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A novel polarization-modulation transient method has been developed for studying fast anisotropic relaxation in electronic excited states of polyatomic and biologically relevant molecules under excitation with femtosecond laser pulses. The…

Chemical Physics · Physics 2020-05-12 Ioanna Gorbunova , Nikolay Bezverkhnii , Maxim Sasin , Idris Gagzhiev , Oleg Vasyutinskii

The analytical and numerical analysis of the dynamics of charged particles in the field of an intensive transverse electromagnetic wave in a vacuum presented in the article. Identifies the conditions for resonant acceleration of particles.…

General Physics · Physics 2021-04-26 Vyacheslav Aleksandrovich Buts

Semiconductor quantum dots driven by the broadband radiation fields of nearby quantum point contacts provide an exciting new setting for probing dynamics in driven quantum systems at the nanoscale. We report on real-time charge-sensing…

Mesoscale and Nanoscale Physics · Physics 2014-03-14 Simon Gustavsson , Mark S. Rudner , Leonid S. Levitov , Renaud Leturcq , Matthias Studer , Thomas Ihn , Klaus Ensslin

We explore the novel capabilities offered by attosecond extreme ultraviolet and x-ray pulses that can be now generated by free-electron lasers and high-harmonics generation sources for probing photon-induced electron dynamics in molecules.…

Quantum Physics · Physics 2023-02-15 Marvin Reuner , Daria Popova-Gorelova

We report generation of cascaded rotational Raman scattering up to 58th orders in coherently excited CO_2 molecules. The high-order Raman scattering, which produces a quasiperiodic frequency comb with more than 600 sidebands, is obtained…

We investigate the propagation of ultra-short laser pulses in atomic rubidium vapor. The pulses are intensive enough to ionize the atoms and are directly resonant with the 780 nm $D_2$ line. We derive a relatively simple theory for…

Optics · Physics 2019-07-03 Gabor Demeter

Ultrafast laser excitation can create coherent superpositions of electronic states in molecules and trigger ultrafast flow of electron density on few- to sub-femtosecond time scales. While recent attosecond experiments have addressed…

Chemical Physics · Physics 2020-11-18 Yuki Kobayashi , Daniel M. Neumark , Stephen R. Leone

We propose a new scenario to apply IR-pump-XUV-probe schemes to resolving strong field ionization induced and attosecond pulse driven electron-hole dynamics and coherence in real time. The coherent driving of both the infrared laser and the…

Atomic Physics · Physics 2016-02-26 Jing Zhao , Jianmin Yuan , Zengxiu Zhao

A study about the reflection and transmission of an electromagnetic pulse through a slab doped with four-level atomic system has been presented. The doped atoms are considered to be in N-configuration with a pump field and a weak probe…

Quantum Physics · Physics 2024-03-26 Yasir Ali

Extreme ultraviolet (XUV) attosecond pulses, generated by a process known as laser-induced electron recollision, are a key ingredient for attosecond metrology, providing a tool to precisely initiate and probe sub-femtosecond dynamics in the…

Atomic Physics · Physics 2016-02-24 Yunpei Deng , Zhinan Zeng , Zhengmao Jia , Pavel Komm , Yinhui Zheng , Xiaochun Ge , Ruxin Li , Gilad Marcus

Ionization of an atom or molecule by a strong laser field produces sub-optical cycle wave packets whose control has given rise to attosecond science. The final states of the wave packets depend on ionization and deflection by the laser…

We show that for collisions of electrons with a high-intensity laser, discrete photon emissions introduce a transverse beam spread which is distinct from that due to classical (or beam shape) effects. Via numerical simulations, we show that…

High Energy Physics - Phenomenology · Physics 2014-08-06 D. G. Green , C. N. Harvey

The dynamics of electron injection in the direct laser acceleration (DLA) regime was investigated by means of three-dimensional particle-in-cell simulations and theoretical analysis. It is shown that when an ultra-intense laser pulse…

Plasma Physics · Physics 2018-09-19 K. Jiang , C. T. Zhou , T. W. Huang , L. B. Ju , H. Zhang , B. Qiao , S. C. Ruan

The single ionization of noble gas atoms by the combined action of XUV attopulses and an infrared laser field is theoretically investigated by means of a non-perturbative model that under certain approximations gives closed-form expressions…

Atomic Physics · Physics 2015-12-21 D. I. R. Boll , O. A. Fojón

The ultrafast electronic and nuclear dynamics of H2 laser-induced double ionization is studied using a time-dependent wave packet approach that goes beyond the fixed nuclei approximation. The double ionization pathways are analyzed by…

Quantum Physics · Physics 2011-11-09 Sebastien Saugout , Christian Cornaggia , Annick Suzor-Weiner , Eric Charron

We investigate the evolution of extreme ultraviolet (XUV) spectral lineshapes in an optically-thick helium gas under near-infrared (IR) perturbation. In our experimental and theoretical work, we systematically vary the IR intensity,…

Atomic Physics · Physics 2016-03-09 Chen-Ting Liao , Seth Camp , Kenneth J. Schafer , Mette B. Gaarde , Arvinder Sandhu

Anisotropic two-dimensional (2D) semiconductors recently have emerged as a promising platform for polarization-controlled Raman amplification. In this study, we probe energy-dependent resonant Raman scattering in few layer ReS2 under…

Optics · Physics 2025-07-22 Pritam Das , Devarshi Chakrabarty , Neha Gill , Sajal Dhara

Time-resolved investigations of ultrafast electronic and molecular dynamics were not possible until recently. The typical time scale of these processes is in the picosecond to attosecond realm. The tremendous technological progress in…

Atomic Physics · Physics 2013-05-14 Stefan Pabst

Tunneling ionization of an atom in ultrashort laser pulses is considered. When the driving laser pulse is switched-on and -off with a steep slope, the photoelectron momentum distribution (PMD) shows an edge-effect because of the…

Atomic Physics · Physics 2022-07-07 M. Klaiber , Q. Z. Lv , K. Z. Hatsagortsyan , C. H. Keitel

An isolated attosecond vortex $\gamma$-ray pulse is generated by using a relativistic spatiotemporal optical vortex (STOV) laser in particle-in-cell simulations. A $\sim$ 300-attosecond electron slice with transverse orbital angular…

Plasma Physics · Physics 2024-11-11 Fengyu Sun , Xinyu Xie , Wenpeng Wang , Stefan Weber , Xin Zhang , Yuxin Leng , Ruxin Li , Zhizhan Xu