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The computational study of energy storage and conversion processes calls for simulation techniques that can reproduce the electronic response of metal electrodes under electric fields. Despite recent advancements in machine-learning methods…

Materials Science · Physics 2024-05-14 Andrea Grisafi , Augustin Bussy , Mathieu Salanne , Rodolphe Vuilleumier

Two main approaches in particle-based simulations for modeling a charged surface are using explicit, discrete charges and continuum, uniform charges. It is well-known that these two approaches could lead to substantially distinct ionic…

Soft Condensed Matter · Physics 2022-08-02 Jiaxing Yuan , Yanwei Wang

We present an efficient method for simulating Coulomb systems confined by metal electrodes. The approach relies on Green functions techniques to obtain the electrostatic potential for an infinite periodically replicated system. This avoids…

Soft Condensed Matter · Physics 2017-12-14 Matheus Girotto , Alexandre P. dos Santos , Yan Levin

We report a general macroscopic theory for the electrodynamic response of semi-infinite metals (SIMs). The theory includes the hitherto overlooked capacitive effects due to the finite spatial extension of a surface. The basic structure of…

Mesoscale and Nanoscale Physics · Physics 2020-05-12 Hai-Yao Deng

Supercapacitors are promising electrochemical energy storage devices due to their prominent performance in rapid charging/discharging rates, long cycle life, stability, etc. Experimental measurement and theoretical prediction on charging…

Numerical Analysis · Mathematics 2023-05-31 Lijie Ji , Zhenli Xu , Shenggao Zhou

Electrochemical interfaces are of fundamental importance in electrocatalysis, batteries, and metal corrosion. Finite-field methods are one of most reliable approaches for modeling electrochemical interfaces in complete cells under realistic…

Chemical Physics · Physics 2025-06-13 Chaoqiang Feng , Bin Jiang

The dynamics of the electrons for a molecule in solution is coupled to the dynamics of its polarizable environment, i.e., the solvent. To theoretically investigate such electronic dynamics, we have recently developed equations of motion…

Chemical Physics · Physics 2017-02-16 Silvio Pipolo , Stefano Corni , Roberto Cammi

Charge Coupled Devices (CCDs) have been successfully used in several high energy physics experiments over the past two decades. Their high spatial resolution and thin sensitive layers make them an excellent tool for studying short-lived…

Polymeric ionic liquids are emerging polyelectrolyte materials for modern electrochemical applications. In this paper, we propose a self-consistent field theory of the polymeric ionic liquid on a charged conductive electrode. Taking into…

Soft Condensed Matter · Physics 2022-02-02 Yury A. Budkov , Nikolai N. Kalikin , Andrei L. Kolesnikov

Flexoelectricity refers to a phenomenon which involves a coupling of the mechanical strain gradient and electric polarization. In this study, a meshless Fragile Points Method (FPM), is presented for analyzing flexoelectric effects in…

Numerical Analysis · Mathematics 2020-11-13 Yue Guan , Leiting Dong , Satya N. Atluri

Electrolyte solutions play an important role in energy storage devices, whose performance highly relies on the electrokinetic processes at sub-micron scales.\ Although fluctuations and stochastic features become more critical at small…

Soft Condensed Matter · Physics 2022-06-08 Mingge Deng , Faisal Tushar , Luis Bravo , Anindya Ghoshal , George Karniadakis , Zhen Li

A modified version of the spinless Anderson model is studied by means of the continuous-time quantum Monte Carlo method. This study is motivated by the peculiar heavy-fermion behavior observed in certain Samarium compounds, which is…

Strongly Correlated Electrons · Physics 2015-10-28 Annamaria Kiss , Yoshio Kuramoto , Junya Otsuki

Constant potential molecular dynamics simulation plays important role for applications of electrochemical systems, yet the calculation of charge fluctuation on electrodes remains a computational bottleneck. We propose a highly scalable,…

Computational Physics · Physics 2025-09-30 Weihang Gao , Qi Zhou , Qianru Zhang , Zhenli Xu

Using the asymptotic iteration method (AIM) we investigate the variation in the 1s energy levels of hydrogen and helium-like static ions in fully degenerate electron gas. The semiclassical Thomas-Fermi (TF), Shukla-Eliasson (SE) and…

Quantum Gases · Physics 2020-04-22 M. Akbari-Moghanjoughi , Alireza Abdikian , Arash Phirouznia

Charge Coupled Devices (CCDs) have been successfully used in several high energy physics experiments over the past two decades. Their high spatial resolution and thin sensitive layers make them an excellent tool for studying short-lived…

We propose a finite element method for the numerical simulation of electroconvection of thin liquid crystals. The liquid is located in between two concentric circular electrodes which are either assumed to be of infinite height or slim.…

Numerical Analysis · Mathematics 2020-01-29 Andrea Bonito , Peng Wei

Nonlinear elements in a rectifying circuit can be used to harvest energy from thermal fluctuations either steadily or transitorily. We study an energy harvesting system comprising a small variable capacitor (e.g., free standing graphene)…

Statistical Mechanics · Physics 2026-02-12 L. L. Bonilla , A. Torrente , J. M. Mangum , P. M. Thibado

The rapid and efficient exchange of ions between porous electrodes and aqueous solutions is important in many applications, such as electrical energy storage by super-capacitors, water desalination and purification by capacitive…

Chemical Physics · Physics 2015-05-14 P. M. Biesheuvel , M. Z. Bazant

In this study the Singlet Reference Interaction Site Model (SRISM) is employed to the study of the electrode charge dependence of the capacitance of a planar electric double layer using the primitive model of the double layer for a high…

Soft Condensed Matter · Physics 2012-02-23 S. Woelki , D. Henderson

In this work, we develop an extended uniform potential (UP) model for a membrane nanopore by including two different charging mechanisms of the pore walls, namely by electronic charge and by chemical charge. These two charging mechanisms…

Chemical Physics · Physics 2019-12-25 L. Zhang , P. M. Biesheuvel , I. I. Ryzhkov