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Enormous enhancement in the viscosity of a liquid near its glass transition is generally connected to the growing many-body static correlations near the transition, often coined as `amorphous ordering'. Estimating the length scales of such…

Large scale simulations of two-dimensional bidisperse granular fluids allow us to determine spatial correlations of slow particles via the four-point structure factor $S_4(q,t)$. Both cases, elastic ($\varepsilon=1$) as well as inelastic…

Statistical Mechanics · Physics 2014-07-16 Karina E. Avila , Horacio E. Castillo , Andrea Fiege , Katharina Vollmayr-Lee , Annette Zippelius

We investigate the occurrence of waterlike thermodynamic and dynamic anomalous behavior in a one dimensional lattice gas model. The system thermodynamics is obtained using the transfer matrix technique and anomalies on density and…

Soft Condensed Matter · Physics 2015-03-11 Marco Aurélio A. Barbosa , Fernando Vito Barbosa , Fernando Albuquerque de Oliveira

We study dynamical heterogeneity and glassy dynamics in a kinetically constrained lattice gas model which has both translational and rotational degrees of freedom. We find that the rotational diffusion constant tracks the structural…

Soft Condensed Matter · Physics 2015-06-25 Albert C. Pan

Stimuli-responsive gels are the gels that vary the volume depending on environmental conditions. It has been reported that the stimuli-responsive gel with an inhomogeneous structure exhibits faster volume change than the gel without it. It…

Soft Condensed Matter · Physics 2024-07-23 Yuhei Yamada , Shingo Maeda

We perform molecular-dynamics simulations of a molecular system in supercooled states for different values of inertia parameters to provide evidence that the long-time dynamics depends only on the equilibrium structure. This observation is…

Soft Condensed Matter · Physics 2009-11-10 S. -H. Chong , F. Sciortino

We use recently introduced three-point dynamic susceptibilities to obtain an experimental determination of the temperature evolution of the number of molecules, N_corr, that are dynamically correlated during the structural relaxation of…

We explore the instabilities developed in a fluid in which viscosity depends on temperature. In particular, we consider a dependency that models a very viscous (and thus rather rigid) lithosphere over a convecting mantle. To this end, we…

Fluid Dynamics · Physics 2014-02-13 Jezabel Curbelo , Ana M. Mancho

We present a comprehensive theoretical study of finite size effects in the relaxation dynamics of glass-forming liquids. Our analysis is motivated by recent theoretical progress regarding the understanding of relevant correlation length…

Statistical Mechanics · Physics 2012-09-12 Ludovic Berthier , Giulio Biroli , Daniele Coslovich , Walter Kob , Cristina Toninelli

Discrete simulation methods are efficient tools to investigate the complex behaviors of complex fluids made of either dry granular materials or dilute suspensions. By contrast, materials made of soft and/or concentrated units (emulsions,…

Fluid Dynamics · Physics 2008-12-18 Pierre Rognon , Cyprien Gay

In models of Pt 111 and Pt 100 surfaces in water, motions of molecules in the first hydration layer are spatially and temporally correlated. To interpret these collective motions, we apply quantitative measures of dynamic heterogeneity that…

Materials Science · Physics 2015-06-15 Adam P. Willard , David T. Limmer , Paul A. Madden , David Chandler

We study the role of elasticity-induced facilitation on the dynamics of glass-forming liquids by a coarse-grained two-dimensional model in which local relaxation events, taking place by thermal activation, can trigger new relaxations by…

Disordered Systems and Neural Networks · Physics 2023-04-05 Misaki Ozawa , Giulio Biroli

Liquids in equilibrium exhibit two types of disorder, simple and complex. Typical simple disorder liquid are liquid nitrogen, or weakly polar liquids. Complex liquids concern those who can form long lived local assemblies, and cover a large…

Chemical Physics · Physics 2023-06-02 Bernarda Lovrinčević , Martina Požar , Ivo Jukić , David Perera , Aurélien Perera

Supercooled liquids and dense colloids exhibit anomalous behaviour known as "spatially heterogeneous dynamics" (SHD), which becomes increasingly pronounced with approach to the glass transition. Recently, SHD has been observed in confined…

Soft Condensed Matter · Physics 2010-12-23 Aaron S. Keys , Adam R. Abate , Sharon C. Glotzer , Douglas J. Durian

We present simulations of stochastic fluid dynamics in the vicinity of a critical endpoint belonging to the universality class of the Ising model. This study is motivated by the challenge of modeling the dynamics of critical fluctuations…

Nuclear Theory · Physics 2024-07-23 Chandrodoy Chattopadhyay , Josh Ott , Thomas Schaefer , Vladimir V. Skokov

We study the dynamics of water confined between hydrophobic flat surfaces at low temperature. At different pressures, we observe different behaviors that we understand in terms of the hydrogen bonds dynamics. At high pressure, the formation…

Soft Condensed Matter · Physics 2015-05-13 Giancarlo Franzese , Francisco de los Santos

Recent studies of the phase diagram for spherical, purely repulsive, active particles established the existence of a transition from a liquid-like to a solid-like phase analogous to the one observed in colloidal systems at thermal…

Statistical Mechanics · Physics 2020-04-30 Lorenzo Caprini , Claudio Maggi , Umberto Marini Bettolo Marconi , Matteo Paoluzzi , Andrea Puglisi

Slow relaxation and plastic deformation in disordered materials such as metallic glasses and supercooled liquids occur at dynamical heterogeneities, or neighboring particles that rearrange in a correlated, cooperative manner. Dynamical…

Statistical Mechanics · Physics 2022-05-20 Charles K. C. Lieou , Takeshi Egami

We report a molecular dynamics simulation of a supercooled simple monatomic glass-forming liquid. It is found that the onset of the supercooled regime results in formation of distinct domains of slow diffusion which are confined to the…

Disordered Systems and Neural Networks · Physics 2009-11-07 Mikhail Dzugutov , Sergei I. Simdyankin , Fredrik H. M. Zetterling

The presence of dynamical heterogeneities, i.e. nanometer-scale regions containing molecules rearranging cooperatively at very different rates compared to the bulk, is increasingly being recognized as crucial in our understanding of the…

Disordered Systems and Neural Networks · Physics 2015-06-25 Horacio E. Castillo , Azita Parsaeian