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In a circular channel passing over-limiting current (faster than diffusion), transient vortices of bulk electroconvection are observed in salt-depleted region within the horizontal plane. The spatiotemporal evolution of the salt…

Fluid Dynamics · Physics 2020-08-25 Zhibo Gu , Bingrui Xu , Peng Huo , Shmuel M. Rubinstein , Martin Z. Bazant , Daosheng Deng

We present an analytical model of salt- and water-ion transport across an ion-selective interface based on an assumption of local equilibrium of the water-dissociation reaction. The model yields current-voltage characteristics and curves of…

Fluid Dynamics · Physics 2014-04-18 Christoffer P. Nielsen , Henrik Bruus

We revisit the classical problem of diffusion-limited ion transport to a membrane (or electrode) by considering the effects of charged side walls. Using simple mathematical models and numerical simulations, we identify three basic…

Fluid Dynamics · Physics 2015-05-30 E. Victoria Dydek , Boris Zaltzman , Isaak Rubinstein , D. S. Deng , Ali Mani , Martin Z. Bazant

Possible mechanisms of overlimiting current in unsupported electrolytes, exceeding diffusion limitation, have been intensely studied for their fundamental significance and applications to desalination, separations, sensing, and energy…

Fluid Dynamics · Physics 2015-06-22 Sungmin Nam , Inhee Cho , Joonseong Heo , Geunbae Lim , Martin Z. Bazant , Gunyong Sung , Sung Jae Kim

A modified Poisson-Nernst-Planck system in a bounded domain with mixed Dirichlet-Neumann boundary conditions is analyzed. It describes the concentrations of ions immersed in a polar solvent and the correlated electric potential due to the…

Analysis of PDEs · Mathematics 2023-05-25 Ansgar Jüngel , Annamaria Massimini

We revisit the theory of ion transport in parallel-plate channels and also discuss how the wettability of a solid and the mobility of adsorbed surface charges impact the transport of ions. It is shown that depending on the ratio of the…

Soft Condensed Matter · Physics 2021-09-29 Olga I. Vinogradova , Elena F. Silkina , Evgeny S. Asmolov

When electrolyte solutions are confined in micro- and nanochannels their conductivity is significantly different from those in a bulk phase. Here we revisit the theory of this phenomenon by focusing attention on the reduction in the ion…

Soft Condensed Matter · Physics 2023-11-08 Olga I. Vinogradova , Elena F. Silkina

We explore a novel transport phenomenon by studying the effect of surface disorder on electron transport through a finite size conductor with side coupled metallic electrodes. In the strong disorder regime the current amplitude increases…

Mesoscale and Nanoscale Physics · Physics 2009-11-06 Santanu K. Maiti

The problem of stochastic advection of passive particles by circulating conserved flows on networks is formulated and investigated. The particles undergo transitions between the nodes with the transition rates determined by the flows…

Statistical Mechanics · Physics 2015-06-18 Shigefumi Hata , Hiroya Nakao , Alexander S. Mikhailov

Salt transport in bulk electrolytes is limited by diffusion and convection, but in microstructures with charged surfaces (e.g. microfluidic devices, porous media, soils, or biological tissues) surface conduction and electro-osmotic flow…

Fluid Dynamics · Physics 2015-05-30 Ali Mani , Martin Z. Bazant

Ion mobility and ionic conductance in nanodevices are known to deviate from bulk behavior, a phenomenon often attributed to surface effects. We demonstrate that dielectric mismatch between the electrolyte and the surface can qualitatively…

Soft Condensed Matter · Physics 2018-09-17 Hanne S. Antila , Erik Luijten

The molecular mechanism of ion channel gating and substrate modulation is elusive for many voltage gated ion channels, such as eukaryotic sodium ones. The understanding of channel functions is a pressing issue in molecular biophysics and…

Biomolecules · Quantitative Biology 2016-11-15 Duan Chen , Guowei Wei

Unrestricted particle transport through microfluidic channels is of paramount importance to a wide range of applications, including lab-on-a-chip devices. In this article, we study using video microscopy the electro-osmotic aggregation of…

Soft Condensed Matter · Physics 2021-04-02 Zhu Zhang , Joost de Graaf , Sanli Faez

The transient electric current of surfactants dissolved in a nonpolar solvent is investigated both experimentally and theoretically in the parallel-plate geometry. Due to a low concentration of free charges the cell can be completely…

Soft Condensed Matter · Physics 2015-05-30 Pavel Kornilovitch , Yoocharn Jeon

The comprehensive depiction of the many-body effects governing nanoconfined electrolytes is an essential step for the conception of nanofluidic devices with optimized performance. By incorporating self-consistently multivalent charges into…

Soft Condensed Matter · Physics 2020-12-14 Sahin Buyukdagli

We present an efficient and robust numerical model for simulation of electrokinetic phenomena in porous networks over a wide range of applications including energy conversion, desalination, and lab-on-a-chip systems. Coupling between fluid…

Fluid Dynamics · Physics 2016-10-04 Shima Alizadeh , Ali Mani

Ion transport in perm-selective media has been extensively investigated in recent years owing to its applications in advancements of fundamental understanding of nanoscale electrokinetics as well as innovative engineering applications. A…

Fluid Dynamics · Physics 2019-10-31 Junsuk Kim , Keon Huh , Ali Mani , Sung Jae Kim

This study investigates the clustering behaviour and surface distributions of buoyant particles at the air-water interface in open-channel turbulent flow, focusing on the interplay between capillary attraction, hydrodynamic drag, and…

Fluid Dynamics · Physics 2026-01-29 Ana Todorova , Robert K. Niven , Matthias Kramer

The ability to induce regions of high and low ionic concentration adjacent to a permeselective membrane or nanochannel subject to an externally applied electric field (a phenomenon termed concentration-polarization) has been used for a…

Fluid Dynamics · Physics 2018-03-12 Sinwook Park , Gilad Yossifon

We consider the problem of electromigration of a sample ion (analyte) within a uniform background electrolyte when the confining channel undergoes a sudden contraction. One example of such a situation arises in microfluidics in the…

Quantitative Methods · Quantitative Biology 2015-06-05 Zhen Chen , Sandip Ghosal
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