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In this work we present a coupled-cluster theory for the propagation of multireference electronic systems initiating at general quantum mechanical states. Our formalism is based on the infinitesimal analysis of modified cluster operators,…

Chemical Physics · Physics 2025-05-09 Martín A. Mosquera

In this paper, we introduce patchwork constructions for multivariate quasi-copulas. These results appear to be new since the kind of approach has been limited to either copulas or only bivariate quasi-copulas so far. It seems that the…

Statistics Theory · Mathematics 2024-11-14 Damjana Kokol Bukovšek , Tomaž Košir , Blaž Mojškerc , Matjaž Omladič

With the aim of constructing an electronic structure approach that systematically goes beyond the GW and random phase approximation (RPA) we introduce a vertex correction based on the exact-exchange (EXX) potential of time-dependent density…

Materials Science · Physics 2018-07-16 Maria Hellgren , Nicola Colonna , Stefano de Gironcoli

A new scheme for producing semidiscrete self-trapped vortices (\textquotedblleft swirling photon droplets\textquotedblright ) in photonic crystals with competing quadratic ($\chi ^{(2)}$) and self-defocusing cubic ($\chi ^{(3)}$)…

Perturbative and non-perturbative expansion methods already constitute a tool of choice to perform ab initio calculations over a significant part of the nuclear chart. In this context, the categories of accessible nuclei directly reflect…

Nuclear Theory · Physics 2022-01-28 Mikael Frosini , Thomas Duguet , Jean-Paul Ebran , Vittorio Somà

Computer models or simulators are widely used across scientific fields, but are computationally expensive limiting their use to explore possible scenarios/outcomes. Gaussian process emulators are statistical surrogates that can rapidly…

Computation · Statistics 2025-08-27 Josh Seidman , Elaine T. Spiller

A diagrammatic multi-reference generalization of many-body perturbation theory was recently introduced [J. Phys. Chem. Lett., 2025, 16, 3047]. This framework allows us to extend single-reference (SR) Green's function methods defined at the…

Quantum Physics · Physics 2025-07-29 Yuqi Wang , Wei-Hai Fang , Zhendong Li

We test local and semi-local density functionals for the electronic exchange for a variety of systems including atoms, molecules, and atomic chains. In particular, we focus on a recent universal extension of the Becke-Johnson exchange…

Materials Science · Physics 2010-11-01 Micael J. T. Oliveira , Esa Räsänen , Stefano Pittalis , Miguel A. L. Marques

Nowadays pseudopotential density-functional theory calculations constitute the standard approach to tackle solid-state electronic problems. These rely on distributed pseudopotential tables that were built from all-electron atomic…

Computational Physics · Physics 2020-03-24 Pedro Borlido , Jan Doumont , Fabien Tran , Miguel Marques , Silvana Botti

Traditionally, interatomic potentials assume local bond formation supplemented by long-range electrostatic interactions when necessary. This ignores intermediate range multi-atom interactions that arise from the relaxation of the electronic…

Materials Science · Physics 2022-11-07 Anton Bochkarev , Yury Lysogorskiy , Christoph Ortner , Gábor Csányi , Ralf Drautz

Parametric amplification is an interesting way of artificially increasing a MEMS Quality factor and could be helpful in many kinds of applications. This paper presents a theoretical study of this principle, based on Matlab/Simulink…

Other Computer Science · Computer Science 2008-02-22 L. Grasser , H. Mathias , F. Parrain , X. Le Roux , J. -P. Gilles

In this paper, we address the problem of the post-prior equivalence in the calculation of inclusive breakup and transfer cross sections. For that, we employ the model proposed by Ichimura, Austern, and Vincent [Phys. Rev. C 32, 431 (1985)],…

Nuclear Theory · Physics 2018-02-07 Jin Lei , Antonio M. Moro

We propose a pseudopotential for the electron-electron Coulomb interaction to improve the efficiency of many-body electronic structure calculations. The pseudopotential accurately replicates the scattering properties of the Coulomb…

Strongly Correlated Electrons · Physics 2015-09-02 J. H. Lloyd-Williams , R. J. Needs , G. J. Conduit

Motivated by the disagreement between recent diffusion Monte Carlo calculations and experiments on the phase transition pressure between the ambient and beta-Sn phases of silicon, we present a study of the HCP to BCC phase transition in…

Chemical Physics · Physics 2015-01-19 Luke Shulenburger , Thomas R. Mattsson , M. P. Desjarlais

We present an approach for including relativistic corrections in lepton-nucleus scattering calculations within the Short-Time Approximation (STA). Previous ab-initio studies employed electromagnetic currents expanded in powers of $q/m$,…

We extend the recently developed converse NMR approach [T. Thonhauser, D. Ceresoli, A. Mostofi, N. Marzari, R. Resta, and D. Vanderbilt, J. Chem. Phys. \textbf{131}, 101101 (2009)] such that it can be used in conjunction with…

Materials Science · Physics 2010-05-21 D. Ceresoli , N. Marzari , G. Lopez , T. Thonhauser

We present an implementation and benchmark of new approximations in multireference algebraic diagrammatic construction theory for simulations of neutral electronic excitations and UV/Vis spectra of strongly correlated molecular systems…

Chemical Physics · Physics 2021-12-02 Ilia M. Mazin , Alexander Yu. Sokolov

We present a numerically feasible semiclassical (SC) method to evaluate quantum fidelity decay (Loschmidt echo, FD) in a classically chaotic system. It was thought that such evaluation would be intractable, but instead we show that a…

Quantum Physics · Physics 2009-11-10 Jiri Vanicek , Eric J. Heller

We present a version of the T-moves approach for treating nonlocal pseudopotentials in diffusion Monte Carlo which has much smaller time-step errors than the existing T-moves approaches, while at the same time preserving desirable features…

Chemical Physics · Physics 2021-07-29 Tyler A. Anderson , C. J. Umrigar

Conventional wisdom presumes that low-coordinated crystal ground states require directional interactions. Using our recently introduced optimization procedure to achieve self-assembly of targeted structures (Phys. Rev. Lett. 95, 228301…

Soft Condensed Matter · Physics 2009-11-11 Mikael C. Rechtsman , Frank H. Stillinger , Salvatore Torquato
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