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Based on first-principles electronic structure calculations, we analyze the chemical and magnetic mechanisms stabilizing the cubic phase in Fe$_2$-based Heusler materials, which were previously predicted to be tetragonal when being…

Materials Science · Physics 2013-08-08 Janos Kiss , Stanislav Chadov , Gerhard H. Fecher , Claudia Felser

Half-metallic ferromagnetism (HMFM) occurs rarely in materials and yet offers great potential for spintronic devices. Recent experiments suggest a class of compounds with the `ThCr$_{2}$Si$_{2}$' (122) structure -- isostructural and…

Materials Science · Physics 2020-08-18 Sinead M. Griffin , Jeffrey B. Neaton

We present a perspective on the status of antiferromagnetism in two-dimensional (2D) materials. Various types of spin-compensated orders are discussed and include non-collinear order, spin spirals and altermagnetism. Spin-orbit effects…

Materials Science · Physics 2024-08-09 Thomas Olsen

Heusler alloys were discovered in 1903, and materials with half-metallic characteristics have drawn more attention from researchers since the advances in semiconductor industry. Heusler alloys have found application as spin-filters, tunnel…

Materials Science · Physics 2025-07-22 Deep Patel

A concept is presented serving to guide in the search for new materials with high spin polarization. It is shown that the magnetic moment of half-metallic ferromagnets can be calculated from the generalized Slater-Pauling rule. Further, it…

Materials Science · Physics 2009-05-21 G. H. Fecher , H. C. Kandpal , S. Wurmehl , C. Felser , G. Schönhense

Low-dimensional magnetic materials with spin-$\frac{1}{2}$ moments can host a range of exotic magnetic phenomena due to the intrinsic importance of quantum fluctuations to their behavior. Here, we report the structure, magnetic structure…

Topological quantum materials represent a new class of matter with both exotic physical phenomena and novel application potentials. Many Heusler compounds, which exhibit rich emergent properties such as unusual magnetism, superconductivity…

Elastic constants and their derived properties of various cubic Heusler compounds were calculated using first-principles density functional theory. To begin with, Cu$_2$MnAl is used as a case study to explain the interpretation of the basic…

Materials Science · Physics 2020-09-03 Shu-Chun Wu , S. Shahab Naghavi , Gerhard H. Fecher , Claudia Felser

We performed magnetic susceptibility and neutron powder diffraction experiments on the ternary compound Pr5Ru3Al2. It belongs to the noncentrosymmetric and nonmirrorsymmetric cubic I213 space group. The previously reported ferromagnetic…

Strongly Correlated Electrons · Physics 2016-06-09 Koya Makino , Daisuke Okuyama , Maxim Avdeev , Taku J Sato

Heusler alloys are promising for several applications, including magnetic refrigeration, due to high magnetocaloric and magnetovolume effects. One way to optimize this potential is by increasing the magnetovolume effect. Using density…

Materials Science · Physics 2016-12-30 J. N. Gonçalves , J. S. Amaral , V. S. Amaral

Half-metallic ferromagnetic (HMF) materials show high spin polarization and are therefore interesting to researchers due to their possible applications in spintronic devices. In these materials, while one spin sub band has a finite density…

Materials Science · Physics 2016-08-11 Lakhan Bainsla , K. G. Suresh

The identification of materials supporting complex, tunable magnetic order at ambient temperatures is foundational to the development of new magnetic device architectures. We report the design of Mn2XY tetragonal inverse Heusler alloys that…

Materials Science · Physics 2021-09-24 Daniil A. Kitchaev , Anton Van der Ven

Conducting and magnetic properties of a material often change in some confined geometries. However, a situation where a non-magnetic semiconductor becomes both metallic and magnetic at the surface is quite rare, and to the best of our…

Strongly Correlated Electrons · Physics 2020-03-04 S. Keshavarz , I. Di Marco , D. Thonig , L. Chioncel , O. Eriksson , Y. O. Kvashnin

The ruthenium content of half-metallic Mn$_2$Ru$_x$Ga thin films, with a biaxially-strained inverse Heusler structure, controls the ferrimagnetism that determines their magnetic and electronic properties. An extensive study of…

Half-metallic Heusler alloys are among the most promising materials for future applications in spintronic devices. Although most Heusler alloys are ferromagnets, ferrimagnetic or antiferromagnetic (also called fully-compensated…

Materials Science · Physics 2015-05-13 I. Galanakis , K. Ozdogan , E. Sasioglu , B. Aktas

Quasiperiodic structures possess long range positional order, but are freed of constraints imposed by translational invariance. For spins interacting via Heisenberg couplings, one may expect therefore to find novel magnetic configurations…

Strongly Correlated Electrons · Physics 2008-10-15 Anuradha Jagannathan , Attila Szallas

Polycrystalline Heusler compounds Ni2Mn0.75Cu0.25Ga0.84Al0.16 with a martensitic transition between ferromagnetic phases and Ni2Mn0.70Cu0.30Ga0.84Al0.16 with a magnetostructural transformation were investigated by magnetization and thermal…

Materials Science · Physics 2021-04-28 Alberto A. Mendonca , Luis Ghivelder , Jesus F. Jurado , Angelo M. Gomes

A detailed investigation of the structural and magnetic properties, including magnetocaloric effect, re-entrant spin-glass behavior at low temperature, and critical behavior in polycrystalline Al$_2$MnFe Heusler alloy is reported. The…

We report crystal structure, electronic structure, and magnetism of manganese tetraboride, MnB4, synthesized under high-pressure high-temperature conditions. In contrast to superconducting FeB4 and metallic CrB4, which are both…

Ferromagnetic solids acquire nontrivial magnetic and caloric properties when the temperature of the structural phase transition approaches the Curie point. Deciphering magneto-structural transitions, i.e. determining their characteristic…

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