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A real-space formalism for density-functional perturbation theory (DFPT) is derived and applied for the computation of harmonic vibrational properties in molecules and solids. The practical implementation using numeric atom-centered…

Materials Science · Physics 2017-03-08 Honghui Shang , Christian Carbogno , Patrick Rinke , Matthias Scheffler

We performed ab initio lattice-dynamics calculations of frame-cluster dodecaborides ZrB12 and LuB12. As a whole, our calculated phonon frequencies and atom-projected density of states are consistent with the results of available…

Chemical Physics · Physics 2019-10-22 N. M. Chtchelkatchev , M. V. Magnitskaya , E. S. Clementyev , P. A. Alekseev

In order to test the Vibration-Transit (V-T) theory of liquid dynamics, ab initio density functional theory (DFT) calculations of thermodynamic properties of Na and Cu are performed and compared with experimental data. The calculations are…

The lattice dynamics of coesite has been studied by a combination of diffuse x-ray scattering, inelastic x-ray scattering and an ab initio lattice dynamics calculation. The combined technique gives access to the full lattice dynamics in…

Using first-principal density functional theory (DFT) we explained the importance of pseudopotential for decribing the electronic and vibrational properties of rutile TiO2 (R-TiO2). Calculations were performed using the generalized gradient…

Chemical Physics · Physics 2018-11-12 Sugata Chowdhury , Nacole King , Winnie Wong-Ng

We present a comprehensive computational study on the properties of face-centered cubic and hexagonal chalcogenide Ge2Sb2Te5. We calculate the electronic structure using density functional theory (DFT); the obtained density of states (DOS)…

Materials Science · Physics 2015-03-17 Thierry Tsafack , Enrico Piccinini , Bong-Sub Lee , Eric Pop , Massimo Rudan

The structural, dynamical, and thermodynamical properties of diamond, graphite and layered derivatives (graphene, rhombohedral graphite) are computed using a combination of density-functional theory (DFT) total-energy calculations and…

Materials Science · Physics 2009-11-10 Nicolas Mounet , Nicola Marzari

Using first-principles electronic structure calculations based on the Nth order muffin tin orbital (NMTO)-downfolding technique, we derived the low-energy spin model for CuTe2O5. Our study reveals that this compound is a 2D coupled…

Materials Science · Physics 2009-11-13 Hena Das , T. Saha-Dasgupta , Claudius Gros , Roser Valenti

Finite-temperature effects can be included by calculating the vibrations properties and this can greatly improve the fidelity of computational screening. An important challenge for DFT-based screening is the sensitivity of the predictions…

Materials Science · Physics 2020-07-07 Pinwen Guan , Gregory Houchins , Venkatasubramanian Viswanathan

Magnetic 2D materials have achieved significantly consideration owing to their encouraging applications. A variation of these 2D materials by occurrence of defects, by the transition-metal doping or adsorption or by the surface…

Materials Science · Physics 2025-06-27 Zarah Khan , Saleem Ayaz Khan , Ayesha Zaheer , Syed Rizwan

Structural stability and vibrational properties of KN$_3$ have been studied under pressure using the first principles calculations based on the density functional theory (DFT) as well as with semi empirical dispersion correction to the DFT…

Materials Science · Physics 2013-11-08 K. Ramesh Babu , G. Vaitheeswaran

The thermodynamic and physical properties of the Laves phase Fe2Mo have been investigated using the finite-temperature quantum mechanical calculations within the frame of the density functional theory (DFT). All relevant free energy…

Materials Science · Physics 2022-07-04 Dmitry Vasilyev

High-resolution synchrotron x-ray diffraction measurements were performed on single crystalline and powder samples of BiMn2O5. A linear temperature dependence of the unit cell volume was found between T_{N}=38$ K and 100 K, suggesting that…

Materials Science · Physics 2009-11-13 E. Granado , M. S. Eleoterio , A. F. Garcia-Flores , J. A. Souza , E. I. Golovenchits , V. A. Sanina

Transition metal penta-tellurides, ZrTe5 and HfTe5 have been recently drawn a lot of attention due to their fascinating physical properties and for being prominent materials showing topological phase transitions. In this study, we…

Materials Science · Physics 2025-04-24 Syed Shovon Mahbub Mahin , Suptajoy Barua , B. Rahman Rano , Ishtiaque M. Syed , S. H. Naqib

Within the framework of density functional theory (DFT), the total energy of crystal structures is calculated at zero temperature. Herein, we briefly discuss the DFT-based lattice-dynamics approach for computing crystal free energy, the…

Materials Science · Physics 2015-07-01 Tran Doan Huan

Plane-wave pseudopotential methods and density functional perturbation theory are used to calculate the phonon density of states and thermodynamic functions of h-P4O10. The calculated vibrational spectrum is in good agreement with the…

Materials Science · Physics 2011-06-30 James R. Rustad

Through first-principles calculation based on the density functional theory (DFT) within the pseudo potential-plane wave (PP-PW) approach, we studied the structural, mechanical and thermal properties of Cu$_2$CdSnSe$_4$ and Cu$_2$HgSnSe$_4$…

Materials Science · Physics 2017-02-13 S. Bensalem , M. Chegaar , A. Bouhemadou

Experimental investigation as well as theoretical calculations, of the Fe-partial phonon density-of-states (DOS) for nominally Fe_52.5Cr_47.5 alloy having (a) alpha- and (b) sigma-phase structure were carried out. The former at sector 3-ID…

Materials Science · Physics 2015-05-14 S. M. Dubiel , J. Cieslak , W. Sturhahn , M. Sternik , P. Piekarz , S. Stankov , K. Parlinski

High-valence actinide oxides are critical to understanding the behavior of 5f-electrons, yet their structural and electronic properties remain poorly understood due to challenges in synthesis and handling. We report the first Raman…

Density functional theory (DFT) provides a theoretical framework for efficient and fairly accurate calculations of the electronic structure of molecules and crystals. The main features of density functional theory are described and DFT…

Chemical Physics · Physics 2012-06-12 Hauke Paulsen , Alfred Xaver Trautwein
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