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We demonstrate an all-optical method for magnetic sensing of individual molecules in ambient conditions at room temperature. Our approach is based on shallow nitrogen-vacancy (NV) centers near the surface of a diamond crystal, which we use…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 A. O. Sushkov , N. Chisholm , I. Lovchinsky , M. Kubo , P. K. Lo , S. D. Bennett , D. Hunger , A. Akimov , R. L. Walsworth , H. Park , M. D. Lukin

Coherent control and optical readout of the electron spin of the $^{29}$SiV$^{-}$ center in diamond has been demonstrated in literature, with exciting prospects for implementations as memory nodes and spin qubits. Nuclear spins may be even…

Quantum Physics · Physics 2022-06-15 Hyma H. Vallabhapurapu , Chris Adambukulam , Andre Saraiva , Arne Laucht

Recently, rotation sensors utilizing the nuclear spins of nitrogen-vacancy color centers in diamond have been demonstrated. However, these devices are power-intensive and challenging to integrate into small chip-based radiofrequency…

We demonstrate fluorescence thermometry techniques with sensitivities approaching 10 mK Hz^(-1/2) based on the spin-dependent photoluminescence of nitrogen vacancy (NV) centers in diamond. These techniques use dynamical decoupling protocols…

Mesoscale and Nanoscale Physics · Physics 2013-05-24 David M. Toyli , Charles F. de las Casas , David J. Christle , Viatcheslav V. Dobrovitski , David D. Awschalom

We introduce an alternate route to dynamically polarize the nuclear spin host of nitrogen-vacancy (NV) centers in diamond. Our approach articulates optical, microwave and radio-frequency pulses to recursively transfer spin polarization from…

Quantum Physics · Physics 2014-12-18 Daniela Pagliero , Abdelghani Laraoui , Jacob D. Henshaw , Carlos A. Meriles

Understanding the profile of a qubit's wavefunction is key to its quantum applications. Unlike conducting systems, where a scanning tunneling microscope can be used to probe the electron distribution, there is no direct method for…

Monolithic integration, which refers to the incorporation of all device functionalities within a single material, shows significant potential for creating scalable solid-state quantum devices. This study demonstrated the coherent control of…

Hands-on experimental experience with quantum systems in the undergraduate physics curriculum provides students with a deeper understanding of quantum physics and equips them for the fast-growing quantum science industry. Here we present an…

The nitrogen vacancy (NV) center in diamond is a versatile color center used for magnetometry, quantum computing, and quantum communications. In this article, using a single laser beam as a pump and probe, we measure the spin states of the…

Applied Physics · Physics 2025-05-28 Reza Kashtiban , Gavin W. Morley , Mark E. Newton , A T M Anishur Rahman

There is a continuous search for solid-state spin qubits operating at room temperature with excitation in the IR communication bandwidth. Recently we have introduced the photoelectric detection of magnetic resonance (PDMR) to read the…

Materials Science · Physics 2018-06-20 E. Londero , E. Bourgeois , M. Nesladek , A. Gali

Fast quantum spin manipulation is needed to design spin-based quantum logic gates and other quantum applications. Here, we construct exact evolution operator of the nitrogen-vacancy-center (NV) spin in diamond under external magnetic fields…

Mesoscale and Nanoscale Physics · Physics 2017-08-25 Wen-Qi Fang , Bang-Gui Liu

Using a high quality factor 3 GHz bulk acoustic wave resonator device, we demonstrate the acoustically driven single quantum spin transition ($\left|m_{s}=0\right>\leftrightarrow\left|\pm1\right>$) for diamond NV centers and characterize…

Quantum Physics · Physics 2020-03-10 H. Y. Chen , S. A. Bhave , G. D. Fuchs

The electrical conductivity of a material can feature subtle, nontrivial, and spatially-varying signatures with critical insight into the material's underlying physics. Here we demonstrate a conductivity imaging technique based on the…

Mesoscale and Nanoscale Physics · Physics 2018-06-26 Amila Ariyaratne , Dolev Bluvstein , Bryan A. Myers , Ania C. Bleszynski Jayich

Hybrid quantum photonic systems connect classical photonics to the quantum world and promise to deliver efficient light-matter quantum interfaces while leveraging the advantages of both, the classical and the quantum, subsystems. However,…

Magnetic resonance techniques provide a powerful tool for controlling spin systems, with applications ranging from quantum information processing to medical imaging. Nevertheless, the behavior of a spin system under strong excitation…

Quantum Physics · Physics 2015-05-19 Lilian Childress , Jean McIntyre

The extension of the spin coherence times is a crucial issue for quantum information and quantum sensing. In solid state systems, suppressing noises with various techniques have been demonstrated. On the other hand, an electrical control…

Quantum Physics · Physics 2020-10-21 S. Kobayashi , Y. Matsuzaki , H. Morishita , S. Miwa , Y. Suzuki , M. Fujiwara , N. Mizuochi

As a potential candidate for quantum computation and metrology, the nitrogen vacancy (NV)center in diamond presented both challenges and opportunities resulted from charge state conversion. By utilizing different lasers for the…

Quantum Physics · Physics 2014-10-20 Xiangdong Chen , Changling Zou , Zhaojun Gong , Chunhua Dong , Guangcan Guo , Fangwen Sun

Spin defects in diamond serve as powerful building blocks for quantum technologies, especially for applications in quantum sensing and quantum networking. Electron-nuclear defects formed in the environment of optically active spins, such as…

Quantum Physics · Physics 2026-04-10 Alexander Ungar , Hao Tang , Andrew Stasiuk , Bo Xing , Boning Li , Ju Li , Alexandre Cooper , Paola Cappellaro

Charge control of color centers in semiconductors promises opportunities for novel forms of sensing and quantum information processing. Here, we articulate confocal fluorescence microscopy and magnetic resonance protocols to induce and…

We created dense ensembles of negatively charged nitrogen-vacancy (NV-) centers in diamond by neutron and electron irradiation for applications in hybrid quantum systems and magnetometry. We characterize fluorescence intensity, optical and…

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