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We have implemented a generic method, based on the 2n+1 theorem within density functional perturbation theory, to calculate the anharmonic scattering coefficients among three phonons with arbitrary wavevectors. The method is used to study…

Materials Science · Physics 2014-06-24 Lorenzo Paulatto , Francesco Mauri , Michele Lazzeri

We present the first Raman spectroscopic study of Bernal bilayer graphene flakes under uniaxial tension. Apart from a purely mechanical behavior in flake regions where both layers are strained evenly, certain effects stem from inhomogeneous…

We demonstrate the first experimental observation of coherent population oscillation, an optical analogue of electromagnetically induced transparency, in graphene based on phase sensitive pump-probe system. Degenerate four-wave-mixing…

Optics · Physics 2016-04-08 Lei Gao , Tao Zhu , Min Liu , Wei Huang , Yu Jia Li , Cong Gao

By considering analytical expressions for the self-energies of intervalley and intravalley phonons in graphene, we describe the behavior of D, 2D, and D$'$ Raman bands with changes in doping ($\mu$) and light excitation energy ($E_L$).…

Mesoscale and Nanoscale Physics · Physics 2013-01-30 K. Sasaki , K. Kato , Y. Tokura , S. Suzuki , T. Sogawa

We report a comprehensive micro-Raman scattering study of electrochemically-gated graphene field-effect transistors. The geometrical capacitance of the electrochemical top-gates is accurately determined from dual-gated Raman measurements,…

Mesoscale and Nanoscale Physics · Physics 2016-08-08 Guillaume Froehlicher , Stéphane Berciaud

We theoretically investigate the double-resonance Raman spectrum of monolayer graphene down to infrared laser excitation energies. By using first-principles density functional theory calculations, we improve upon previous theoretical…

Mesoscale and Nanoscale Physics · Physics 2025-05-21 Lorenzo Graziotto , Francesco Macheda , Thibault Sohier , Matteo Calandra , Francesco Mauri

Recent advances in strain engineering at the nanoscale have shown the feasibility to modulate the properties of graphene. Although the electron-phonon (e-ph) coupling and Kohn anomalies in graphene define the phonon branches contributing to…

Mesoscale and Nanoscale Physics · Physics 2016-08-02 M. E. Cifuentes-Quintal , O. de la Peña-Seaman , R. Heid , R. de Coss , K. -P. Bohnen

Precise infrared magnetotransmission experiments have been performed in magnetic fields up to 32 T on a series of multilayer epitaxial graphene samples. We observe changes in the spectral features and broadening of the main cyclotron…

Mesoscale and Nanoscale Physics · Physics 2012-06-15 M. Orlita , Liang Z. Tan , M. Potemski , M. Sprinkle , C. Berger , W. A. de Heer , Steven G. Louie , G. Martinez

Although plasmon modes exist in doped graphene, the limited range of doping achieved by gating restricts the plasmon frequencies to a range that does not include visible and infrared. Here we show, through the use of first-principles…

Mesoscale and Nanoscale Physics · Physics 2018-05-30 Sharmila N. Shirodkar , Marios Mattheakis , Paul Cazeaux , Prineha Narang , Marin Soljačić , Efthimios Kaxiras

The symmetry group analysis is applied to classify the phonon modes of $N$-stacked graphene layers (NSGL's) with AB- and AA-stacking, particularly their infra-red and Raman properties. The dispersions of various phonon modes are calculated…

Materials Science · Physics 2008-06-30 Jin-Wu Jiang , Hui Tang , Bing-Shen Wang , Zhao-Bin Su

The interaction of graphene with metallic substrates reveals phenomena and properties of great relevance for applications in nanotechnology. In this review, the vibrational characterization by means of various inelastic scattering…

Materials Science · Physics 2016-01-08 Antonio Politano

The phonon dispersion of graphene on Ir(111) has been determined by means of angle-resolved inelastic electron scattering and density functional calculations. Kohn anomalies of the highest optical-phonon branches are observed at the…

Materials Science · Physics 2015-06-17 M. Endlich , A. Molina-Sánchez , L. Wirtz , J. Kröger

Recent infrared measurements of phonon peaks in gated bilayer graphene reveal two striking signatures of electron-phonon interaction: an asymmetric Fano lineshape and a giant variation of the peak intensity as a function of the applied gate…

Strongly Correlated Electrons · Physics 2010-07-26 E. Cappelluti , L. Benfatto , A. B. Kuzmenko

We study the variations of electron-phonon coupling and their spectroscopic consequences in response to sliding of two layers in bilayer graphene using first-principles calculations and a model Hamiltonian. Our study shows that the long…

Mesoscale and Nanoscale Physics · Physics 2013-07-25 Seon-Myeong Choi , Seung-Hoon Jhi , Young-Woo Son

Density functional perturbation theory is used to analyze electron-phonon interaction in bilayer graphene. The results show that phonon scattering in bilayer graphene bears more resemblance with bulk graphite than monolayer graphene. In…

Mesoscale and Nanoscale Physics · Physics 2010-11-29 K. M. Borysenko , J. T. Mullen , X. Li , Y. G. Semenov , J. M. Zavada , M. Buongiorno Nardelli , K. W. Kim

We present a first-principles study of the electron-phonon (e-ph) interactions and their contributions to the linewidths for the optical phonon modes at $\Gamma$ and K in one to three-layer graphene. It is found that due to the interlayer…

Materials Science · Physics 2009-03-31 Jia-An Yan , W. Y. Ruan , M. Y. Chou

We propose a two-dimensional plasmonic platform - periodically patterned monolayer graphene - which hosts topological one-way edge states operable up to infrared frequencies. We classify the band topology of this plasmonic system under…

Mesoscale and Nanoscale Physics · Physics 2017-06-21 Dafei Jin , Thomas Christensen , Marin Soljačić , Nicholas X. Fang , Ling Lu , Xiang Zhang

Twisted bilayer graphene (tBLG) devices with ion gel gate dielectrics are studied using Raman spectroscopy in the twist angle regime where a resonantly enhanced G band can be observed. We observe prominent splitting and intensity quenching…

Mesoscale and Nanoscale Physics · Physics 2015-02-18 Ting-Fung Chung , Rui He , Tai-Lung Wu , Yong P. Chen

We report a comprehensive study of the two-phonon inter-valley (2D) Raman mode in graphene monolayers, motivated by recent reports of asymmetric 2D-mode lineshapes in freestanding graphene. For photon energies in the range $1.53 \rm eV -…

Mesoscale and Nanoscale Physics · Physics 2014-06-26 Stéphane Berciaud , Xianglong Li , Han Htoon , Louis E. Brus , Stephen K. Doorn , Tony F. Heinz

We report the dispersion measurements, using angle-resolved reflection electron-energy-loss-spectroscopy (AREELS), on two-dimensional (2D) plasmons in single and multilayer graphene which couple strongly to surface optical phonon (FK…

Mesoscale and Nanoscale Physics · Physics 2010-05-03 Yu Liu , Roy F. Willis