Drichko , Martin Dressel , Cecile Meziere , Patrick Batail

We present a combined study of thermal expansion and resistance fluctuation spectroscopy measurements exploring the static and dynamic aspects of the charge-glass formation in the quasi-two-dimensional organic conductors…

Strongly Correlated Electrons · Physics 2022-02-03 Tatjana Thomas , Yohei Saito , Yassine Agarmani , Tim Thyzel , Kenichiro Hashimoto , Takahiko Sasaki , Michael Lang , Jens Müller
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