Related papers: Selective Vibrational Population Transfer using Co…
We report the creation of ultracold ground state $^{6}\textrm{Li}^{40}\textrm{K}$ polar molecules with high efficiency. Starting from weakly-bound molecules state, stimulated Raman adiabatic passage (STIRAP) is adopted to coherently…
The rapid experimental progress in the field of superconducting nanocircuits gives rise to an increasing quest for advanced quantum-control techniques for these macroscopically coherent systems. Here we demonstrate theoretically that…
The influence of excited-state absorption (ESA) and two-exciton processes on a coherent population transfer with intense ultrashort chirped pulses in molecular systems in solution has been studied. An unified treatment of adiabatic rapid…
We propose a multilevel scheme to coherently transfer the population of a diatomic molecule from a rovibrational level to a target rovibrational level of the same electronic state or another. It involves a linear chain of N rovibrational…
The efficient transfer of excitations between different levels of a quantum system is a task with many applications. Among the various protocols to carry out such a state transfer in driven systems, rapid adiabatic passage (RAP) is one of…
An automated and robust method for adiabatic population transfer and the preparation of an arbitrary quantum superposition state in atomic system using the oscillating dark states (ODS) is presented. Quantum state of a three-level $\Lambda$…
We report on an experimental investigation of rapid adiabatic passage (RAP) in a trapped barium ion system. RAP is implemented on the transition from the $6S_{1/2}$ ground state to the metastable $5D_{5/2}$ level by applying a laser at 1.76…
In this paper, we investigate coherent control of nonadiabatic dynamics at a conical intersection (CI) using engineered ultrafast laser pulses. Within a model vibronic system, we tailor pulse chirp and temporal profile and compute the…
In this work we investigate the theory for three different uni-directional population transfer schemes in trapped multilevel systems which can be utilized to cool molecular ions. The approach we use exploits the laser-induced coupling…
We examine the stability of population transfer in two- and three-level systems against unwanted additional transitions. This population inversion is achieved by using recently proposed schemes called "shortcuts to adiabaticity". We…
Population transfer between low lying Rydberg states independent of the initial state is realized using a train of half-cycle pulses with pulse durations much less than the classical orbit period. We demonstrate experimentally the transfer…
Many experimental platforms for quantum science depend on state control via laser fields. Frequently, however, the control fidelity is limited by optical phase noise. This is exacerbated in stabilized laser systems where high-frequency…
Using the technique of stimulated Raman adiabatic passage (STIRAP) we have coherently transferred ultracold 87Rb2 Feshbach molecules into a more deeply bound vibrational quantum level. Our measurements indicate a high transfer efficiency of…
We study the population transfer between resonance states for a time-dependent loop around exceptional points in spectra of the hydrogen atom in parallel electric and magnetic fields. Exceptional points are well-suited for population…
We study quantum control techniques, specifically Adiabatic Rapid Passage (ARP) and Gradient Ascent Pulse Engineering (GRAPE), for transferring atoms trapped in an optical lattice between different vibrational states. We compare them with…
The space-time method is applied to a model system-the Simple Harmonic Oscillator in a laser field to simulate the Stimulated Raman Adiabatic Passage (STIRAP) process. The Space-Time method is a computational theory first introduced by…
An interesting method of fast enantio-specific state transfer is proposed for cyclic three-level systems of chiral molecules. We show that the fast population transfer via shortcut to adiabaticity can be accomplished for the cyclic…
We present a new method, called SISYPHUS (Stochastic Iterations to Strengthen Yield of Path Hopping over Upper States), for extending accessible time-scales in atomistic simulations. The method proceeds by separating phase space into…
A two level system is considered which has no static dipole moment, e.g. molecule $H_2$ in its ground electronic state. If strong enough external field is applied, it will dynamically distort such a system and supply it with time (and…
We study the population trapping extensively in a periodically driven Rydberg pair. The periodic modulation of the atom-light detuning effectively suppresses the Rabi couplings and, together with Rydberg-Rydberg interactions, leads to the…