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The effect of the electron temperature on both the light absorption and the scattering by metal nanoparticles (MNs) with excitation of the surface plasmon electron vibrations is studied in the framework of the kinetic theory. The formulae…

Mesoscale and Nanoscale Physics · Physics 2013-11-25 N. I. Grigorchuk

Current thermometry techniques lack the spatial resolution required to see the temperature gradients in typical, highly-scaled modern transistors. As a step toward addressing this problem, we have measured the temperature dependence of the…

Mesoscale and Nanoscale Physics · Physics 2018-01-17 Matthew Mecklenburg , Brian Zutter , B. C. Regan

We study the linewidth of the surface plasmon resonance in the optical absorption spectrum of metallic nanoparticles, when the decay into electron-hole pairs is the dominant channel. Within a semiclassical approach, we find that the…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Rafael A. Molina , Dietmar Weinmann , Rodolfo A. Jalabert

Multipolar plasmon oscillation frequencies and corresponding damping rates for nanospheres formed of the simplest free-electron metals are studied. The possibility of controlling plasmon features by choosing the size and dielectric…

Optics · Physics 2008-04-15 A. Derkachova , K. Kolwas

The temperature dependence of the surface plasmon resonance in small metal spheres is calculated using an electron gas model within the Random Phase Approximation. The calculation is mainly devoted to the study of spheres with diameters up…

Mesoscale and Nanoscale Physics · Physics 2017-06-07 Claudia Fasolato , Francesco Sacchetti , Pietro Tozzi , Caterina Petrillo

The temperature dependences of the energy and the width of a surface plasmon resonance are studied for copper nanoparticles 17 - 59 nm in size in the silica host matrix in the temperature interval 293 - 460 K. An increase of the temperature…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 O. A. Yeshchenko

The electronic environment causes decoherence and dissipation of the collective surface plasmon excitation in metallic nanoparticles. We show that the coupling to the electronic environment influences the width and the position of the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Guillaume Weick , Gert-Ludwig Ingold , Rodolfo A. Jalabert , Dietmar Weinmann

We present an analysis of the temperature dependence of the optical response of small sodium clusters in a temperature range bracketing the melting phase transition. When the temperature increases, the mean excitation energy undergoes a red…

chem-ph · Physics 2009-10-28 Aurel Bulgac , Caio Lewenkopf

Theoretical description of oscillations of electron liquid in large metallic nanospheres (with radius of few tens nm) is formulated within random-phase-approximation semiclassical scheme. Spectrum of plasmons is determined including both…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 W. Jacak , J. Krasnyj , J. Jacak , R. Gonczarek , A. Chepok , L. Jacak , D. Z. Hu , D. Schaadt

We report size-dependent melting of spherical copper nanoparticles embedded into silica matrix. Based on the temperature dependence of the surface plasmon resonance energy and its width we observe two distinct melting regimes. For particles…

Materials Science · Physics 2007-05-23 Oleg A. Yeshchenko , Igor M. Dmytruk , Alexandr A. Alexeenko , Andriy M. Dmytruk

A systematic and detailed investigation of the finite-temperature behavior of small sodium clusters, Na_n, in the size range of n= 8 to 50 are carried out. The simulations are performed using density-functional molecular-dynamics with…

Statistical Mechanics · Physics 2015-06-25 Mal-Soon Lee , S. Chacko , D. G. Kanhere

In order to clarify the relationship between the phonon spectra of nanoparticles and their melting temperature, we studied in detail the size-dependent low energy vibration modes. A minimum model with atoms on a lattice and harmonic…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Kai Kang , Shaojing Qin , Chuilin Wang

The kinetic approach is applied to calculate oscillations of a surface plasmon linewidth in a spheroidal metal nanoparticle embedded in any dielectric media. The principal attention is focused on the case, when the free electron path is…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Nicolas I. Grigorchuk

Two-dimensional hexagonal boron nitride (hBN) has attracted large attentions as platforms for realizations for integrated nanophotonics and collective effort has been focused on the spin defect centers. Here, the temperature dependence of…

A precision measurement of the photoionization of pure sodium and potassium nanoparticles isolated in a beam enabled an accurate determination of their work functions as a function of temperature. In addition to resolving and quantifying…

Mesoscale and Nanoscale Physics · Physics 2026-02-18 Abdelrahman O. Haridy , Atef A. Sheekhoon , Vitaly V. Kresin

A method is proposed for determining the temperature of hot electrons in a metallic nanoparticle embedded in a dielectric matrix under ultrashort laser pulses irradiation. The amplitude and power of the longitudinal spherical acoustic…

Mesoscale and Nanoscale Physics · Physics 2017-12-15 N. I. Grigorchuk

Damping rates of multipolar, localized surface plasmons (SP) of gold and silver nanospheres of radii up to $1000nm$ were found with the tools of classical electrodynamics. The significant increase in damping rates followed by noteworthy…

Optics · Physics 2012-11-21 Krystyna Kolwas , Anastasiya Derkachova

Formation of surface plasmon modes in sodium nanoclusters containing 20-300 atoms was studied using the GW method. It is shown that in the small Na nanoparticles up to 2 nm in size, the loss function $Im[\epsilon^{-1}]$ is dominated by a…

Computational Physics · Physics 2020-06-16 N. L. Matsko

We explore the temperature-dependent plasmonic modes of an n-doped double-layer silicene system which is composed of two spatially separated single layers of silicene with a distance large enough to prevent the interlayer electron…

Mesoscale and Nanoscale Physics · Physics 2021-10-07 N. Dadkhah , T. Vazifehshenas , M. Farmanbar , T. Salavati-fard

We study the role of collective surface excitations in the electron relaxation in small metal particles. We show that the dynamically screened electron-electron interaction in a nanoparticle contains a size-dependent correction induced by…

Condensed Matter · Physics 2009-10-31 T. V. Shahbazyan , I. E. Perakis
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