Related papers: Quantum spin coherence in halogen-modified Cr$_7$N…
Quantum coherence control usually requires extremely low temperature environments. Even for spins in diamond, a remarkable exception, the coherence signal is lost as temperature approaches 700 K. Here we demonstrate quantum coherence…
This mini-review presents a simple and accessible summary on the fascinating physics of quantum nanomagnets coupled to a nuclear spin bath. These chemically synthesized systems are an ideal test ground for the theories of decoherence in…
Molecular nanomagnets show clear signatures of coherent behavior and have a wide variety of effective low-energy spin Hamiltonians suitable for encoding qubits and implementing spin-based quantum information processing. At the nanoscale,…
The substitution of one metal ion in a Cr-based molecular ring with dominant antiferromagnetic couplings allows to engineer its level structure and ground-state degeneracy. Here we characterize a Cr7Ni molecular ring by means of…
We theoretically investigate the influence of the fluctuating Overhauser field on the spin of an electron confined to a quantum dot (QD). The fluctuations arise from nuclear angular momentum being exchanged between different nuclei via the…
The main part of this review is devoted to the comprehensive description of coherent radiation by nuclear spins. The theory of nuclear spin superradiance is developed and the experimental observations of this phenomenon are considered. The…
The ability to design quantum systems that decouple from environmental noise sources is highly desirable for development of quantum technologies with optimal coherence. The chemical tunability of electronic states in magnetic molecules…
The assemblies of either quantum dots or magnetic nanoclusters are studied. It is shown that such assemblies can produce coherent radiation. A method is developed for solving the systems of nonlinear equations describing the dynamics of…
We examine the coherence/incoherence transition temperature of a generic molecular spin. Our results demonstrates that a molecular spin with a high coherence/incoherence transition temperature should possess a low spin number and low…
We theoretically study the decoherence and the dynamical decoupling control of nitrogen-vacancy center electron spins in high-purity diamond, where the hyperfine interaction with $^{13}$C nuclear spins is the dominating decoherence…
Direct evidence of quantum coherence in a single-molecule magnet in frozen solution is reported with coherence times as long as T2 = 630 ns. We can strongly increase the coherence time by modifying the matrix in which the single-molecule…
The strong influence of nuclear spins on resonant quantum tunneling in the molecular cluster Fe_8 is demonstrated for the first time by comparing the relaxation rate of the standard Fe_8 sample with two isotopic modified samples: (i) 56_Fe…
The dynamics of non-polar diatomic molecules interacting with a far-detuned narrow-band laser field, that only may drive rotational transitions, is studied. The rotation of the molecule is considered both classically and quantum…
Numerical modelling of coherent spin relaxation in nanomagnets, formed by magnetic molecules of high spins, is accomplished. Such a coherent spin dynamics can be realized in the presence of a resonant electric circuit coupled to the magnet.…
Decoherence in many solid-state systems is anomalously high, frustrating efforts to make solid-state qubits. We show that in nanomagnetic insulators in large transverse fields, there can be a fairly narrow field region in which both phonon…
Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…
We review recent theoretical results for hole spins influenced by spin-orbit coupling and Coulomb interaction in two-dimensional quantum wells as well as the decoherence of single hole spins in quantum dots due to hyperfine interaction with…
We present a quantum solution to the electron spin decoherence by a nuclear pair-correlation method for the electron-nuclear spin dynamics under a strong magnetic field and a temperature high for the nuclear spins but low for the electron.…
A theoretical model of nuclear spin conversion in molecules controlled by an external electromagnetic radiation resonant to rotational transition has been developed. It has been shown that one can produce an enrichment of spin isomers and…
The spin coherence phenomena and the possibility of their observation in nanomagnetic insulators attract more and more attention in the last several years. Recently it has been shown that in these systems in large transverse magnetic field…