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Related papers: Selectively Localized Wannier Functions

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Within this paper we outline a method able to generate truly minimal basis sets which describe either a group of bands, a band, or even just the occupied part of a band accurately. These basis sets are the so-called NMTOs, Muffin Tin…

Strongly Correlated Electrons · Physics 2009-09-29 Eva Zurek , Ove Jepsen , Ole K. Andersen

Accurate prediction of electronic and optical excitations in van der Waals (vdW) materials is a long-standing challenge for density functional theory. The recently proposed Wannier-localized optimally-tuned screened range-separated hybrid…

The Hartree-Fock equations are modified to directly yield Wannier functions following a proposal of Shukla et al. [Chem. Phys. Lett. 262, 213-218 (1996)]. This approach circumvents the a posteriori application of the Wannier transformation…

Other Condensed Matter · Physics 2007-05-23 Christian Buth

Variational wave function ansatze are an invaluable tool to study the properties of strongly correlated systems. We propose such a wave function, based on the theory of auxiliary fields and combining aspects of auxiliary-field quantum Monte…

Strongly Correlated Electrons · Physics 2024-03-13 Ryan Levy , Miguel A. Morales , Shiwei Zhang

We formulate Wannier orbital overlap population and Wannier orbital Hamilton population to describe the contribution of different orbitals to electron distribution and their interactions. These methods, which are analogous to the well known…

Computational Physics · Physics 2021-03-31 Sudipta Kundu , Satadeep Bhattacharjee , Seung-Cheol Lee , Manish Jain

The DFT/vdW-WF2s1 method based on the generation of localized Wannier functions, recently developed to include the van der Waals interactions in the Density Functional Theory and describe adsorption processes on metal surfaces by taking…

Chemical Physics · Physics 2016-04-06 Pier Luigi Silvestrelli , Alberto Ambrosetti

We present a first-principles calculation of the electronic properties of crystalline silicon and gallium arsenide in a uniform electric field. Polarized Wannier-like functions which are confined in a finite region are obtained by…

Materials Science · Physics 2007-05-23 Pablo Fernández , Andrea Dal Corso , Alfonso Baldereschi

A robust, user-friendly, and automated method to determine quantum conductance in disordered quasi-one-dimensional systems is presented. The scheme relies upon an initial density- functional theory calculation in a specific geometry after…

Computational Physics · Physics 2015-03-17 Matthew Shelley , Nicolas Poilvert , Arash A Mostofi , Nicola Marzari

In a tight-binding lattice model with $n$ orbitals (single-particle states) per site, Wannier functions are $n$-component vector functions of position that fall off rapidly away from some location, and such that a set of them in some sense…

Mesoscale and Nanoscale Physics · Physics 2017-03-29 N. Read

We present an efficient first-principles approach for calculating Fermi surface averages and spectral properties of solids, and use it to compute the low-field Hall coefficient of several cubic metals and the magnetic circular dichroism of…

Materials Science · Physics 2009-11-13 Jonathan R. Yates , Xinjie Wang , David Vanderbilt , Ivo Souza

The exponential localization of Wannier functions in two or three dimensions is proven for all insulators that display time-reversal symmetry, settling a long-standing conjecture. Our proof relies on the equivalence between the existence of…

We present a computational approach which is tailored for reducing the complexity of the description of extended systems at the density functional theory level. We define a recipe for generating a set of localized basis functions which are…

Materials Science · Physics 2019-04-16 Laura E. Ratcliff , Luigi Genovese

A scheme within density functional theory is proposed that provides a practical way to generalize to unrestricted geometries the method applied with some success to layered geometries [H. Rydberg, et al., Phys. Rev. Lett. 91, 126402…

Materials Science · Physics 2009-11-10 M. Dion , H. Rydberg , E. Schroder , D. C. Langreth , B. I. Lundqvist

Localization of molecular orbitals finds its importance in the representation of chemical bonding (and anti-bonding) and in the local correlation treatments beyond mean-field approximation. In this paper, we generalize the intrinsic atomic…

Chemical Physics · Physics 2021-02-11 Bruno Senjean , Souloke Sen , Michal Repisky , Gerald Knizia , Lucas Visscher

It is believed that the density functional theory (DFT) describes most elements with s, p and d orbitals very well, except some materials that having strongly localized and correlated valence electrons. In this work, we find that the widely…

Materials Science · Physics 2020-03-17 Y. X. Wang , Hua Y. Geng , Q. Wu , Xiang R. Chen

The Wegner orbital model is a class of random operators introduced by Wegner to model the motion of a quantum particle with many internal degrees of freedom (orbitals) in a disordered medium. We consider the case when the matrix potential…

Mathematical Physics · Physics 2017-09-22 Jeffrey Schenker , Ron Peled , Mira Shamis , Sasha Sodin

Following the operator algebraic approach to Gabor analysis, we construct frames of translates for the Hilbert space localisation of the Morita equivalence bimodule arising from a groupoid equivalence between Hausdorff groupoids, where one…

Operator Algebras · Mathematics 2021-08-06 Chris Bourne , Bram Mesland

The Wannier localization problem in quantum physics is mathematically analogous to finding a localized representation of a subspace corresponding to a nonlinear eigenvalue problem. While Wannier localization is well understood for…

Computational Physics · Physics 2018-06-07 Anil Damle , Lin Lin

Efficient electronic structure methods can be built around efficient tensor representations of the wavefunction. Here we describe a general view of tensor factorization for the compact representation of electronic wavefunctions. We use…

Computational Physics · Physics 2015-05-19 Jun Yang , Yuki Kurashige , Frederick R. Manby , Garnet K. L. Chan

We present a study of the construction and spatial properties of localized Wannier orbitals in large supercells of insulating solids using plane waves as the underlying basis. The Pipek-Mezey (PM) functional in combination with intrinsic…

Chemical Physics · Physics 2025-10-22 Benjamin Wöckinger , Alexander Rumpf , Tobias Schäfer