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We model polydomain liquid-crystal elastomers by extending the neo-classical soft and semi-soft free energies used successfully to describe monodomain samples. We show that there is a significant difference between polydomains cross-linked…

Soft Condensed Matter · Physics 2014-07-09 J. S. Biggins , M. Warner , K. Bhattacharya

We present a detailed analysis of the molecular packing of a strained liquid crystal elastomer composed of chiral mesogens in the smectic A phase. X-ray diffraction patterns of the elastomer collected over a range of orientations with…

Semiflexible polymers in concentrated lyotropic solution are studied within a bead-spring model by molecular dynamics simulations, focusing on the emergence of a smectic A phase and its properties. We systematically vary the density of the…

Soft Condensed Matter · Physics 2019-01-28 Andrey Milchev , Arash Nikoubashman , Kurt Binder

We present a numerical study of stretching monodomain smectic-A elastomer sheets, computed using the finite element method. When stretched parallel to the layer normal the microscopic layers in smectic elastomers are unstable to a…

Soft Condensed Matter · Physics 2013-08-06 Andrew W. Brown , James M. Adams

Randomly disordered (polydomain) liquid crystalline elastomers align under stress. We study the dynamics of stress relaxation before, during and after the Polydomain-Monodomain transition. The results for different materials show the…

Soft Condensed Matter · Physics 2016-08-31 S. M. Clarke , E. M. Terentjev

Liquid crystal elastomers are cross-linked polymer networks covalently bonded with liquid crystal mesogens. In the nematic phase, due to strong coupling between mechanical strain and orientational order, these materials display…

Soft Condensed Matter · Physics 2011-11-04 Badel L. Mbanga , Fangfu Ye , Jonathan V. Selinger , Robin L. B. Selinger

Liquid crystals (LCs) composed of mesogens play important roles in various scientific and engineering problems. How a system with many mesogens can enter a LC state is an interesting and important problem. Using stiff and free-joint…

Models of smectic-C liquid crystal elastomers predict that it can display soft elasticity, in which the shape of the elastomer changes at no energy cost. The amplitude of the soft mode and the accompanying shears are dependent on the…

Soft Condensed Matter · Physics 2012-01-16 A. W. Brown , J. M. Adams

We model within the framework of finite elasticity two inherent instabilities observed in liquid crystal elastomers under uniaxial tension. First is necking which occurs when a material sample suddenly elongates more in a small region where…

Soft Condensed Matter · Physics 2024-10-15 Rabin Poudel , Yasemin Sengul , L. Angela Mihai

Modeling liquid crystal elastomers (LCEs) at the molecular level is crucial for the predictable design of energy-conversion and stimuli-responsive materials. Here, we develop a self-consistent field theory for LCEs which captures the…

Soft Condensed Matter · Physics 2023-10-05 Luofu Liu , Rui Wang

Experimental and modeling/simulation studies of phase equilibrium and growth morphologies of novel polymer-dispersed liquid crystal (PDLC) mixtures of PS (polystyrene) and liquid crystals that exhibit a direct isotropic/smectic-A (lamellar)…

Soft Condensed Matter · Physics 2015-05-13 Ezequiel R. Soule , Nasser Mohieddin Abukhdeir , Alejandro D. Rey

Atomistic deformation simulations in the nominally elastic regime are performed for a model binary glass with strain rates as low as $10^{4}$/sec (corresponding to 0.01 shear strain per 1$\mu$sec). A robust elasticity is revealed that…

Soft Condensed Matter · Physics 2020-11-21 P. M. Derlet , R. Maass

Liquid crystal elastomers are cross-linked elastomer networks with liquid crystal mesogens incorporated into the main or side chain. Polydomain liquid crystalline (nematic) elastomers exhibit unusual mechanical properties like soft…

Soft Condensed Matter · Physics 2024-05-21 Ameneh Maghsoodi , Kaushik Bhattacharya

We present a model for smectic elastomer membranes which includes elastic and liquid crystalline degrees of freedom. Based on our model, we determined the qualitative phase diagram of a smectic elastomer membrane using mean-field theory.…

Soft Condensed Matter · Physics 2009-11-13 Olaf Stenull

We study two aspects of the elasticity of smectic-$A$ elastomers that make these materials genuinely and qualitatively different from conventional uniaxial rubbers. Under strain applied parallel to the layer normal, monodomain smectic-$A$…

Soft Condensed Matter · Physics 2009-11-13 Olaf Stenull , T. C. Lubensky

Spherical colloidal crystals (CCs) self-assemble on the interface between two liquids. These 2D structures unconventionally combine local hexagonal order and spherical geometry. Nowadays CCs are actively studied by altering their…

Soft Condensed Matter · Physics 2015-10-28 D. S. Roshal , A. E. Myasnikova , S. B. Rochal

Liquid crystal elastomers (LCEs) are elastomeric networks with rod-like mesogens that reorient under load. In polydomain LCEs, this reorientation drives a polydomain-to-monodomain transition that produces a soft-elastic plateau. Coupling…

Soft Condensed Matter · Physics 2026-05-13 Zhengxuan Wei , Beijun Shen , Zumrat Usmanova , Umme Hani Bootwala , Ruobing Bai

Smectic liquid crystals are charcterized by layers that have a preferred uniform spacing and vanishing curvature in their ground state. Dislocations in the smectics play an important role in phase nucleation, layer reorientation, and…

Soft Condensed Matter · Physics 2017-06-28 Hillel Aharoni , Thomas Machon , Randall D. Kamien

The yet virtually unexplored class of soft colloidal rods with small aspect ratio is investigated and shown to exhibit a very rich phase and dynamic behavior, spanning from liquid to nearly melt state. Instead of nematic order, these short…

Polydomain liquid crystalline (nematic) elastomers have highly unusual mechanical properties, dominated by the dramatically non-linear stress-strain response that reflects stress-induced evolution of domain patterns. Here, we study the…

Soft Condensed Matter · Physics 2023-05-02 Ameneh Maghsoodi , Mohand O. Saed , Eugene M. Terentjev , Kaushik Bhattacharya
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