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The nonlinear interaction between intense laser light and a quantum plasma is modeled by a collective Dirac equation coupled with the Maxwell equations. The model is used to study the nonlinear propagation of relativistically intense laser…

Plasma Physics · Physics 2015-05-28 Bengt Eliasson , Padma K. Shukla

We apply a time-dependent perturbation theory based on unitary transformations combined with averaging techniques, on molecular orientation dynamics by ultrashort pulses. We test the validity and the accuracy of this approach on LiCl…

Quantum Physics · Physics 2007-05-23 D. Sugny , A. Keller , O. Atabek , D. Daems , S. Guérin , H. R. Jauslin

We present a detailed semiclassical study on the propagation of a pair of optical fields in resonant media with and without adiabatic approximation. In the case of near and on resonance excitation, we show detailed calculation, both…

Quantum Physics · Physics 2009-11-07 M. G. Payne , L. Deng , Chris Schmitt , Shannon Anderson

Nonstationary pump-probe interaction between short laser pulses propagating in a resonant optically dense coherent medium is considered. A special attention is paid to the case, where the density of two-level particles is high enough that a…

Quantum Physics · Physics 2007-05-23 V. S. Egorov , V. N. Lebedev , I. B. Mekhov , P. V. Moroshkin , I. A. Chekhonin , S. N. Bagayev

We theoretically analyze the effectiveness of multiple-pulse laser alignment methods for asymmetric-top molecules. As an example, we choose SO_2 and investigate the alignment dynamics induced by two different sequences, each consisting of…

Atomic Physics · Physics 2010-10-01 Stefan Pabst , Robin Santra

We consider deflection of rotating symmetric molecules by inhomogeneous optical and static electric fields, compare results with the case of linear molecules, and find new singularities in the distribution of the scattering angle.…

Chemical Physics · Physics 2015-05-28 Erez Gershnabel , Ilya Sh. Averbukh

Nonlinear effects in pulse propagation through a medium consisting of four-level double-$\Lambda$-type systems are studied theoretically. We apply three continous-wave driving fields and a pulsed probe field such that they form a closed…

Quantum Physics · Physics 2009-11-13 Robert Fleischhaker , Jörg Evers

We investigate ultrafast vibronic dynamics triggered by intense femtosecond infrared pulses in small molecules. Our study is based on numerical simulations performed with 2D model molecules, and analyzed in the perspective of the renown…

This work investigates the utility of femtosecond pulse shaping in increasing the efficiency of Raman excitation of molecules in the strong-field interaction regime. We study experimentally and theoretically the effect of pulse shaping on…

Atomic Physics · Physics 2015-06-05 Martin Bitter , Evgeny A. Shapiro , Valery Milner

In ultrafast experiments with gas phase molecules, the alignment of the molecular axis relative to the polarization of the interacting laser pulses plays a crucial role in determining the dynamics following this light-matter interaction.…

Chemical Physics · Physics 2025-04-14 Shashank Kumar , Eric Liu , Liang Z. Tan , Varun Makhija , Niranjan Shivaram

We investigate fast collisions between pulsed optical beams in a linear medium with weak cubic loss that arises due to nondegenerate two-photon absorption. We introduce a perturbation method with two small parameters and use it to obtain…

Pattern Formation and Solitons · Physics 2024-01-30 Avner Peleg , Toan T. Huynh

We consider deflection of polarizable molecules by inhomogeneous optical fields, and analyze the role of molecular orientation and rotation in the scattering process. It is shown that molecular rotation induces spectacular rainbow-like…

Quantum Physics · Physics 2015-05-19 E. Gershnabel , I. Sh. Averbukh

A new perspective on how to manipulate molecules by means of very strong laser pulses is emerging with insights from the so-called light-induced potentials, which are the adiabatic potential energy surfaces of molecules severely distorted…

Chemical Physics · Physics 2016-03-03 Bo Y. Chang , Ignacio R. Sola , Seokmin Shin

The propagation of light-pulse with negative group-velocity in a nonlinear medium is studied theoretically. We show that the necessary conditions for these effects to be observable are realized in a three-level $\Lambda$-system interacting…

Classical Physics · Physics 2009-11-07 R. G. Ghulghazaryan , Yu. P. Malakyan

Raman backscattered radiation of intense laser pulses in plasma is investigated for a wide range of intensities relevant to laser wakefield acceleration. The weakly nonlinear dispersion relation for Raman backscattering predicts an…

Plasma Physics · Physics 2016-12-21 D. Kaganovich , B. Hafizi , J. P. Palastro , A. Ting , M. H. Helle , Y. -H. Chen , T. G. Jones , D. F. Gordon

We demonstrate that Freeman resonances have a strong impact on the nonlinear optical response in femtosecond filaments. These resonances decrease the transient refractive index within a narrow intensity window and strongly affect the…

Optics · Physics 2014-12-18 Michael Hofmann , Carsten Brée

An influence of pass-through optics on femtosecond laser pulse filamentation in ambient air is analyzed for the first time both experimentally and numerically. Propagation of high-power femtosecond laser pulse through solid optical elements…

Properties of filaments ignited by multi-millijoule, 90-fs mid-IR pulses centered at 3.9 {\mu}m are examined experimentally by monitoring plasma density and losses as well as spectral dynamics and beam profile evolution at different…

The uncorrelated (``sequential'') and correlated (``nonsequential'') double ionization of the H2 molecule in strong laser pulses is investigated using the tools of nonlinear dynamics. We focus on the phase-space dynamics of this system,…

Chaotic Dynamics · Physics 2009-11-30 François Mauger , Cristel Chandre , T. Uzer

Specific features of nonlinear interference processes at quantum transitions in near- and fully-resonant optically-dense Doppler-broadened medium are studied. The feasibility of overcoming of the fundamental limitation on a…

Quantum Physics · Physics 2009-11-11 A. K. Popov , S. A. Myslivets , Thomas F. George