Related papers: Complete quantum state selectivity in cold molecul…
Ultrafast electron diffraction and time-resolved serial crystallography are the basis of the ongoing revolution in capturing at the atomic level of detail the structural dynamics of molecules. However, most experiments employ the classical…
We make use of an inhomogeneous electrostatic dipole field to impart a quantum-state-dependent deflection to a pulsed beam of OCS molecules, and show that those molecules residing in the absolute ground state, $X ^1\Sigma^+$, $\ket{00^00}$,…
Inspired by a recent experiment [Phys. Rev. Letts. \textbf{122}, 253201(2019)] that an unprecedented quantum interference was observed in the way of Stimulated Raman adiabatic passage (STIRAP) due to the coexisting resonant- and…
Using the technique of stimulated Raman adiabatic passage (STIRAP) we have coherently transferred ultracold 87Rb2 Feshbach molecules into a more deeply bound vibrational quantum level. Our measurements indicate a high transfer efficiency of…
Control strategies for dissipative preparation of target quantum states, both pure and mixed, and subspaces are obtained by switching between a set of available semigroup generators. We show that the class of problems of interest can be…
We report the creation of ultracold ground state $^{6}\textrm{Li}^{40}\textrm{K}$ polar molecules with high efficiency. Starting from weakly-bound molecules state, stimulated Raman adiabatic passage (STIRAP) is adopted to coherently…
We devise an autonomous quantum thermal machine consisting of three pairwise-interacting qubits, two of which are locally coupled to thermal reservoirs. The machine operates autonomously, as it requires no time-coherent control, external…
We study dynamics of a two-color photoassociation of atoms into diatomic molecules via nonlinear Stimulated Raman adiabatic passage (STIRAP) process. This system has a famous counterpart in (linear) quantum mechanics, and been discussed…
Quantum control of reactive systems has enabled microscopic probes of underlying interaction potentials, the opening of novel reaction pathways, and the alteration of reaction rates using quantum statistics. However, extending such control…
STImulated Raman Adiabatic Passage (STIRAP) is a powerful technique for robust state transfer capabilities in quantum systems. This method, however encounters challenges for its implementation as a gate in qubit-subspace due to its…
Stimulated Raman adiabatic passage (STIRAP) is a standard technique to combat experimental imperfections and can be used to realize robust quantum state control, which has many applications in physics, chemistry, and beyond. However, STIRAP…
We discuss the use of electromagnetically modified absorption to achieve selective excitation in atoms: that is, the laser excitation of one transition while avoiding simultaneously exciting another transition whose frequency is the same as…
This work addresses a fundamental problem of controllability of open quantum systems, meaning the ability to steer arbitrary initial system density matrix into any final density matrix. We show that under certain general conditions open…
We describe how stimulated Raman adiabatic passage (STIRAP) can be applied to create spectral holes in an inhomogeneously broadened system. Due to the robustness of STIRAP, our proposal guarantees high flexibility and accuracy and, at…
We propose a general scheme for dissipatively preparing arbitrary pure quantum states on a multipartite qubit register in a finite number of basic control blocks. Our "splitting-subspace" approach relies on control resources that are…
Dark states are eigenstates or steady-states of a system that are decoupled from the radiation. Their use, along with associated techniques such as Stimulated Raman Adiabatic Passage, has extended from atomic physics where it is an…
Quantum optomechanical STIRAP (Stimulated Raman Adiabatic Passage) is investigated for a system of two mechanical modes coupled to an optical mode. We show analytically that in a system without loss, fractional STIRAP can generate a…
We propose an experimentally accessible procedure for conditional preparation of highly non-classical states of collective spin of an atomic ensemble. The quantum state engineering is based on a combination of QND interaction between atoms…
We present an X-ray based stimulated Raman approach to control the preparation of optically dark electronic states in generic molecular systems. Leveraging on the unique properties of core-level excited states, we demonstrate that optically…
Stimulated Raman adiabatic passage (STIRAP) is a widely-used technique of coherent state-to-state manipulation for many applications in physics, chemistry, and beyond. The adiabatic evolution of the state involved in STIRAP, called…