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We have studied structure formation in a confined block copolymer melt by means of dynamic density functional theory (DDFT). The confinement is two-dimensional, and the confined geometry is that of a cylindrical nanopore. Although the…

Soft Condensed Matter · Physics 2009-11-13 G. J. A. Sevink , A. V. Zvelindovsky

The packing geometry of macromolecules in complex mesophases is of key importance to self-organization in synthetic and biological soft materials. While approximate or heuristic models rely on often-untested assumptions about how flexible…

Soft Condensed Matter · Physics 2023-10-05 Benjamin R. Greenvall , Michael S. Dimitriyev , Gregory M. Grason

We model a melt of monodisperse side-chain liquid crystalline polymers as a melt of comb copolymers in which the side groups are rod-coil diblock copolymers. We consider both excluded volume and Maier-Saupe interactions. The first acts…

Soft Condensed Matter · Physics 2007-05-23 Marcela Hernandez , Harry Westfahl Junior

A new Monte Carlo method for computing thermodynamical properties of very large polyelectrolytes is presented. It is based on a renormalization group relating the original polymer to a smaller system, where in addition to the naively…

chem-ph · Physics 2009-10-28 C. Peterson , O. Sommelius , B. Soderberg

Steady state dynamics of clustering, long range order, and inelastic collapse are experimentally observed in vertically shaken granular monolayers. At large vibration amplitudes, particle correlations show only short range order like…

Soft Condensed Matter · Physics 2009-10-31 J. S. Olafsen , J. S. Urbach

We propose a hybrid Molecular Dynamics/Multi-particle Collision Dynamics model to simulate a set of self-assembled semiflexible filaments and free monomers. Further, we introduce a Monte-Carlo scheme to deal with single monomer addition…

Soft Condensed Matter · Physics 2012-02-29 Mathieu Caby , Priscilla Hardas , Sanoop Ramachandran , Jean-Paul Ryckaert

The equilibrium thermodynamic properties of a linear polymer chain confined to a space between two impenetrable walls (lines) at a distance $D$ under various solvent conditions have been studied using series analysis and exact enumeration…

Statistical Mechanics · Physics 2007-05-23 P. K. Mishra , Sanjay Kumar

Multi-component polymer systems are important for the development of new materials because of their ability to phase-separate or self-assemble into nano-structures. The Single-Chain-in-Mean-Field (SCMF) algorithm in conjunction with a soft,…

Computational Physics · Physics 2018-09-05 Ludwig Schneider , Marcus Müller

We use Monte Carlo simulations to study polymer melts consisting of fully flexible and moderately stiff chains in the bond fluctuation model at a volume fraction $0.5$. In order to reduce the local density fluctuations, we test a…

Soft Condensed Matter · Physics 2015-06-24 Hsiao-Ping Hsu

This study reports a general scenario for the out-of-equilibrium features of collapsing polymeric architectures. We use molecular dynamics simulations to characterize the coarsening kinetics, in bad solvent, for several macromolecular…

Soft Condensed Matter · Physics 2019-12-10 Mariarita Paciolla , Daniel J. Arismendi-Arrieta , Angel J. Moreno

Using Monte Carlo simulations, we investigate the self-assembly of model nanoparticles inside a matrix of model equilibrium polymers (or matrix of Wormlike micelles) as a function of the polymeric matrix density and the excluded volume…

Soft Condensed Matter · Physics 2018-04-03 Sk. Mubeena , Apratim Chatterji

A Monte Carlo (MC) simulation method based on the Gillespie algorithm is developed for the polymerization of branched polyetherimides from two back-bone monomers [4,4'-bisphenol A dianhydride (BPADA) and m-phenylenediamine (MPD)], a chain…

Soft Condensed Matter · Physics 2023-04-05 Chengyuan Wen , Roy Odle , Shengfeng Cheng

We use computer simulations to investigate how a catalytic reaction in a polymer sol can induce the formation of a polymer gel. To this aim we consider a solution of homopolymers in which freely-diffusing catalysts convert the originally…

Soft Condensed Matter · Physics 2017-11-10 Virginie Hugouvieux , Walter Kob

Recent developments of microscopic mechanical experiments allow the manipulation of individual polymer molecules in two main ways: \textit{uniform} stretching by external forces and \textit{non-uniform} stretching by external fields. Many…

Biological Physics · Physics 2015-06-11 Fabio Manca , Stefano Giordano , Pier Luca Palla , Fabrizio Cleri , Luciano Colombo

The magnetic order resulting from an indirect exchange between magnetic moments in the metallic phase of a Ga(1-x)Mn(x)As bilayered structure is studied "via" Monte Carlo simulation. The coupling mechanism involves a perturbative…

Materials Science · Physics 2007-05-23 A. Boselli , L. Loureiro da Silva , I. C. da Cunha Lima , A. Ghazali

In conventional molecular simulation, metastable structures often survive over considerable computational time, resulting in difficulties in simulating equilibrium states. In order to overcome this difficulty, here we propose a newly…

Computational Physics · Physics 2011-10-21 Yuki Norizoe , Toshihiro Kawakatsu

Metal-polymer nanocomposites have been investigated extensively during the last years due to their interesting functional applications. They are often produced by vapor phase deposition which generally leads to the self-organized formation…

Materials Science · Physics 2013-09-19 L. Rosenthal , H. Greve , V. Zaporojtchenko , T. Strunskus , F. Faupel , M. Bonitz

We study uniform 3-star polymers with one branch tethered to an attractive surface and another branch pulled by a force away from the surface. Each branch of the 3-star lattice is modelled as a self-avoiding walk on the simple cubic lattice…

Statistical Mechanics · Physics 2019-05-30 C J Bradly , A L Owczarek

We present an effective and simple multiscale method for equilibrating Kremer Grest model polymer melts of varying stiffness. In our approach, we progressively equilibrate the melt structure above the tube scale, inside the tube and finally…

Soft Condensed Matter · Physics 2016-09-21 Carsten Svaneborg , Hossein Ali Karimi-Varzaneh , Nils Hojdis , Frank Fleck , Ralf Everaers

A phase diagram for a surface interacting long flexible partially directed polymer chain in a two-dimensional poor solvent where the possibility of collapse in the bulk exists is determined using exact enumeration method. We used a model of…

Statistical Mechanics · Physics 2020-12-29 Pramod K Mishra , Yashwant Singh