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In this work, we have systematically studied the role of point defects in the recombination time of monolayer MoS$_2$ using time-dependent ab initio non-adiabatic molecular dynamics simulations. Various types of point defects, such as S…

Materials Science · Physics 2021-07-07 Raquel Esteban-Puyuelo , Biplab Sanyal

Auger recombination in semiconductors is a many-body phenomenon in which recombination of electrons and holes is accompanied by excitation of other charge carriers. Being nonradiative, it is detrimental to light emission. The excess energy…

Strong Coulomb interactions in two-dimensional systems, together with quantum confinement, make many-body processes particularly effective for carrier dynamics, which plays a crucial role in determining carrier lifetime, photoconductivity,…

Mesoscale and Nanoscale Physics · Physics 2022-02-01 Di Li , Wenjie Zhang , Peng Suo , Jiaming Chen , Kaiwen Sun , Yuqin Zou , Hong Ma , Xian Lin , Xiaona Yan , Saifeng Zhang , Bo Li , Guohong Ma

We report results from ultrafast two-color optical pump-probe spectroscopy on bulk $\beta$-Ga$_2$O$_3$. A two-photon absorption scheme is used to photoexcite carriers with the pump pulse and free-carrier absorption of the probe pulse is…

Materials Science · Physics 2019-01-30 Okan Koksal , Nicholas Tanen , Debdeep Jena , Huili Xing , Farhan Rana

We present results on photoexcited carrier lifetimes in few-layer transition metal dichalcogenide MoS2 using nondegenerate ultrafast optical pump-probe technique. Our results show a sharp increase of the carrier lifetimes with the number of…

Mesoscale and Nanoscale Physics · Physics 2016-01-20 Haining Wang , Changjian Zhang , Farhan Rana

Recent photoluminescence experiments presented by M. Binder et al. [Appl. Phys. Lett. 103, 071108 (2013)] demonstrated the visualization of high-energy carriers generated by Auger recombination in (AlInGa)N multi quantum wells. Two…

In quantum dots (QDs) the Auger recombination is a non-radiative process, where the electron-hole recombination energy is transferred to an additional carrier. It has been studied mostly in colloidal QDs, where the Auger recombination time…

Mesoscale and Nanoscale Physics · Physics 2019-07-03 Annika Kurzmann , Arne Ludwig , Andreas D. Wieck , Axel Lorke , Martin Geller

The strong Coulomb interactions and the small exciton radii in two-dimensional metal dichalcogenides can result in very fast capture of electrons and holes of excitons by mid-gap defects from Auger processes. In the Auger processes…

Mesoscale and Nanoscale Physics · Physics 2015-04-22 Haining Wang , Jared H. Strait , Changjian Zhang , Weimin Chan , Christina Manolatou , Sandip Tiwari , Farhan Rana

Van der Waals (vdW) heterostructures constructed with two-dimensional (2D) materials have attracted great interests, due to their fascinating properties and potential for novel applications. While earlier efforts have advanced the…

Mesoscale and Nanoscale Physics · Physics 2018-11-13 Zhonghui Nie , Yuhan Wang , Ziling Li , Yue Sun , Xiaoping Liu , Edmond Turcu , Yi Shi , Rong Zhang , Yu Ye , Yongbing Xu , Fengqiu Wang

Auger recombination is a non-radiative process, where the recombination energy of an electron-hole pair is transferred to a third charge carrier. It is a common effect in colloidal quantum dots that quenches the radiative emission with an…

Mesoscale and Nanoscale Physics · Physics 2020-04-22 Pia Lochner , Annika Kurzmann , Jens Kerski , Philipp Stegmann , Jürgen König , Andreas D. Wieck , Arne Ludwig , Axel Lorke , Martin Geller

Auger processes play a critical role in the behavior of colloidal quantum dots (QDs). While nonradiative Auger recombination is a key performance-limiting factor in light-emitting applications, Auger effects also present exciting…

Mesoscale and Nanoscale Physics · Physics 2025-04-29 Valerio Pinchetti , Ho Jin , Clément Livache , Victor I. Klimov

The Auger recombination in bulk semiconductors can depopulate the charge carriers in a non-radiative way, which, fortunately, only has detrimental impact on optoelectronic device performance under the condition of high carrier density…

Chemical Physics · Physics 2020-02-07 Hongyan Liao , Yunyan Fan , Yumei Lin , Kang Wang , Renfu Li , Xueyuan Chen , Kelvin H. L. Zhang , Ye Yang

In a semiconductor heterostructure with type II energy band alignment, the spatial separation between electrons and holes slows down their radiative recombination. With increasing excitation intensity, Auger recombination quickly becomes…

Materials Science · Physics 2008-09-09 E. -K. Lee , D. J. Lockwood , J. -M. Baribeau , A. M. Bratkovsky , T. I. Kamins , L. Tsybeskov

The principal mechanisms of Auger recombination of nonequilibrium carriers in semiconductor heterostructures with quantum wells are investigated. It is shown for the first time that there exist three fundamentally different Auger…

Materials Science · Physics 2009-10-31 Anatoli S. Polkovnikov , Georgy G. Zegrya

Auger scattering channels are of fundamental importance to describe and understand the non-equilibrium charge carrier dynamics in graphene. While impact excitation increases the number of carriers in the conduction band and has been…

We propose a novel phonon assisted Auger process unique to the electronic band structure of monolayer transition metal dichalcogenides (TMDCs), which dominates the radiative recombination of ground state excitons in Tungsten based TMDCs.…

Mesoscale and Nanoscale Physics · Physics 2016-09-12 Mark Danovich , Viktor Zólyomi , Igor L. Aleiner , Vladimir I. Fal'ko

Ultrafast optical pump-probe spectroscopy is used to track carrier dynamics in the large magnetoresistance material WTe$_{2}$. Our experiments reveal a fast relaxation process occurring on a sub-picosecond time scale that is caused by…

The ultrafast relaxation and recombination dynamics of photogenerated electrons and holes in epitaxial graphene are studied using optical-pump Terahertz-probe spectroscopy. The conductivity in graphene at Terahertz frequencies depends on…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Paul A. George , Jared Strait , Jahan Dawlaty , Shriram Shivaraman , Mvs Chandrashekhar , Farhan Rana , Michael G. Spencer

The intriguing physics of carrier-carrier interactions, which likewise affect the operation of light emitting devices, stimulate the research on semiconductor structures at high densities of excited carriers, a limit reachable at large…

Spectroscopic studies of semiconductor quantum dots (SQDs) addressing the problem of non-radiative carrier losses is vital for the improvement in the efficiency of various light-emitting devices. Various designs of SQDs emitter like doping,…

Mesoscale and Nanoscale Physics · Physics 2020-08-07 Sabina Gurung , Asha Singh , J. Jayabalan
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