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We present a robust quantum optimal control framework for implementing fast entangling gates on ion-trap quantum processors. The framework leverages tailored laser pulses to drive the multiple vibrational sidebands of the ions to create…
Quantum control of the pathway along which a Rydberg electron field ionizes is experimentally and computationally demonstrated. Selective field ionization is typically done with a slowly rising electric field pulse. The $(1/n^*)^4$ scaling…
Laser-produced plasma (LPP) induced during irradiation of a liquid tin droplet with diameter of 150 um and 180 um by CO2 laser pulse with various pulse durations and energies is considered. The two-dimensional radiative magnetohydrodynamic…
We have studied the formation of ultracold RbSr molecules with laser pulses. After discussing the advantages of the Mott insulator phase for the control with pulses, we present two classes of strategies. The first class involves two…
Well isolated quantum systems are exquisite sensors of electromagnetic fields. In this work, we use a single trapped ion for characterizing chirped ultraviolet (UV) picosecond laser pulses. The frequency swept pulses resonantly drive a…
The next generation of lithography machines uses extreme ultraviolet (EUV) light originating from laser-produced plasma (LPP) sources, where a small tin droplet is ionized by an intense laser pulse to emit the requested light at 13.5 nm.…
We demonstrate how the shape of femtosecond laser pulses can be tailored in order to obtain maximal ionization of atoms or molecules. For that purpose, we have overlayed a direct-optimization scheme on top of a fully unconstrained…
A model for THz generation by optical rectification using tilted-pulse-fronts is developed. It simultaneously accounts for (i) the spatio-temporal distortions of the optical pump pulse, (ii) the nonlinear coupled interaction of THz and…
We show how to create quantum gates of arbitrary speed between trapped ions, using a laser walking wave, with complete insensitivity to drift of the optical phase, and requiring cooling only to the Lamb-Dicke regime. We present pulse…
The laser-driven acceleration of high quality proton beams from a double-layer target, comprised of a high-Z ion layer and a thin disk of hydrogen, is investigated with three-dimensional particle-in-cell simulations in the case of oblique…
The ion acceleration driven by a laser pulse at intensity $I = 10^{20} - 10^{22} $W/cm$^2\times(\mu$m$/\lambda)^2$ from a double layer target is investigated with multi-parametric Particle-in-Cell (PIC) simulations. For targets with a wide…
We have investigated strong-field-induced electronic coherences in argon and molecular nitrogen ions created by high-intensity, few-cycle infrared laser pulses. This is a step toward the long-sought goal of strong-field coherent control in…
Laser cooling of molecules employing broadband optical pumping involves a timescale separation between laser excitation and spontaneous emission. Here, we optimize the optical pumping step using shaped laser pulses. We derive two…
A paradigm shift in the physics of laser-plasma interactions is approaching with the commissioning of multi-petawatt laser facilities world-wide. Radiation reaction processes will result in the onset of electron-positron pair cascades and,…
We propose a scheme to overcome the great challenge of polarization loss in spin-polarized ion acceleration. When a petawatt laser pulse penetrates through a compound plasma target consisting of a double layer slab and prepolarized hydrogen…
Forward and backward THz emission by ionizing two-color laser pulses in gas is investigated by means of a simple semi-analytical model based on Jefimenko's equation and rigorous Maxwell simulations in one and two dimensions. We find the…
Tunneling ionization followed by strong-field excitation leads to important ultrafast phenomena such as charge migration and lasing. Recent theoretical developments suggest that the population of the ionic excited state can be greatly…
Coherence among rotational ion channels during photoionization is exploited to control the anisotropy of the resulting photoelectron angular distributions at specific photoelectron energies. The strategy refers to a robust and single…
We present the characterization of ultrashort laser pulses by using the plasma-induced frequency resolved optical switching (PI-FROSt) technique, implemented in ambient air. This recently developed method allows for a temporal…
On the basis of optimal control theory, we numerically study how to optimally manipulate molecular vibrational dynamics by using cycle-averaged polarizability interactions induced by mildly intense non-resonant laser (NR) pulses. As the…