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We present a rigorous theoretical description of excitonic dynamics in molecular light-harvesting aggregates photoexcited by weak-intensity radiation of arbitrary properties. While the interaction with light is included up to the second…

Chemical Physics · Physics 2021-01-01 Veljko Janković , Tomáš Mančal

We show that coherence between two excited ro-vibrational states belonging to the same molecular electronic configuration arises quite naturally due to their interaction with electromagnetic vacuum. For initial preparation of a molecule in…

Atomic Physics · Physics 2012-01-12 Sumanta Das , Arpita Rakshit , Bimalendu Deb

We investigate, theoretically and numerically, the spin dynamics of a two-component exciton-polariton condensate created and sustained by non-resonant spin-polarized optical pumping of a semiconductor microcavity. Using the open-dissipative…

Quantum Gases · Physics 2015-08-26 G. Li , T. C. H. Liew , O. A. Egorov , E. A. Ostrovskaya

Inertial modes have been observed on the Sun at low longitudinal wavenumbers. These modes probe the dynamics and structure of the solar convection zone down to the tachocline. While linear analysis allows the complex eigenfrequencies and…

Solar and Stellar Astrophysics · Physics 2023-05-31 J. Philidet , L. Gizon

Ultrafast laser pulse has provided a systematic way to inspect the dynamics of electrons in condensed matter systems. In this paper, by means of time-dependent density matrix renormalization group, we study an ultrafast laser driven Kondo…

Strongly Correlated Electrons · Physics 2021-06-23 W. Zhu , Benedikt Fauseweh , Alexis Chacon , Jian-Xin Zhu

In the primary step of light-harvesting, the energy of a photon is captured in antenna chlorophyll as an exciton. Its efficient conversion to stored chemical potential occurs in the special pair reaction center, which has to be reached by…

We present a fully quantum-mechanical model of the electronic dynamics of primary photoexcitations in a polymeric semiconductor heterojunction, which includes both polymer stacking and phonon relaxation. By examining the phonon-induced…

Materials Science · Physics 2014-03-05 Eric R. Bittner , Carlos Silva

Semiconductor microcavities with artificial single-photon emitters have become one of the backbones of semiconductor quantum optics. In many cases however, technical and physical issues limit the study of optical fields to incoherently…

Quantum Physics · Physics 2015-12-01 L. Teuber , P. Grünwald , W. Vogel

Solid systems with strong correlations and interactions under light illumination have the potential for exhibiting interesting bulk photovoltaic behavior in the non-perturbative regime, which has remained largely unexplored in the past…

Strongly Correlated Electrons · Physics 2022-04-06 Sangeeta Rajpurohit , C. Das Pemmaraju , Tadashi Ogitsu , Liang Z Tan

Phenomena involving electron transfer are ubiquitous in nature, photosynthesis and enzymes or protein activity being prominent examples. Their deep understanding thus represents a mandatory scientific goal. Moreover, controlling the…

Chemical Physics · Physics 2017-12-01 Carlo Andrea Rozzi , Filippo Troiani , Ivano Tavernelli

We present closed-form analytic solutions to non-secular Bloch-Redfield master equations for quantum dynamics of a V-type system driven by weak coupling to a thermal bath. We focus on noise-induced Fano coherences among the excited states…

Chemical Physics · Physics 2016-07-27 Amro Dodin , Timur V. Tscherbul , Paul Brumer

Coherent scattering of light by a single quantum emitter is a fundamental process at the heart of many proposed quantum technologies. Unlike atomic systems, solid-state emitters couple to their host lattice by phonons. Using a quantum dot…

Exposing a molecule to intense light pulses may bring this molecule to a nonstationary quantum state, thus launching correlated dynamics of electronic and nuclear subsystems. Although much had been achieved in the understanding of…

Chemical Physics · Physics 2024-04-11 Nikolay V. Golubev , Jiří Vaníček

Excitons are key quasiparticles determining the optical properties of solids. As such, they can be utilized to coherently control the electronic structure of materials using optical femtosecond pulses. Identifying the decoherence mechanism…

We demonstrate that the coupling of excitonic and vibrational motion in biological complexes can provide mechanisms to explain the long-lived oscillations that have been obtained in non linear spectroscopic signals of different…

Chemical Physics · Physics 2015-06-17 M. B. Plenio , J. Almeida , S. F. Huelga

Examining phototactic bioconvection in non-scattering suspensions with upper heating and collimated irradiation, this study delves into the intricate dynamics influenced by light and microorganisms. The study focuses on the linear stability…

Dynamical Systems · Mathematics 2024-03-13 Sandeep Kumar , Shaowei Wang

Many microorganisms, with phytoplankton and zooplankton as prominent examples, display phototactic behaviour, that is, the ability to perform directed motion within a light gradient. Here we experimentally demonstrate that sensing of light…

Soft Condensed Matter · Physics 2016-10-03 Celia Lozano , Borge ten Hagen , Hartmut Löwen , Clemens Bechinger

The rotational dynamics of particles subject to external illumination is found to produce light amplification and inelastic scattering at high rotation velocities. Light emission at frequencies shifted with respect to the incident light by…

Quantum Physics · Physics 2015-05-28 Ana Asenjo-Garcia , Alejandro Manjavacas , F. Javier García de Abajo

Bose-Einstein condensate of exciton polaritons in a semiconductor microcavity is a macroscopically populated coherent quantum state subject to concurrent pumping and decay. Debates about the fundamental nature of the condensed phase in this…

We examine the photoconductivity of an intrinsic graphene associated with far- and mid-infrared irradiation at low temperatures. The model under consideration accounts for the excitation of the electron-hole pairs by incident radiation, the…

Materials Science · Physics 2008-05-27 F. T. Vasko V. Ryzhii