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The results of ac and dc magnetization and heat capacity measurements as a function of temperature (T = 1.8 to 300 K) are reported for a quasi-one-dimensional compound, Ca$_3$CuMnO$_6$, crystallizing in a triclinically distorted…

Strongly Correlated Electrons · Physics 2009-11-10 Kausik Sengupta , S. Rayaprol , K. K. Iyer , E. V. Sampathkumaran

We report a neutron diffraction and muon spin relaxation muSR study of static and dynamical magnetic properties of BaCo2V2O8, a quasi-one-dimensional spin-chain system. A proposed model for the antiferromagnetic structure includes: a…

We explore the spin states in the quantum spin chain compound SrCo$_{2}$V$_{2}$O$_{8}$ up to 14.9 T and down to 50 mK, using single-crystal neutron diffraction. Upon cooling in zero-field, antiferromagnetic (AFM) order of N\'eel type…

Strongly Correlated Electrons · Physics 2019-07-05 L. Shen , O. Zaharko , J. O. Birk , E. Jellyman , Z. He , E. Blackburn

CoSe$_2$O$_5$ has a crystal structure consisting of zig-zag chains of edge shared CoO$_6$ octahedra running along the c axis, with the chains separated by Se$_2$O$_5^{2-}$ units. Magnetic susceptibility measurements indicate a transition at…

Materials Science · Physics 2012-02-02 Brent C. Melot , Brian Paden , Ram Seshadri , Ambesh Dixit , Gavin Lawes , Emmanuelle Suard

CsO2 is a member of the family of alkali superoxides (formula AO2 with A= Na, K, Rb and Cs) that exhibit magnetic behavior arising from open $p$-shell electrons residing on O2- molecules. We use neutron diffraction to solve the crystal and…

Strongly Correlated Electrons · Physics 2023-11-10 R. A. Ewings , M. Reehuis , F. Orlandi , P. Manuel , D. D. Khalyavin , A. S. Gibbs , A. D. Fortes , A. Hoser , A. J. Princep , M. Jansen

We report on the magnetic properties of CsCo$_2$Se$_2$ with ThCr$_2$Si$_2$ structure, which we have characterized through a series of magnetization and neutron diffraction measurements. We find that CsCo$_2$Se2$_2$ undergoes a phase…

Strongly Correlated Electrons · Physics 2016-05-20 F. von Rohr , A. Krzton-Maziopa , V. Pomjakushin , H. Grundmann , Z. Guguchia , W. Schnick , A. Schilling

We present a detailed powder and single crystal neutron diffraction study of the spin chain compound Ca3Co2O6. Below 25 K, the system orders magnetically with a modulated partially disordered antiferromagnetic structure. We give a…

Strongly Correlated Electrons · Physics 2008-09-17 S. Agrestini , L. C. Chapon , A. Daoud-Aladine , J. Schefer , A. Gukasov , C. Mazzoli , M. R. Lees , O. A. Petrenko

The magnetic structure of the spin-chain antiferromagnet SrCo2V2O8 is determined by single-crystal neutron diffraction experiment. The system undergoes magnetic long range order below T_N = 4.96 K. The moment of 2.16{\mu}_B per Co at 1.6 K…

Strongly Correlated Electrons · Physics 2016-03-28 Juanjuan Liu , Jinchen Wang , Wei Luo , Jieming Sheng , Zhangzhen He , S. A. Danilkin , Wei Bao

Identifying and characterizing new magnetic systems with Co2+ ions can enhance our understanding of quantum behavior since Co2+ can host a pseudospin-1/2 magnetic ground state. Understanding the magnetic ground state and the phase diagrams…

We present a detailed investigation of the magnetic properties of the spin-$\frac{3}{2}$ system Li$_2$Co(WO$_4$)$_2$ by means of magnetic susceptibility and specific heat. Our experimental results show that in Li$_2$Co(WO$_4$)$_2$ a…

Strongly Correlated Electrons · Physics 2014-11-25 I. Panneer Muthuselvam , R. Sankar , A. V. Ushakov , G. Narsinga Rao , Sergey V. Streltsov , F. C. Chou

Magnetic systems with noncentrosymmetric crystal structures are renowned for their complex magnetic ordering and diverse and fascinating physical properties. In this report, we provide a comprehensive study of the chiral magnetic system…

Using powder neutron diffraction we have discovered an unusual magnetic order-order transition in the Ising spin chain compound Ca3Co2O6. On lowering the temperature an antiferromagnetic phase with propagation vector k=(0.5,-0.5,1) emerges…

Strongly Correlated Electrons · Physics 2011-05-17 S. Agrestini , C. L. Fleck , L. C. Chapon , C. Mazzoli , A. Bombardi , M. R. Lees , O. A. Petrenko

We have performed a powder neutron diffraction study on CsO$_2$, where the unpaired electron with $s=1/2$ in the $\pi^*$ orbital of the O$_2^-$ ion is responsible for the magnetism. The magnetic reflections 0 $\frac{1}{2}$ 0 and 0…

Strongly Correlated Electrons · Physics 2023-09-07 Takehito Nakano , Shun Kontani , Masatoshi Hiraishi , Kaito Mita , Mizuki Miyajima , Takashi Kambe

We report an investigation on structure and magnetic properties of the $S=3/2$ zigzag spin chain compound BaCoTe$_2$O$_7$. Neutron diffraction measurements reveal BaCoTe$_2$O$_7$ crystallizes in the noncentrosymmetric space group $Ama2$…

Strongly Correlated Electrons · Physics 2021-07-06 Lisi Li , Xunwu Hu , Zengjia Liu , Jia Yu , Benyuan Cheng , Sihao Deng , Lunhua He , Kun Cao , Dao-Xin Yao , Meng Wang

To study the relationship between the properties of low-dimensional spin systems with weakly coupled Cu-triangles and their crystal structure, single crystals of $Cs_3Cu_3Cl_8OH$ (1) and the new $Cs_3Cu_3Cl_{7.6}Br_{0.4}OH$ (2) were grown.…

Alkali superoxides differ from conventional transition metal magnets, exhibit magnetism from partially occupied oxygen molecular $\pi^*$-orbitals. Among them, CsO$_2$ stands out for its potential to exhibit novel quantum collective…

Strongly Correlated Electrons · Physics 2024-11-12 Ryota Ono , Ravi Kaushik , Sergey Artyukhin , Martin Jansen , Igor Solovyev , Russell A. Ewings

$^{59}$Co and $^{31}$P nuclear magnetic resonance (NMR) measurements in external magnetic and zero magnetic fields have been performed to investigate the magnetic properties of the A-type antiferromagnetic (AFM) CaCo$_2$P$_2$. NMR data,…

Strongly Correlated Electrons · Physics 2018-12-26 N. Higa , Q. -P. Ding , A. Teruya , M. Yogi , M. Hedo , T. Nakama , Y. Ōnuki , Y. Furukawa

Magnetic correlations of two iso-structural quasi-one-dimensional (1D) antiferromagnetic spin-chain compounds Sr$M_2$V$_2$O$_8$ ($M$ = Co, Mn) have been investigated by magnetization and powder neutron diffraction. Two different collinear…

Strongly Correlated Electrons · Physics 2014-12-17 A. K. Bera , B. Lake , W. -D. Stein , S. Zander

This paper presents results of a recent study of multiferroic \CCO\ by means of single crystal neutron diffraction. This system has two close magnetic phase transitions at $T\nsub{N1}=24.2$ K and $T\nsub{N2}=23.6$ K. The low temperature…

Materials Science · Physics 2015-05-30 M. Frontzek , G. Ehlers , A. Podlesnyak , H. Cao , M. Matsuda , O. Zaharko , N. Aliouane , S. Barilo , S. V. Shiryaev

Neutron and synchrotron resonant X-ray magnetic scattering (RXMS) complemented by heat capacity and resistivity measurements reveal the evolution of the magnetic structures of Fe and Ce sublattices in single crystal CeFeAsO. The RXMS of…

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