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We use R-Matrix with Time-dependence (RMT) theory, with spin-orbit effects included, to study krypton irradiated by two time-delayed XUV ultrashort pulses. The first pulse excites the atom to 4s$^{2}$4p$^{5}$5s. The second pulse then…

We employ the recently developed multi-photon R-matrix method for molecular above-threshold photoionization to obtain second-order ionization amplitudes that govern the interference in RABITT experiments. This allows us to extract RABITT…

Atomic Physics · Physics 2022-05-03 Jakub Benda , Zdeněk Mašín , Jimena D. Gorfinkiel

We predict a significant delay of two-electron photoemission from the helium atom after absorption of an attosecond XUV pulse. We establish this delay by solving the time dependent Schr\"odinger equation and by subsequent tracing the…

Atomic Physics · Physics 2026-03-03 A. S. Kheifets , I. A. Ivanov , Igor. Bray

Recent angle-resolved RABBITT experiments have shown that the photoionization time delay depends on the emission angle of the photoelectron. In this work we demonstrate that for photoemission from helium accompanied by shake-up (correlation…

Atomic Physics · Physics 2020-09-30 Stefan Donsa , Manuel Ederer , Renate Pazourek , Joachim Burgdörfer , Iva Březinová

We analyze two-photon double ionization of helium in both the nonsequential and sequential regime. We show that the energy spacing between the two emitted electrons provides the key parameter that controls both the energy and the angular…

Atomic Physics · Physics 2013-05-24 R. Pazourek , J. Feist , S. Nagele , E. Persson , B. I. Schneider , L. A. Collins , J. Burgörfer

In this work we develop an approach for a molecular hydrogen ion (H2+) in the Born-Oppenheimer approximation while exposed to intense short-pulse radiation. Our starting point is the R-Matrix incorporating Time (RMT) formulation for atomic…

Atomic Physics · Physics 2016-01-01 Cathal Ó Broin , Lampros A. A. Nikolopoulos

We analyze the photoelectron angular distribution in two-pathway interference between non\-resonant one-photon and resonant two-photon ionization of neon. We consider a bichromatic femtosecond XUV pulse whose fundamental frequency is tuned…

We present accurate time-dependent ab initio calculations on fully differential and total integrated (generalized) cross sections for the nonsequential two-photon double ionization of helium at photon energies from 40 to 54 eV. Our…

Atomic Physics · Physics 2008-05-07 J. Feist , S. Nagele , R. Pazourek , E. Persson , B. I. Schneider , L. A. Collins , J. Burgdörfer

Photoelectron emission from excited states of laser-dressed atomic helium is analyzed with respect to laser intensity-dependent excitation energy shifts and angular distributions. In the two-color XUV (exteme ultra\-violet) -- IR (infrared)…

We investigate the role of electron correlation in the two-photon double ionization of helium for ultrashort XUV pulses with durations ranging from a hundred attoseconds to a few femtoseconds. We perform time-dependent ab initio…

Measured photoionization time delays may exhibit large variations as a function of the emission angles, even for spherically symmetric targets, as shown in recent RABBITT (reconstruction of attosecond beating by interference of two-photon…

Atomic Physics · Physics 2022-12-29 D. I. R. Boll , L. Martini , A. Palacios , O. A. Fojón

Double photo-electron momentum spectra of the Helium atom are calculated \textit{ab initio} at extreme ultra-violet and near infrared wavelengths. At short wavelengths two-photon double ionization yields, two-electron energy spectra, and…

Computational Physics · Physics 2016-02-17 Alejandro Zielinski , Vinay Pramod Majety , Armin Scrinzi

The angular distribution of the emitted electrons, following the two-photon ionization of the hydrogen-like ions, is studied within the framework of second order perturbation theory and the Dirac equation. Using a density matrix approach,…

Atomic Physics · Physics 2007-05-23 Peter Koval , Stephan Fritzsche , Andrey Surzhykov

We investigate an angular dependence of the photoemission time delay in helium as measured by the RABBITT (Reconstruction of Attosecond Beating By Interference of Two-photon Transitions) technique. The measured time delay $…

Atomic Physics · Physics 2016-05-17 I A Ivanov , J M Dahlström , E Lindroth , A S Kheifets

We perform numerical simulations for photoionization of the argon atom when exposed to a combined field of an infrared laser (abbreviated IR) and its 13th harmonic (H13) by solving the Time-Dependent Schr\"odinger Equation (TDSE)], noting…

Atomic Physics · Physics 2022-08-26 Soumia Chqondi , Souhaila Chaddou , Abdelkader Makhoute

A fully relativistic calculation of the double photoionization of helium-like atoms is presented. The approach is based on the partial-wave representation of the Dirac continuum states and accounts for the retardation in the…

Atomic Physics · Physics 2015-05-30 V. A. Yerokhin , A. Surzhykov

Opacity determines radiation transport through material media. In a plasma source the primary contributors to atomic opacity are bound-bound line transitions and bound-free photoionization into the continuum. We review the theoretical…

Solar and Stellar Astrophysics · Physics 2023-03-08 Anil Pradhan

We study nondipole effects in multiphoton ionization of a two-dimensional hydrogen-like atom by a flat-top laser pulse of varied intensity. For this purpose, we solve numerically a two-dimensional Schr\"odinger equation treating a…

Atomic Physics · Physics 2024-12-25 J. Z. Kamiński , K. Krajewska

We present a theoretical study of ionization of the hydrogen atom due to an XUV pulse in the presence of an IR laser with both fields linearly polarized in the same direction. In particular, we study the energy distribution of…

Atomic Physics · Physics 2017-08-23 A. A. Gramajo , R. Della Picca , D. G. Arbó

A strong helicity dependence of reconstruction of attosecond bursts by beating of two-photon transitions (RABBITT) with circularly polarized XUV and IR pulses was reported by Han et al. [Nature Physics 19, 230 and arXiv 2302.04137 (2023)].…

Atomic Physics · Physics 2026-03-03 Anatoli Kheifets