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Ultrafast two-dimensional spectroscopy utilizes correlated multiple light-matter interactions for retrieving dynamic features that may otherwise be hidden under the linear spectrum. Its extension to the terahertz regime of the…

We theoretically demonstrate the possibility to tune the temporal waveform of optical unipolar pulses upon their coherent interaction with a multi-level resonant medium. This is achieved through the coherent control of the response of a…

We investigate the effect of phase modulation of laser beams on the coherent and incoherent non-linear signals arising from the interaction of femtosecond pulses with matter. We observe that two collinear beams, whose phases are modulated…

Optics · Physics 2015-05-29 Khadga Jung Karki , Loni Kringle , Andrew H. Marcus , Tõnu Pullerits

Two-level systems (TLS) of unclear physical origin are a major contributor to decoherence in superconducting qubits. The interactions of individual TLS with a qubit can be detected via various spectroscopic methods, most of which have…

We show that useful non-instantaneous nonlinear phase shifts can be obtained from cascaded quadratic processes in the presence of group velocity mismatch. The two-field nature of the process permits responses that can be effectively…

Optics · Physics 2009-11-10 F. Ö. Ilday , K. Beckwitt , Y. -F. Chen , H. Lim , F. W. Wise

Terahertz time domain spectroscopy employing free-space radiation has frequently been used to probe the elementary excitations of low-dimensional systems. The diffraction limit blocks its use for the in-plane study of individual laterally…

We propose an efficient all-optical phase modulation based on a double-{\Lambda} system and demonstrate a {\pi} phase shift of a few-photon pulse induced by another few-photon pulse in cold rubidium atoms with this scheme. By changing the…

We experimentally generate three-dimensional speckles with customized intensity statistics. By modulating the phase front of a laser beam, far-field speckle patterns maintain the designed intensity probability density function while…

Optics · Physics 2023-03-15 SeungYun Han , Nicholas Bender , Hui Cao

Strong-field phenomena driven by an intense infrared (IR) laser depend on during what part of the field cycle they are initiated. By changing the sub-cycle character of the laser electric field it is possible to control such phenomena. For…

This paper presents a novel approach using multiple linear regression to process transient signals from silicon photomultipliers. The method provides excellent noise suppression and pulse detection in scenarios with a high pulse count rate…

Instrumentation and Detectors · Physics 2023-07-19 Wolfgang Schmailzl , Claudio Piemonte , Erika Garutti , Walter Hansch

In this work, we experimentally manipulate the spectrum and phase of a biphoton wave packet in a two-dimensional frequency space. The spectrum is shaped by adjusting the temperature of the crystal, and the phase is controlled by tilting the…

Quantum Physics · Physics 2018-08-14 Rui-Bo Jin , Ryoji Shiina , Ryosuke Shimizu

A study about the reflection and transmission of an electromagnetic pulse through a slab doped with four-level atomic system has been presented. The doped atoms are considered to be in N-configuration with a pump field and a weak probe…

Quantum Physics · Physics 2024-03-26 Yasir Ali

We report the experimental observation of a cross-Kerr nonlinearity in a free-space medium based on resonantly-excited, interacting Rydberg atoms and electromagnetically induced transparency. The nonlinearity is used to implement…

We introduce the concept of phase-synchronous undersampling in nonlinear spectroscopy. The respective theory is presented and validated experimentally in a phase-modulated quantum beat experiment by sampling high phase modulation…

Chemical Physics · Physics 2018-03-14 Lukas Bruder , Marcel Binz , Frank Stienkemeier

A theory of pump-probe spectroscopy is developed in which optical fields drive two-quantum, Raman-like transitions between ground state sublevels. Three fields are incident on an ensemble of atoms. Two of the fields act as the pump field…

Atomic Physics · Physics 2009-11-06 P. R. Berman , B. Dubetsky

We calculate the utility of high-frequency squeezed-state enhanced two-frequency interferometry for low-frequency phase measurement. To use the high-frequency sidebands of the squeezed light, a two-frequency intense laser is used in the…

Quantum Physics · Physics 2015-05-27 Zehui Zhai , Jiangrui Gao

We show that photon wave packets can be manipulated and reshaped in various ways by a quantum junction comprising a set of three-level atoms coupling two waveguides. We consider atomic nodes with the $\Lambda$-scheme of allowed optical…

Quantum Physics · Physics 2020-01-20 M. Ahumada , P. A. Orellana , A. V. Malyshev

We present a simple approach to predict the main features of optical spectra affected by self-phase modulation (SPM), which is based on regarding the spectrum modification as an interference effect. A two-wave interference model is found…

Optics · Physics 2018-12-26 Christophe Finot , Frédéric Chaussard , Sonia Boscolo

We introduce a novel analysis technique for pulsar secondary spectra. The power spectrum of pulsar scintillation (referred to as the "secondary spectrum") shows differential delays and Doppler shifts due to interference from multi-path…

Instrumentation and Methods for Astrophysics · Physics 2020-12-02 Tim Sprenger , Olaf Wucknitz , Robert Main , Daniel Baker , Walter Brisken

The major development recently undergone by quantum cascade lasers has effectively extended frequency comb emission to longer-wavelength spectral regions, i.e. the mid and far infrared. Unlike classical pulsed frequency combs, their…