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We present a lattice Monte Carlo simulation for a multiblock copolymer chain of length N=240 and microarchitecture $(10-10)_{12}$.The simulation was performed using the Monte Carlo method with the Metropolis algorithm. We measured average…

Soft Condensed Matter · Physics 2017-08-24 Jakub Krajniak , Michal Banaszak

Single-chain Monte Carlo simulations of amphiphilic diblock star copolymers were carried out in continuous space using implicit solvents. Two distinct architectures were studied: stars with the hydrophobic blocks attached to the core, and…

Soft Condensed Matter · Physics 2009-11-10 Ronan Connolly , Edward G. Timoshenko , Yuri A. Kuznetsov

The structure of a polystyrene matrix filled with tightly cross-linked polystyrene nanoparticles, forming an athermal nanocomposite system, is investigated by means of a Monte Carlo sampling formalism. The polymer chains are represented as…

Soft Condensed Matter · Physics 2014-01-17 Georgios G. Vogiatzis , Evangelos Voyiatzis , Doros N. Theodorou

The structure of polymer coils near interfaces between coexisting phases of symmetrical polymer mixtures (AB) is discussed, as well as the structure of symmetric diblock copolymers of the same chain length N adsorbed at the interface. The…

Soft Condensed Matter · Physics 2015-06-25 K. Binder , M. Mueller , F. Schmid , A. Werner

A technique is presented which maps the parameters of a bead spring model, using the Flory Huggins theory, to a specific experimental system. By keeping only necessary details, for the description of these systems, the mapping procedure…

Soft Condensed Matter · Physics 2016-04-19 George J. Papakonstantopoulos , Kostas Ch. Daoulas , Marcus Muller , Juan J. de Pablo

We present results of Monte Carlo study of the monomer-monomer correlation functions, static structure factor and asphericity characteristics of a single homopolymer in the coil and globular states for three distinct architectures of the…

Soft Condensed Matter · Physics 2009-11-07 Edward G. Timoshenko , Yuri A. Kuznetsov , Ronan Connolly

We use molecular dynamics simulations to study the static properties of a single linear multiblock copolymer chain under poor solvent conditions varying the block length $N$, the number of blocks $n$, and the solvent quality by variation of…

Soft Condensed Matter · Physics 2015-03-19 N. G. Fytas , P. E. Theodorakis

We investigate the phase behavior of symmetric AB diblock copolymers confined into a thin film. The film boundaries are parallel, impenetrable and attract the A component of the diblock copolymer. Using a self-consistent field technique…

Statistical Mechanics · Physics 2009-10-31 Thorsten Geisinger , Marcus Mueller , Kurt Binder

The structure of lamellar phases of symmetric $AB$ diblock copolymers in a thin film is investigated. We quantitatively compare the composition profiles and profiles of individual segments in self-consistent field calculations with Monte…

Statistical Mechanics · Physics 2009-10-31 Thorsten Geisinger , Marcus Mueller , Kurt Binder

We study the phase behavior of single homopolymers in a simple hydrophobic/hydrophilic off-lattice model with sequence independent local interactions. The specific heat is, not unexpectedly, found to exhibit a pronounced peak well below the…

Soft Condensed Matter · Physics 2009-10-31 Anders Irbäck , Erik Sandelin

Molecular dynamics simulations are used to study the phase behavior of linear multiblock copolymers with two types of monomers, A and B, where the length of the polymer blocks $N_{A}$ and $N_{B}$ ($N_{A}=N_{B}=N$), the number of the blocks…

Soft Condensed Matter · Physics 2011-02-04 Panagiotis E. Theodorakis , Nikolaos G. Fytas

In this article, a novel cluster analysis algorithm was employed in the study of polymer coil to globule transition via single chain Monte Carlo simulations. The algorithm, which has been recently applied in Molecular Dynamics simulations…

Soft Condensed Matter · Physics 2013-11-21 T. E. Raptis , Vasilios E. Raptis

Block copolymer melts self-assemble in the bulk into a variety of nanostructures, making them perfect candidates to template the position of nanoparticles. The morphological changes of block copolymers are studied in the presence of a…

Soft Condensed Matter · Physics 2019-10-31 Javier Diaz , Marco Pinna , Andrei V. Zvelindovsky , Ignacio Pagonabarraga

We investigate the thermal and structural properties of knotted diblock copolymer rings using a coarse-grained lattice model in an implicit solvent. The system is studied by means of the Wang--Landau Monte Carlo algorithm, allowing us to…

Soft Condensed Matter · Physics 2026-05-18 Neda Abbasi Taklimi , Franco Ferrari , Marcin R. Piątek , Luca Tubiana

A linear copolymer made of two reciprocally attracting N-monomer blocks collapses to a compact phase through a novel transition, whose exponents are determined with extensive MC simulations in two and three dimensions. In the former case,…

Soft Condensed Matter · Physics 2009-10-31 E. Orlandini , F. Seno , A. L. Stella

The properties of diluted symmetric A-B diblock copolymers at the interface between A and B homopolymer phases are studied by means of Monte Carlo (MC) simulations of the bond fluctuation model. We calculate segment density profiles as well…

Chemical Physics · Physics 2015-06-26 A. Werner , F. Schmid , K. Binder , M. Mueller

The coil-globule transition has been studied for A-B copolymer chains both by means of lattice Monte Carlo simulations using bond fluctuation algorithm and by a numerical self-consistent field method. Copolymer chains of fixed length with A…

Collapse of the polymer chain upon the sharp decrease of solvent quality is studied. During collapse, any pair of polymer units appearing in a sufficiently close vicinity in space has the possibility with a certain probability to form an…

Soft Condensed Matter · Physics 2019-11-07 A. M. Astakhov , S. K. Nechaev , K. E. Polovnikov

We examine the phase transition of polymer adsorption as well as the underlying kinetics of polymer binding from dilute solutions on a structureless solid surface. The emphasis is put on the properties of regular multiblock copolymers,…

Soft Condensed Matter · Physics 2009-09-03 A. Milchev , V. Rostiashvili , S. Bhattacharya , T. Vilgis

Block copolymer (BCP) melt assembly has been the subject of decades of study, with focus largely on self-organized spatial patterns of periodically-ordered segment density. In this study, we demonstrate that underlying these otherwise…

Soft Condensed Matter · Physics 2017-06-21 Ishan Prasad , Youngmi Seo , Lisa M. Hall , Gregory M. Grason
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