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Different approaches have improved the sensitivity of either electron or nuclear magnetic resonance to the single spin level. For optical detection it has essentially become routine to observe a single electron spin or nuclear spin.…

Mesoscale and Nanoscale Physics · Physics 2016-06-29 Jörg Wrachtrup , Amit Finkler

Magnetic resonance spectroscopy is universally regarded as one of the most important tools in chemical and bio-medical research. However, sensitivity limitations typically restrict imaging resolution to length scales greater than 10 \mu m.…

The rapid decay of target signal strength with distance from the sensor presents a key challenge in nanoscale magnetic sensing with nitrogen-vacancy (NV) centers in diamond, limiting both sensitivity and spatial resolution. Here we…

Nitrogen vacancy (NV) color centers in diamond are a leading modality for both superresolution optical imaging and nanoscale magnetic field sensing. In this work, we solve the remaining key challenge of performing optical magnetic imaging…

Nuclear spin imaging at the atomic level is essential for the understanding of fundamental biological phenomena and for applications such as drug discovery. The advent of novel nano-scale sensors has given hope of achieving the…

Quantum Physics · Physics 2015-11-25 Ashok Ajoy , Ulf Bissbort , Mikhail D. Lukin , Ronald L. Walsworth , Paola Cappellaro

Spins associated to optically accessible solid-state defects have emerged as a versatile platform for exploring quantum simulation, quantum sensing and quantum communication. Pioneering experiments have shown the sensing, imaging, and…

Isolated nuclear spins offer a promising building block for quantum information processing systems, but their weak interactions often impede preparation, control, and detection. Hyperfine coupling to a proximal electronic spin can enhance…

Quantum Physics · Physics 2013-05-29 Benjamin Smeltzer , Jean McIntyre , Lilian Childress

Magnetic Resonance Imaging (MRI) can characterize and discriminate among tissues using their diverse physical and biochemical properties. Unfortunately, submicrometer screening of biological specimens is presently not possible, mainly due…

Mesoscale and Nanoscale Physics · Physics 2010-11-03 C. A. Meriles , L. Jiang , G. Goldstein , J. S. Hodges , J. R. Maze , M. D. Lukin , P. Cappellaro

Nuclear magnetic resonance (NMR) is a powerful method for determining the structure of molecules and proteins. While conventional NMR requires averaging over large ensembles, recent progress with single-spin quantum sensors has created the…

Efficiently detecting and characterizing individual spins in solid-state hosts is an essential step to expand the fields of quantum sensing and quantum information processing. While selective detection and control of a few 13C nuclear spins…

Quantum Physics · Physics 2020-10-22 Hyunseok Oh , Jiwon Yun , M. H. Abobeih , Kyung-Hoon Jung , Kiho Kim , T. H. Taminiau , Dohun Kim

Electron and nuclear spins of diamond nitrogen-vacancy (NV) centers are good candidates for quantum information processing as they have long coherence time and can be initialized and read out optically. However, creating a large number of…

Quantum Physics · Physics 2019-11-19 Zhujing Xu , Zhang-qi Yin , Qinkai Han , Tongcang Li

We use the electronic spin of a single Nitrogen-Vacancy (NV) defect in diamond to observe the real-time evolution of neighboring single nuclear spins under ambient conditions. Using a diamond sample with a natural abundance of $^{13}$C…

Quantum Physics · Physics 2015-06-11 A. Dréau , P. Spinicelli , J. R. Maze , J. -F. Roch , V. Jacques

A new method for detecting the magnetic resonance of electronic spins at low temperature is demonstrated. It consists in measuring the signal emitted by the spins with a superconducting qubit that acts as a single-microwave-photon detector,…

A single nitrogen-vacancy (NV) center in diamond is a prime candidate for a solid-state quantum magnetometer capable of detecting single nuclear spins with prospective application to nuclear magnetic resonance (NMR) at the nanoscale.…

Quantum Physics · Physics 2020-02-07 Daiki Misonou , Kento Sasaki , Shuntaro Ishizu , Yasuaki Monnai , Kohei M. Itoh , Eisuke Abe

Magnetic resonance imaging (MRI) has revolutionized biomedical science by providing non-invasive, three-dimensional biological imaging. However, spatial resolution in conventional MRI systems is limited to tens of microns, which is…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 M. S. Grinolds , M. Warner , K. De Greve , Y. Dovzhenko , L. Thiel , R. L. Walsworth , S. Hong , P. Maletinsky , A. Yacoby

Sensing single nuclear spins is a central challenge in magnetic resonance based imaging techniques. Although different methods and especially diamond defect based sensing and imaging techniques in principle have shown sufficient…

We describe a technique that enables a strong, coherent coupling between a single electronic spin qubit associated with a nitrogen-vacancy impurity in diamond and the quantized motion of a magnetized nano-mechanical resonator tip. This…

Other Condensed Matter · Physics 2009-12-20 P. Rabl , P. Cappellaro , M. V. Gurudev Dutt , L. Jiang , J. R. Maze , M. D. Lukin

Studies of individual quantum systems, which have led to considerable progress in our understanding of quantum physics, have traditionally been associated with atomic gases. In the last decades however, the emphasis has shifted towards…

Materials Science · Physics 2020-11-26 J. -P. Tetienne , L. P. McGuinness , V. Jacques

Characterization of the molecular properties of surfaces under ambient or chemically reactive conditions is a fundamental scientific challenge. Moreover, many traditional analytical techniques used for probing surfaces often lack dynamic or…

Quantum sensors have attracted broad interest in the quest towards sub-micronscale NMR spectroscopy. Such sensors predominantly operate at low magnetic fields. Instead, however, for high resolution spectroscopy, the high-field regime is…

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