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Electronically-induced desorption from solid Ar pre-irradiated by a low-energy electron beam was investigated by activation spectroscopy methods - photon-stimulated exoelectron emission and photon-stimulated luminescence in combination with…

We propose a new mechanism to explain the origin of optical gain in the transitions between excited and ground state of the ionized nitrogen molecule following irradiation of neutral nitrogen molecules with an intense ultra short laser…

Experiments carried out at our laboratories have led to observing a new type of electrification, now called surface photocharging. For a consistent description, we are weighing carefully the experimental evidence against the common…

Materials Science · Physics 2007-05-23 O. Ivanov , R. Dyulgerova , M. Georgiev

The dynamics following the photoexcitation of Na and Li atoms located on the surface of helium nanodroplets has been investigated in a joint experimental and theoretical study. Photoelectron spectroscopy has revealed that excitation of the…

Atomic and Molecular Clusters · Physics 2017-08-23 Alberto Hernando , Manuel Barranco , Martí Pi , Evgeniy Loginov , Marina Langlet , Marcel Drabbels

The excitation of nitromethane CH$_3$NO$_2$, which is an important propellant and prototypic molecule for large class of explosives, has been investigated by electron impact and subsequent emission of photons in the UV-VIS spectral region…

Core-excitation of water ice releases many different molecules and ions in the gas phase. Studying these desorbed species and the underlying mechanisms can provide useful information on the effects of X-ray irradiation in ice. We report a…

Chemical Physics · Physics 2020-10-20 R. Dupuy , G. Féraud , M Bertin , C. Romanzin , L. Philippe , T. Putaud , X. Michaut , R. Cimino , V. Baglin , J. -H. Fillion

Recent results on the study of spontaneous and stimulated luminescence of solid nitrogen in the near-infrared NIR range are presented. Irradiation was performed with an electron beam of subthreshold energy in the dc mode. Three series of…

Chemical Physics · Physics 2025-01-13 M. A. Bludov , I. V. Khyzhniy , S. A. Uyutnov , G. B. Gumenchuk , E. V. Savchenko

New results on the study of radiation effects in solid nitrogen and N$_2$-doped Ne matrix are presented with a focus on the so-called $\gamma$-line origin. The irradiation was carried out in dc regime with an electron beam of subthreshold…

Chemical Physics · Physics 2023-11-30 E. V. Savchenko , I. V. Khyzhniy , S. A. Uyutnov , M. A. Bludov

Electrically detected magnetic resonance is used to identify recombination centers in a set of Czochralski grown silicon samples processed to contain strained oxide precipitates with a wide range of densities (~ 1e9 cm-3 to ~ 7e10 cm-3).…

Materials Science · Physics 2012-01-11 V. Lang , J. D. Murphy , R. J. Falster , J. J. L. Morton

We report direct evidence of two mechanisms responsible for the excitation of optically active Er3+ ions in GaN epilayers grown by metal-organic chemical vapor deposition. These mechanisms, resonant excitation via the higher-lying inner 4f…

Materials Science · Physics 2015-07-21 D. K. George , M. Hawkins , M. McLaren , H. X. Jiang , J. Y. Lin , J. M. Zavada , N. Q. Vinh

The absorption of a photon and the emission of an electron is not a simple, two-particle process. The complicated many-electron features observed during core photo-ionization can therefore reveal many of the hidden secrets about the ground…

Strongly Correlated Electrons · Physics 2018-07-04 J. C. Woicik , J. M. Ablett , N. F. Quackenbush , A. K. Rumaiz , C. Weiland , T. C. Droubay , S. A. Chambers

Electron injection from an adsorbed molecule to the substrate (heterogeneous electron transfer) is studied. One reaction coordinate is used to model this process. The surface phonons and/or the electron-hole pairs together with the internal…

Chemical Physics · Physics 2009-11-07 Michael Schreiber , Ivan Kondov , Ulrich Kleinekathoefer

When redox active molecules are covalently tethered to the surface of the n-doped silicon, light induces their oxidation by the semiconductor. To visualize this charge separation we have followed the formation and decay of the surface…

Materials Science · Physics 2008-12-31 Andrei V. Pakoulev , Vladimir Burtman , Dmitry Zaslavsky

Electron scattering and dielectronic recombination with an ion in the presence of a neighboring atom is studied. The incident electron is assumed to be captured by the ion, leading to resonant excitation of the atom which afterwards may…

Atomic Physics · Physics 2018-08-01 A. Eckey , A. Jacob , A. B. Voitkiv , C. Müller

Electronic excitations near the surface of water ice lead to the desorption of adsorbed molecules, through a so far debated mechanism. A systematic study of photon-induced indirect desorption, revealed by the spectral dependence of the…

Quantum coherence in quantum optics is an essential part of optical information processing and light manipulation. Alkali metal vapors, despite the numerous shortcomings, are traditionally used in quantum optics as a working medium due to…

The adsorption and dissociation of nitrogen molecule on Fe(111) surface is studied by density functional theory calculations. The simulation results show that the molecule needs to acquire parallel orientation with respect to the surface…

Materials Science · Physics 2014-12-30 Myong-Song Ryang , Nam-Hyok Kim , Song-Jin Im

Ce-doped SiO x N y films are deposited by magnetron reactive sputtering from a CeO 2 target under nitrogen reactive gas atmosphere. Visible photoluminescence measurements regarding the nitrogen gas flow reveal a large emission band centered…

We study the dissociation of H$_2$$^+$ in uv laser pulses by solving the non-Born-Oppenheimer time-dependent Schr\"{o}dinger equation as a function of the photon energy $\omega$ of the pulse. Significant enhancements of the dissociation…

Atomic and Molecular Clusters · Physics 2014-07-22 Kunlong Liu , Qianguang Li , Pengfei Lan , Peixiang Lu

The nitrogen-vacancy (NV) centre in diamond is emerging as a promising platform for solid-state quantum information processing and nanoscale metrology. Of interest in these applications is the manipulation of the NV charge, which can be…

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