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We report theoretical investigations of the tomographic procedure suggested by Itatani {\it et al.} [Nature, {\bf 432} 867 (2004)] for reconstructing highest occupied molecular orbitals (HOMO) using high-order harmonic generation (HHG).…

Atomic Physics · Physics 2009-10-30 Van-Hoang Le , Anh-Thu Le , Rui-Hua Xie , C. D. Lin

We investigate the orientation dependence of high-order harmonic generation (HHG) from H$_2^+$ with different internuclear distances irradiated by intense laser fields both numerically and analytically. The calculated molecular HHG spectra…

Atomic Physics · Physics 2009-11-13 Yanjun Chen , Jie Liu , Bambi Hu

We present studies of high-order harmonic generation (HHG) at laser intensities well above saturation. We use driving laser pulses which present a particular electron dynamics in the turn-on stage. Our results predict an increasing on the…

Atomic Physics · Physics 2015-06-19 J. A. Pérez-Hernández , M. F. Ciappina , M. Lewenstein , A. Zaïr , L. Roso

High harmonic emissions from crystalline solids contain rich information on the dynamics of electrons driven by intense infrared laser fields and have been intensively studied owing to their potential use as a probe of microscopic…

Materials Science · Physics 2023-05-01 K. Uchida , K. Tanaka

High-order harmonic responses from three $C_{20}$ isomers: fullerene, ring, and bowl, are calculated within the modified Lewenstein model for molecular systems. Spectra for all three structures exhibit intense modulations of the harmonic…

Quantum Physics · Physics 2022-03-31 F. Cajiao - Vélez , A. Jaron

This Letter brings together two topics that, until now, have been the focus of intense but non-overlapping research efforts. The first concerns high harmonic generation in solids, which occurs when intense light field excites highly…

Strongly Correlated Electrons · Physics 2022-04-06 R. E. F. Silva , Igor V. Blinov , Alexey N. Rubtsov , O. Smirnova , M. Ivanov

High-order harmonic generation (HHG) with relativistically strong laser pulses is considered employing electron ionization-recollisions from multiply charged ions in counterpropagating, linearly polarized attosecond pulse trains. The…

Atomic Physics · Physics 2015-05-19 Markus C. Kohler , Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

We find that, for sufficiently strong mid-IR fields, transitions between different conduction bands play an important role in the generation of high-order harmonics in a dielectric. The transitions make a significant contribution to the…

Other Condensed Matter · Physics 2015-06-22 Peter G. Hawkins , Misha Yu. Ivanov , Vladislav S. Yakovlev

We investigate High-harmonic generation (HHG) in a dimerized Kitaev chain. The dimerization in the model is introduced through a site-dependent modulating potential, determined by a parameter $\lambda \in [-1:1]$. This parameter also…

Other Condensed Matter · Physics 2025-06-06 Nivash R. , S. Srinidhi , Jayendra N. Bandyopadhyay , Amol R. Holkundkar

High-order harmonic generation in multiphoton ionization regime is studied theoretically to examine the resonant effects of the generating particle. We solve the time-dependent Schr\"odinger equation for In+ in the laser field by expanding…

Atomic Physics · Physics 2023-12-12 Alexander I. Magunov , Vasily V. Strelkov

High harmonic generation (HHG) is an extreme nonlinear frequency up-conversion process during which extremely short duration optical pulses at very short wavelengths are emitted. A major concern of HHG is the small conversion efficiency at…

We studied the high-order harmonic generation (HHG) from 2D solid materials in circularly and bichromatic circularly polarized laser fields numerically by simulating the dynamics of single-active-electron processes in 2D periodic…

We experimentally disentangle the contributions of different quantum paths in high-order harmonic generation (HHG) from the spectrally and spatially resolved harmonic spectra. By adjusting the laser intensity and focusing position, we…

Atomic Physics · Physics 2015-10-08 Lixin He , Pengfei Lan , Qingbin Zhang , Chunyang Zhai , Feng Wang , Wenjing Shi , Peixiang Lu

We present the generation of high order harmonics in crystalline silicon subjected to intense near-infrared 30fs laser pulse. The harmonic spectrum extends from the near infrared to the extreme ultraviolet spectral region. Depending on the…

Atomic Physics · Physics 2020-08-10 Boyan Obreshkov , Tzveta Apostolova

Attosecond light sources based on high-order harmonic generation (HHG) constitute to date the only table-top solution for producing coherent broadband radiation covering the spectral range from the extreme ultraviolet to the soft X-rays.…

High harmonic generation (HHG) is a manifestation of the strongly nonlinear response of matter to intense laser fields and has, as the basis for coherent XUV sources a variety of applications. Recently, HHG from atoms in a phase and…

Optics · Physics 2020-05-20 Jonas Wätzel , Jamal Berakdar

An important goal in molecular physics and chemistry today is to obtain structure-dependent information about molecular function to obtain a deeper understanding into chemical reactions. However, until now, asymmetric tops, which comprise…

By using Bohmian trajectory method, we investigate the dynamic interference in diatomic molecular high-order harmonic generation progress. It is demonstrated that the main characteristics of the molecular harmonic spectrum can be well…

Atomic Physics · Physics 2013-08-05 Yang Song , Bing-Bing Wang , Fu-Ming Guo , Su-Yu Li , Xue-Shen Liu , Ji-Gen Chen , Si-Liang Zeng , Yu-Jun Yang

We investigate the process of circularly polarized high harmonic generation in molecules using a bicircular laser field. In this context, we show that molecules offer a very robust framework for the production of circularly polarized…

Atomic Physics · Physics 2016-06-22 F Mauger , A. D. Bandrauk , T Uzer

We theoretically propose a multidimensional high-harmonic echo spectroscopy technique which utilizes strong optical fields to resolve coherent electron dynamics spanning an energy range of multiple electron Volts. Using our recently…