Related papers: Bloch-Redfield equations for modeling light-harves…
We are interested in numerically solving a transitional model derived from the Bloch model. The Bloch equation describes the time evolution of the density matrix of a quantum system forced by an electromagnetic wave. In a high frequency and…
Starting from the many-body Schr\"odinger equation, we derive a new type of Lindblad Master equations describing a cyclic exciton/electron dynamics in the light harvesting complex and the reaction center. These equations resemble the Master…
Variational solutions of the Boltzmann equation usually rely on the concept of linear response. We extend the variational approach for tight-binding models at high entropies to a regime far beyond linear response. We analyze both weakly…
The conversion of an absorbed photon from the exciton energy into the reaction centre in the photosynthetic complex has a near unit efficiency. It is becoming clear that any classical model, where the exciton hopping is modeled by a…
Bloch oscillations, the oscillatory motion of a quantum particle in a periodic potential, are one of the most fascinating effects of coherent quantum transport. Originally studied in the context of electrons in crystals, Bloch oscillations…
We demonstrate that the spatial profiles of both propagating and evanescent Bloch-modes in a periodic structure can be extracted from a single measurement of electric field at the specified optical wavelength. We develop a systematic…
Understanding the relationship between the structure of light-harvesting systems and their excitation energy transfer properties is of fundamental importance in many applications including the development of next generation photovoltaics.…
Underlying physical principles for the high efficiency of excitation energy transfer in light-harvesting complexes are not fully understood. Notably, the degree of robustness of these systems for transporting energy is not known considering…
We introduce a non-Hermitian approximation of Bloch optical equations. This approximation provides a complete description of the excitation, relaxation and decoherence dynamics of ensembles of coupled quantum systems in weak laser fields,…
We present an efficient theoretical method for calculating the time evolution of the density matrix of a multilevel quantum system weakly interacting with incoherent light. The method combines the Bloch-Redfield theory with a partial…
The ultrafast conversion of coherent excitons into incoherent excitons, as well as the subsequent exciton diffusion and thermalization, are central topics in current scientific research due to their relevance in optoelectronics,…
We investigate the influence of static disorder and thermal excitations on excitonic energy transport in the light-harvesting apparatus of photosynthetic systems by solving the Schr\"{o}dinger equation and taking into account the coherent…
Low-light photography produces images with low signal-to-noise ratios due to limited photons. In such conditions, common approximations like the Gaussian noise model fall short, and many denoising techniques fail to remove noise…
Bloch oscillations of atoms in optical lattices are a powerful technique that can boost the sensitivity of atom interferometers to a wide range of signals by large momentum transfer. To leverage this method to its full potential, an…
Dynamical mean-field theory is generalized to solve the nonequilibrium Keldysh boundary problem: a system is started in equilibrium at a temperature T=0.1, a uniform electric field is turned on at t=0, and the system is monitored as it…
The engineering of synthetic dimensions allows for the construction of fictitious lattice structures by coupling the discrete degrees of freedom of a physical system, such as the quantized modes of an electromagnetic cavity or the internal…
This work develops photoacoustic-based experimental methods for comprehensive characterization of multispecies mass transport from donor compartments to thin-membrane acceptor systems in perfect contact, supported by a dedicated mass…
We study the time dynamics of the ohmic spin boson model at arbitrary bias $\epsilon$ and small coupling $\alpha$ to the bosonic bath. Using perturbation theory and the real-time renormalization group (RG) method we present a consistent…
Biomolecular light-harvesting antennas operate as nanoscale devices in a regime where the coherent interactions of individual light, matter and vibrational quanta are non-perturbatively strong. The complex behaviour arising from this could,…
This thesis looks at the electronic energy transfer in the Fenna-Matthews-Olson complex, in which evidence of long-lived coherence has been observed in 2-dimensional infrared experiments. I use three techniques: the numerically exact…