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Related papers: New structural anomaly induced by nanoconfinement

200 papers

Spatial confinement in nanoporous media affects the structure, thermodynamics and mobility of molecular soft matter often markedly. This article reviews thermodynamic equilibrium phenomena, such as physisorption, capillary condensation,…

Soft Condensed Matter · Physics 2015-02-17 Patrick Huber

We study the phase behavior of a classical system of particles interacting through a strictly convex soft-repulsive potential which, at variance with the pairwise softened repulsions considered so far in the literature, lacks a region of…

Soft Condensed Matter · Physics 2009-09-17 Franz Saija , Santi Prestipino , Gianpietro Malescio

Using molecular dynamic simulations we study three families of continuous core-softened potentials consisting of two length scales: a shoulder scale and an attractive scale. All the families have the same slope between the two length scales…

Statistical Mechanics · Physics 2015-05-28 Ney M. Barraz , Evy Salcedo , Marcia C. Barbosa

We have studied structure formation in a confined block copolymer melt by means of dynamic density functional theory (DDFT). The confinement is two-dimensional, and the confined geometry is that of a cylindrical nanopore. Although the…

Soft Condensed Matter · Physics 2009-11-13 G. J. A. Sevink , A. V. Zvelindovsky

Molecular dynamics simulations are used to examine the relationship between water-like anomalies and the liquid-liquid critical point in a family of model fluids with multi-Gaussian, core-softened pair interactions. The core-softened pair…

Soft Condensed Matter · Physics 2015-05-27 Evy Salcedo , Alan B. de Oliveira , Ney M. Barraz , Charusita Chakravarty , Marcia C. Barbosa

Low temperature structural and superfluid properties of $^4$He confined in cylindrical nanopores are theoretically investigated by means of first principle Quantum Monte Carlo (QMC) simulations. We vary the density of $^4$He inside the…

Mesoscale and Nanoscale Physics · Physics 2022-02-03 Andrea Nava , Domenico Giuliano , Phong H. Nguyen , Massimo Boninsegni

Molecular Dynamics simulations of water molecules in nanometre sized cylindrical channels connecting two reservoirs show that the permeation of water is very sensitive to the channel radius and to electric polarization of the embedding…

Soft Condensed Matter · Physics 2009-11-07 Rosalind Allen , Simone Melchionna , Jean-Pierre Hansen

In this paper the amorphous/solid to disorder liquid structural phase transitions of an anomalous confined fluid is analyzed using their local fractal dimension. The model is a system of particles interacting through a two length scales…

Soft Condensed Matter · Physics 2016-02-17 Elsa M. de la Calleja-Mora , Leandro B. Krott , Marcia C. Barbosa

Predicting the spatial configuration of gas molecules in nanopores of shale formations is crucial for fluid flow forecasting and hydrocarbon reserves estimation. The key challenge in these tight formations is that the majority of the pore…

We investigate using molecular dynamics the effect of the structure of nanoconfinement for liquids with water-like anomalies and liquid-liquid phase transition (LLPT). We find that if the confinement is in an ordered matrix of nanoparticles…

Statistical Mechanics · Physics 2015-03-13 Elena G. Strekalova , Jiayuan Luo , H. Eugene Stanley , Giancarlo Franzese , Sergey V. Buldyrev

It is well stablished that confinement of supercooled liquids in nano-pores induces various effects as a strong modification of the dynamics and a layering of the local structure. In this work we raise the issue as how these confinement…

Mesoscale and Nanoscale Physics · Physics 2021-09-07 Felix Mercier , Gaetan Delhaye , Victor Teboul

We investigate the thermodynamic, structural, and dynamic behavior of a three-dimensional coarse-grained ramp-shoulder fluid derived from effective interactions between polymer-grafted nanoparticles. The interaction combines a softened…

Soft Condensed Matter · Physics 2026-05-25 Murilo S. Marques , Lucas Axel R. Santana , Gabriel San R. R. Câmara , José Rafael Bordin

We investigated the equilibrium properties of a one-dimensional system of classical particles which interact in pairs through a bounded repulsive potential with a Gaussian shape. Notwithstanding the absence of a proper fluid-solid phase…

Soft Condensed Matter · Physics 2012-01-11 Cristina Speranza , Santi Prestipino , Paolo V. Giaquinta

We investigate the structural, thermodynamic and dynamic behavior of of a two dimensional core-corona system using Langevin Dynamics simulations. The particles are modeled using a core-softened potential that exhibits waterlike anomalies…

Soft Condensed Matter · Physics 2018-02-14 José Rafael Bordin , Marcia C. Barbosa

Reactions at solid-water interfaces play a foundational role in water treatment systems, catalysis, chemical separations, and in predicting chemical fate and transport in the environment. Over the last century, experimental measurements and…

Chemical Physics · Physics 2022-12-14 Anastasia G. Ilgen , Kevin Leung , Louise J. Criscenti , Jeffery A. Greathouse

The mechanism of the collapse of the superhydrophobic state is elucidated for submerged nanoscale textures forming a three-dimensional interconnected vapor domain. This key issue for the design of nanotextures poses significant simulation…

Soft Condensed Matter · Physics 2017-03-31 Matteo Amabili , Alberto Giacomello , Simone Meloni , Carlo Massimo Casciola

We study the effect of volumetric constraints on the structure and electronic transport properties of distilled water in a nanopore with embedded electrodes. Combining classical molecular dynamics simulations with quantum scattering theory,…

Soft Condensed Matter · Physics 2014-01-30 P. Boynton , M. Di Ventra

Soft-core attractive potentials can give rise to a phase diagram with three fluid phases at different densities (gas, low-density liquid and high-density liquid), separated by first order phase transition lines ending in critical points.…

Statistical Mechanics · Physics 2009-10-22 Giancarlo Franzese

We use molecular dynamics simulations in two dimensions to investigate the possibility that a core-softened potential can reproduce static and dynamic anomalies found experimentally in liquid water: (i) the increase in specific volume upon…

Soft Condensed Matter · Physics 2009-10-31 A. Scala , M. Reza Sadr-Lahijany , N. Giovambattista , S. V. Buldyrev , H. E. Stanley

Using molecular dynamic simulations we study a family of continuous core-softened potentials consisting of a hard core, a shoulder at closest distances and an attractive well at further distance. The repulsive shoulder and the well…

Statistical Mechanics · Physics 2015-05-13 Ney M. Barraz , Evy Salcedo , Marcia C. Barbosa