English
Related papers

Related papers: Probing an excited-state atomic transition using h…

200 papers

Vibrational coherences in ultrafast pump-probe (PP) and 2D electronic spectroscopy (2DES) provide insight into the excited state dynamics of molecules. Femtosecond coherence spectra (FCS) and 2D beat maps yield information about…

Chemical Physics · Physics 2024-06-07 Dale Green , Giovanni Bressan , Ismael A. Heisler , Stephen R. Meech , Garth A. Jones

We report excited-state spectroscopy on a quantum dot side-coupled to a quantum wire with accurate energy estimation. Our method utilizes periodic voltage pulses on the dot, and the energy calibration is performed with reference to the bias…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Tomohiro Otsuka , Eisuke Abe , Yasuhiro Iye , Shingo Katsumoto

We report on direct detection of excited states absorption cross-section using dual wavelength pump-probe technique. Also, we experimentally demonstrate using porphyrin composite molecules (porphyrin derivatives such as…

Optics · Physics 2019-03-06 A. Srinivasa Rao , Alok Sharan , N Venkatramaiah , R Venkatesan

We report the measurement of hyperfine splitting in the $7d$ $^{2}D_{3/2}$ state of $^{133}$Cs using high resolution Doppler-free two-photon spectroscopy in a Cs vapor cell. We determine the hyperfine coupling constants $A = 7.3509(9)$ MHz…

Atomic Physics · Physics 2022-10-05 Bubai Rahaman , Sourav Dutta

The ground state and spectral properties of Bose gases in double-well potentials are studied in two different scenarios: i) an interacting atomic Bose gas, and ii) a mixture of an atomic gas interacting with diatomic molecules. A ground…

Quantum Physics · Physics 2015-06-22 Armando Relaño , Jorge Dukelsky , Pedro Perez-Fernandez , Jose M. Arias

We have completed a measurement of the Stark shift within the $^{115}$In $6s_{1/2} \rightarrow 6p_{1/2}$ excited-state transition using two-step laser spectroscopy in an indium atomic beam. Combining this measurement with recent…

Atomic Physics · Physics 2016-09-07 Benjamin L. Augenbraun , Allison Carter , P. M. Rupasinghe , P. K. Majumder

The character of an electronically excited state is one of the most important descriptors employed to discuss the photophysics and photochemistry of transition metal complexes. In transition metal complexes, the interaction between the…

Chemical Physics · Physics 2018-02-14 Sebastian Mai , Felix Plasser , Johann Dorn , Maria Fumanal , Chantal Daniel , Leticia González

The electronic structure of atomic quantum systems and their dynamical interaction with light is reflected in transition dipole matrix elements coupling the system's energy eigenstates. In this work, we measure phase shifts of the…

We present an investigation of the effects of constant but random shifts of the ground hyperfine qubit states in the setting of quantum computing with ion doped crystals. Complex hyperbolic secant pulses can be used to transfer ions…

Quantum Physics · Physics 2013-05-29 Karl Tordrup , Klaus Mølmer

We induce quantum jumps between the hyperfine ground states of one and two Cesium atoms, strongly coupled to the mode of a high-finesse optical resonator, and analyze the resulting random telegraph signals. We identify experimental…

We study the non-integrable Dicke model, and its integrable approximation, the Tavis-Cummings model, as functions of both the coupling constant and the excitation energy. Excited-state quantum phase transitions (ESQPT) are found analyzing…

Quantum Physics · Physics 2014-03-24 M. A. Bastarrachea-Magnani , S. Lerma-Hernandez , J. G. Hirsch

Using the Husimi function, we investigate the phase space signatures of the excited state quantum phase transitions (ESQPTs) in the Lipkin and coupled top models. We show that the time evolution of the Husimi function exhibits distinct…

Quantum Physics · Physics 2021-09-22 Qian Wang , Francisco Pérez-Bernal

The open inner-shell electronic structure of lanthanides with large magnetic moments gives rise to a rich spectrum of transitions available for laser cooling, trapping, and coherent control. Despite this, the large number of ultraviolet…

We propose a two-step protocol for inverting ultrafast spectroscopy experiments on a molecular aggregate to extract the time-evolution of the excited state density matrix. The first step is a deconvolution of the experimental signal to…

Quantum Physics · Physics 2013-05-29 Stephan Hoyer , K. Birgitta Whaley

Phenomena analogous to ground state quantum phase transitions have recently been noted to occur among states throughout the excitation spectra of certain many-body models. These excited state phase transitions are manifested as simultaneous…

Quantum Physics · Physics 2008-05-06 M. A. Caprio , P. Cejnar , F. Iachello

We present measurements of the hyperfine coefficients and isotope shifts of the Dy I $683.731 $nm transition, using saturated absorption spectroscopy on an atomic beam. A King Plot is drawn resulting in an updated value for the specific…

Atomic Physics · Physics 2014-02-27 M. Schmitt , E. A. L. Henn , J. Billy , H. Kadau , T. Maier , A. Griesmaier , T. Pfau

We study the excitation redistribution from cesium $7\mathrm{P}_{1/2}$ or $7\mathrm{P}_{3/2}$ to neighboring energy levels by Black Body Radiation (BBR) and inter atomic collisions using pump-probe spectroscopy inside a vapor cell. At low…

Atomic Physics · Physics 2021-01-21 J. C. de Aquino Carvalho , I. Maurin , H. Failache , D. Bloch , A. Laliotis

Studying the spontaneous emission of a V-type three-level atom embedded in a photonic crystal (PC) by fractional calculus, we found that the atomic excited states in the anisotropic PC can be expressed as a superposition of four dressed…

Quantum Physics · Physics 2011-01-26 Chih-Hsien Huang Jing-Nuo Wu , Yen-Yin Li , Szu-Cheng Cheng , Wen-Feng Hsieh

We experimentally study the heating of trapped atomic ions during measurement of their internal qubit states. During measurement, ions are projected into one of two basis states and discriminated by their state-dependent fluorescence. We…

Quantum Physics · Physics 2024-10-16 A. J. Rasmusson , Ilyoung Jung , Frank G. Schroer , Antonis Kyprianidis , Philip Richerme

We present two-color modulation transfer spectroscopy as a tool for precision studies of atomic properties of excited states. The bi-colored technique addresses a narrow set of velocity groups of a thermal atomic vapour using a two-step…

Atomic Physics · Physics 2008-12-09 A. Perez Galvan , D. Sheng , L. A. Orozco , Y. Zhao