Related papers: Practical Witness for Electronic Coherences
In many problems, the scattering amplitudes of weak coherent pulse are almost equivalent to the ones of single propagating photon. We thoroughly compare the scattering of: (i) short microwave coherent pulse from rf generator and (ii)…
The development of spectroscopic techniques able to detect and verify quantum coherence is a goal of increasing importance given the rapid progress of new quantum technologies, the advances in the field of quantum thermodynamics, and the…
A general theory of electronic excitations in aggregates of molecules coupled to intramolecular vibrations and the harmonic environment is developed for simulation of the third-order nonlinear spectroscopy signals. The model is applied in…
We develop an ultrafast frequency-resolved Raman spectroscopy with entangled photons for polyatomic molecules in condensed phases, to probe the electronic and vibrational coherences. Using quantum correlation between the photons, the signal…
The entrainment between weakly-coupled nonlinear oscillators, as well as between complex signals such as those representing physiological activity, is frequently assessed in terms of whether a stable relationship is detectable between the…
Pump-probe experiments are used as a controllable way to investigate the properties of photoexcited semiconductors, in particular, the absorption saturation. We present an experiment-theory comparison for ZnSe quantum wells, investigating…
Amplified spontaneous emission is a common noise source in active optical systems, it is generally seen as being an incoherent process. Here we excite an ensemble of rare earth ion dopants in a solid with a {\pi}-pulse, resulting in…
We present experimental coherent two-dimensional Fourier transform spectra of the exciton resonances in semiconductor quantum wells for a pulse sequence that isolates two-quantum coherences. By measuring the real part of the spectra, we can…
Pump-probe spectroscopy is a powerful tool for probing response dynamics of quantum many-body systems in and out-of-equilibrium. Quantum computers have proved useful in simulating such experiments by exciting the system, evolving, and then…
We show that for a class of quantum light spectroscopy (QLS) experiments using n = 0,1,2,$\cdots$ classical light pulses and an entangled photon pair (a biphoton state) where one photon acts as a reference without interacting with the…
Long-lived electronic coherences in various photosynthetic complexes at cryogenic and room temperature have generated vigorous efforts both in theory and experiment to understand their origins and explore their potential role to biological…
The equations governing the interaction between incoherent light and electron-acoustic waves are presented. The modulational instability properties of the system are studied, and the effect of partially coherent light is discussed. It is…
Nonlinear optics experiments measuring phase shifts induced in a weak probe pulse by a strong pump pulse must account for coherent effects that only occur when the pump and probe pulses are temporally overlapped. It is well known that a…
Ultrafast pump-probe spectroscopy is a powerful tool to study the nonequilibrium dynamics in high-Tc cuprate superconductors. The photo-induced quasiparticle (QP) dynamics revealed by pump-probe spectroscopy are sensitive to the near-Fermi…
The non-equilibrium dynamics of matter excited by light may produce electronic phases that do not exist in equilibrium, such as laser-induced high-transition-temperature superconductivity. Here we simulate the dynamics of a metal driven at…
A new method is described for determining the quantum correlations at different times in optical pulses by using balanced homodyne detection. The signal pulse and sequences of ultrashort test pulses are superimposed, where for chosen…
The present review is devoted to our recent studies on the excitonic motion in photosynthetic systems. In photosynthesis, the light photon is absorbed to create an exciton in the antenna complex of the photosynthetic pigments. This exciton…
Coherent light pulses of few to hundreds of femtoseconds (fs) duration have prolifically served the field of ultrafast phenomena. While fs pulses address mainly dynamics of nuclear motion in molecules or lattices in the gas, liquid or…
The non-classical spectral and temporal features of entangled photons offer new possibilities to investigate the interactions of excitons in photosynthetic complexes, and to target the excitation of specific states. Simulations of…
Coherent and squeezed phonon oscillations can be excited in solids impulsively by a single femtosecond pulse whose duration is shorter that a phonon period. By applying the second ultrafast pump pulse these oscillations can be…