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We present a detailed investigation of the exciton and trion dynamics in naturally doped MoSe2 and WSe2 single atomic layers as a function of temperature in the range 10-300K under above band-gap laser excitation. By combining…

To study relaxation dynamics of the two-dimensional XY gauge glass, we integrate directly the equations of motion and investigate the energy function. As usual, it decays exponentially at high temperatures; at low but non-zero temperatures,…

Superconductivity · Physics 2008-02-03 Beom Jun Kim , M. Y. Choi , S. Ryu , D. Stroud

Photoluminescence (PL) and reflectivity spectra of a high-quality InGaAs/GaAs quantum well structure reveal a series of ultra-narrow peaks attributed to the quantum confined exciton states. The intensity of these peaks decreases as a…

Unconventional emissions from exciton and trion in monolayer WS2 are studied by photoexcitation. Excited by 532nm laser beam, the carrier species in the monolayer WS2 are affected by the excess electrons escaping from photoionization of…

Mesoscale and Nanoscale Physics · Physics 2016-08-08 Ke Wei , Yu Liu , Hang Yang , Xiangai Cheng , Tian Jiang

Heavy metal-based two-dimensional van der Waals materials have a large, coupled spin and valley Hall effect (SVHE) that has potential use in spintronics and valleytronics. Optical measurements of the SVHE have largely been performed below…

Mesoscale and Nanoscale Physics · Physics 2022-02-25 Xintong Li , Zhida Liu , Yihan Liu , Suyogya Karki , Xiaoqin Li , Deji Akinwande , Jean Anne C. Incorvia

We exploit the influence of the Coulomb interaction between electrons and holes on the electron spin relaxation in a (110)-GaAs quantum well to unveil excitonic signatures within the many particle electron-hole system. The temperature…

Mesoscale and Nanoscale Physics · Physics 2011-04-07 S. Oertel , S. Kunz , D. Schuh , W. Wegscheider , J. Hübner , M. Oestreich

While conventional semiconductor technology relies on the manipulation of electrical charge for the implementation of computational logic, additional degrees of freedom such as spin and valley offer alternative avenues for the encoding of…

The emergence of spatial and temporal coherence of light emitted from solid-state systems is a fundamental phenomenon, rooting in a plethora of microscopic processes. It is intrinsically aligned with the control of light-matter coupling,…

Monolayer transition metal dichalcogenides (TMDs) are characterized by relatively large carrier effective masses and suppressed screening of the Coulomb interaction, which substantially enhances the correlation effects in these structures.…

We investigate the valley related carrier dynamics in monolayer MoS2 using helicity resolved non-degenerate ultrafast pump-probe spectroscopy at the vicinity of the high-symmetry K point under the temperature down to 78 K. Monolayer MoS2…

Optics · Physics 2014-05-08 Qinsheng Wang , Shaofeng Ge , Xiao Li , Jun Qiu , Yanxin Ji , Ji Feng , Dong Sun

Exciton binding energy and excited states in monolayers of tungsten diselenide (WSe2) are investigated using the combined linear absorption and two-photon photoluminescence excitation spectroscopy. The exciton binding energy is determined…

Materials Science · Physics 2015-06-19 Keliang He , Nardeep Kumar , Liang Zhao , Zefang Wang , Kin Fai Mak , Hui Zhao , Jie Shan

In van der Waals heterostructures (HS) consisting of stacked MoSe$_2$ and WSe$_2$ monolayers, optically bright interlayer excitons (ILE) can be observed when the constituent layers are crystallographically aligned. The symmetry of the…

Monolayers of semiconducting transition metal dichalcogenides are two-dimensional direct-gap systems which host tightly-bound excitons with an internal degree of freedom corresponding to the valley of the constituting carriers. Strong…

Abstract The valley degree of freedom in two-dimensional materials provides an opportunity to extend the functionalities of valleytronics devices. Very short valley lifetimes demand the ultrafast control of valley pseudospin. Here, we…

We present here a formalism based on time-dependent density-functional theory (TDDFT) to describe characteristics of both intra- and inter-valley excitons in semiconductors, the latter of which had remained a challenge. Through the usage of…

Materials Science · Physics 2023-05-10 Jia Shi , Volodymyr Turkowski , Duy Le , Talat S. Rahman

We present time-resolved Kerr rotation measurements, showing spin lifetimes of over 100 ns at room temperature in monolayer MoSe$_2$. These long lifetimes are accompanied by an intriguing temperature dependence of the Kerr amplitude, which…

Monolayers of transition-metal dichalcogenides (TMDs) are characterized by an extraordinarily strong Coulomb interaction giving rise to tightly bound excitons with binding energies of hundreds of meV. Excitons dominate the optical response…

Materials Science · Physics 2018-05-30 Samuel Brem , Gunnar Berghaeuser , Malte Selig , Ermin Malic

We report the results of X-ray photon correlation spectroscopy (XPCS) experiments on Langmuir Blodgett multilayers of a photosensitive azo-polymer. Time correlation functions have been measured at different temperatures and momentum…

Soft Condensed Matter · Physics 2012-03-29 Davide Orsi , Luigi Cristofolini , Marco P. Fontana , Anders Madsen , Andrei Fluerasu

The variety of excitonic states in tungsten-based dichalcogenide monolayers stems from unique interplay between the spin and valley degrees of freedom. One of the exciton species is the indirect exciton (momentum or valley dark), which is…

Mesoscale and Nanoscale Physics · Physics 2022-08-23 Pengke Li , Cedric Robert , Dinh Van Tuan , Lei Ren , Xavier Marie , Hanan Dery

The macroscopic exciton rings observed in the photoluminescence (PL) patterns of excitons in coupled quantum wells (CQWs) are explained by a series of experiments and a theory based on the idea of carrier imbalance, transport and…

Condensed Matter · Physics 2008-04-12 L. V. Butov , L. S. Levitov , A. V. Mintsev , B. D. Simons , A. C. Gossard , D. S. Chemla
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